Keldysh field theory for nonequilibrium condensation in a parametrically pumped polariton system

We develop a quantum field theory for parametrically pumped polaritons using Keldysh Green's function techniques with which the occupations of the excitation spectra can be calculated. By considering the mean field and Gaussian fluctuations, we find that the highly nonequilibrium phase transition to the optical parametric oscillator regime is in some ways similar to equilibrium condensation. In particular, we show that this phase transition can be associated with an effective chemical potential, at which the system's bosonic distribution function diverges, and an effective temperature for low energy modes. As in equilibrium systems, the transition is achieved by tuning this effective chemical potential to the energy of the lowest normal mode. Since the nonequilibrium occupations of the modes are available, we determine experimentally observable properties such as the luminescence and absorption spectra

Interactions in dye-microcavity photon condensates and the prospects for their observation

We derive the equation of motion for a Bose-Einstein condensate of photons in a dye-microcavity system, starting from Maxwell's equations. Our theory takes into account mirror shape, Kerr-type intensity-dependent refractive index and incoherent pumping and loss. The resulting equation is remarkably similar to the Gross-Pitaevskii equation for exciton-polariton condensates, despite the different microscopic origins. We calculate the incoherent photoluminescence spectrum of the photon condensate, which shows the Bogoliubov-type excitations around the mean field at thermal equilibrium. Both open- and closed-system models are presented to account for, respectively dissipation and inhomogeneities. Considering realistic parameters and experimental resolution, we estimate that by observing the angle-resolved spectrum of incoherent photoluminescence it is possible to resolve dimensionless interaction parameters of order 10 − 5 , two orders of magnitude below current estimates. Thus we expect that this technique will lead to accurate measurements of the interactions in photon condensates

Stable iPEPO Tensor-Network Algorithm for Dynamics of Two-Dimensional Open Quantum Lattice Models

Being able to accurately describe the dynamics steady states of driven and/or dissipative but quantum correlated lattice models is of fundamental importance in many areas of science: from quantum information to biology. An efficient numerical simulation of large open systems in two spatial dimensions is a challenge. In this work, we develop a tensor network method, based on an infinite projected entangled pair operator ansatz, applicable directly in the thermodynamic limit. We incorporate techniques of finding optimal truncations of enlarged network bonds by optimizing an objective function appropriate for open systems. Comparisons with numerically exact calculations, both for the dynamics and the steady state, demonstrate the power of the method. In particular, we consider dissipative transverse quantum Ising, driven-dissipative hard-core boson, and dissipative anisotropic X Y models in non-mean-field limits, proving able to capture substantial entanglement in the presence of dissipation. Our method enables us to study regimes that are accessible to current experiments but lie well beyond the applicability of existing techniques

Polariton condensation into vortex states in the synthetic magnetic field of a strained honeycomb lattice

Photonic materials are a rapidly growing platform for studying condensed matter physics with light, where the exquisite control capability is allowing us to learn about the relation between microscopic dynamics and macroscopic properties. One of the most interesting aspects of condensed matter is the interplay between interactions and the effect of an external magnetic field or rotation, responsible for a plethora of rich phenomena-Hall physics and quantized vortex arrays. At first sight, however, these effects for photons seem vetoed: they do not interact with each other and they are immune to magnetic fields and rotations. Yet in specially devised structures these effects can be engineered. Here, we propose the use of a synthetic magnetic field induced by strain in a honeycomb lattice of resonators to create a non-equilibrium Bose-Einstein condensate of light-matter particles (polaritons) in a rotating state, without the actual need for external rotation nor reciprocity-breaking elements. We show that thanks to the competition between interactions, dissipation and a suitably designed incoherent pump, the condensate spontaneously becomes chiral by selecting a single Dirac valley of the honeycomb lattice, occupying the lowest Landau level and forming a vortex array. Our results offer a new platform where to study the exciting physics of arrays of quantized vortices with light and pave the way to explore the transition from a vortex-dominated phase to the photonic analogue of the fractional quantum Hall regime

Unconventional Berezinskii-Kosterlitz-Thouless Transition in the Multicomponent Polariton System

We study a four-component polariton system in the optical parametric oscillator regime consisting of exciton, photon, signal, and idler modes across the Berezinskii-Kosterlitz-Thouless (BKT) transition. We show that all four components share the same BKT critical point, and algebraic decay of spatial coherence with the same critical exponent. However, while the collective excitations in different components are strongly locked, both close to and far from criticality, the spontaneous creation of topological defects in the vicinity of the phase transition is found to be largely independent of the intercomponent mode locking, and instead strongly dependent on the density within a given mode. This peculiar characteristic allows us to reveal a novel state of matter, characterized by configurations of topological defects proliferating on top of a superfluid with algebraic decay of coherence, observation of which is demonstrated to be within reach of current experiments

Condensation in hybrid superconducting-cavity–microscopic-spins systems with finite-bandwidth drive

Using Keldysh field theory, we find conditions for nonequilibrium condensation in the open Tavis-Cummings model under a direct finite-bandwidth incoherent cavity drive. Experimentally, we expect the condensation transition to be easily accessible to hybrid superconducting systems coupled to microscopic spins, as well as to many other incoherently driven light-matter systems. In our theoretical analysis, we explicitly incorporate the drive's spectral distribution into the saddle-point description. We show that the injected incoherent photons create a drive-dependent effective coupling between spin-1/2 particles. The condensation transition arises at a critical regime of driving which we can now accurately predict. Our results also provide important guidelines for future quantum simulation experiments of nonequilibrium phases with hybrid devices

Searching for the Kardar-Parisi-Zhang phase in microcavity polaritons

Recent approximate analytical work has suggested that, at certain values of the external pump, the optical parametric oscillator (OPO) regime of microcavity polaritons may provide a long sought realisation of Kardar-Parisi-Zhang (KPZ) physics in 2D. Here, by solving the full microscopic model numerically using the truncated Wigner method, we prove that this predicted KPZ phase for OPO is robust against the appearance of vortices or other effects. For those pump strengths, spatial correlations in the direction perpendicular to the pump, and the distribution of phase fluctuations, match closely to the forms characteristic of the KPZ universality. This strongly indicates the viability of observing KPZ behaviour in future polariton OPO experiments

First-order dissipative phase transition in an exciton-polariton condensate

We investigate the phase diagram of a two-dimensional driven-dissipative system of polaritons coupled to an excitonic reservoir. We find that two critical points exists. The first corresponds to the quasicondensation and the second to a first-order phase transition from the nonuniform state with spatially modulated density to a uniform state. The latter is related to the modulational instability of a homogeneous state due to the repulsive interactions with the noncondensed reservoir. The first-order character of the transition is evidenced by a discontinuity in the density and the correlation length as well as the phase coexistence and metastability. Moreover, we show that a signature of a Berezinskii-Kosterlitz-Thouless-like transition can be observed in the nonuniform phase

Fully Quantum Scalable Description of Driven-Dissipative Lattice Models

Methods for modeling large driven-dissipative quantum systems are becoming increasingly urgent due to recent experimental progress in a number of photonic platforms. We demonstrate the positive-P method to be ideal for this purpose across a wide range of parameters, focusing on the archetypal driven-dissipative Bose-Hubbard model. Notably, these parameters include intermediate regimes where interactions and dissipation are comparable, and especially cases with low occupations for which common semiclassical approximations can break down. The presence of dissipation can alleviate instabilities in the method that are known to occur for closed systems, allowing the simulation of dynamics up to and including the steady state. Throughout the parameter space of the model, we determine the magnitude of dissipation that is sufficient to make the method useful and stable, finding its region of applicability to be complementary to that of the truncated Wigner method. We then demonstrate its use in a number of examples with nontrivial quantum correlations, including a demonstration of solving the urgent open problem of large and highly nonuniform systems with tens of thousands of sites

Kibble-Zurek Mechanism in Driven Dissipative Systems Crossing a Nonequilibrium Phase Transition

The Kibble-Zurek mechanism constitutes one of the most fascinating and universal phenomena in the physics of critical systems. It describes the formation of domains and the spontaneous nucleation of topological defects when a system is driven across a phase transition exhibiting spontaneous symmetry breaking. While a characteristic dependence of the defect density on the speed at which the transition is crossed was observed in a vast range of equilibrium condensed matter systems, its extension to intrinsically driven dissipative systems is a matter of ongoing research. In this Letter, we numerically confirm the Kibble-Zurek mechanism in a paradigmatic family of driven dissipative quantum systems, namely exciton-polaritons in microcavities. Our findings show how the concepts of universality and critical dynamics extend to driven dissipative systems that do not conserve energy or particle number nor satisfy a detailed balance condition