572 research outputs found
Laser-induced rotation of iodine molecules in He-nanodroplets: revivals and breaking-free
Rotation of molecules embedded in He nanodroplets is explored by a
combination of fs laser-induced alignment experiments and angulon quasiparticle
theory. We demonstrate that at low fluence of the fs alignment pulse, the
molecule and its solvation shell can be set into coherent collective rotation
lasting long enough to form revivals. With increasing fluence, however, the
revivals disappear -- instead, rotational dynamics as rapid as for an isolated
molecule is observed during the first few picoseconds. Classical calculations
trace this phenomenon to transient decoupling of the molecule from its He
shell. Our results open novel opportunities for studying non-equilibrium
solute-solvent dynamics and quantum thermalization.Comment: 6+7 pages; 4+1 figures; 1 tabl
Laboratory Determination of the Infrared Band Strengths of Pyrene Frozen in Water Ice: Implications for the Composition of Interstellar Ices
Broad infrared emission features (e.g., at 3.3, 6.2, 7.7, 8.6, and 11.3
microns) from the gas phase interstellar medium have long been attributed to
polycyclic aromatic hydrocarbons (PAHs). A significant portion (10%-20%) of the
Milky Way's carbon reservoir is locked in PAH molecules, which makes their
characterization integral to our understanding of astrochemistry. In molecular
clouds and the dense envelopes and disks of young stellar objects (YSOs), PAHs
are expected to be frozen in the icy mantles of dust grains where they should
reveal themselves through infrared absorption. To facilitate the search for
frozen interstellar PAHs, laboratory experiments were conducted to determine
the positions and strengths of the bands of pyrene mixed with H2O and D2O ices.
The D2O mixtures are used to measure pyrene bands that are masked by the strong
bands of H2O, leading to the first laboratory determination of the band
strength for the CH stretching mode of pyrene in water ice near 3.25 microns.
Our infrared band strengths were normalized to experimentally determined
ultraviolet band strengths, and we find that they are generally ~50% larger
than those reported by Bouwman et al. based on theoretical strengths. These
improved band strengths were used to reexamine YSO spectra published by Boogert
et al. to estimate the contribution of frozen PAHs to absorption in the 5-8
micron spectral region, taking into account the strength of the 3.25 micron CH
stretching mode. It is found that frozen neutral PAHs contain 5%-9% of the
cosmic carbon budget, and account for 2%-9% of the unidentified absorption in
the 5-8 micron region.Comment: Accepted for publication in ApJ on 14 Feb 201
Hubble Space Telescope Observations of the HD 202628 Debris Disk
A ring-shaped debris disk around the G2V star HD 202628 (d = 24.4 pc) was imaged in scattered light at visible wavelengths using the coronagraphic mode of the Space Telescope Imaging Spectrograph on the Hubble Space Telescope. The ring is inclined by approx.64deg from face-on, based on the apparent major/minor axis ratio, with the major axis aligned along PA = 130deg. It has inner and outer radii (> 50% maximum surface brightness) of 139 AU and 193 AU in the northwest ansae and 161 AU and 223 AU in the southeast ((Delta)r/r approx. = 0.4). The maximum visible radial extent is approx. 254 AU. With a mean surface brightnesses of V approx. = 24 mag arcsec.(sup -2), this is the faintest debris disk observed to date in reflected light. The center of the ring appears offset from the star by approx.28 AU (deprojected). An ellipse fit to the inner edge has an eccentricity of 0.18 and a = 158 AU. This offset, along with the relatively sharp inner edge of the ring, suggests the influence of a planetary-mass companion. There is a strong similarity with the debris ring around Fomalhaut, though HD 202628 is a more mature star with an estimated age of about 2 Gyr. We also provide surface brightness limits for nine other stars in our study with strong Spitzer excesses around which no debris disks were detected in scattered light (HD 377, HD 7590, HD 38858, HD 45184, HD 73350, HD 135599, HD 145229, HD 187897, and HD 201219)
Debris disks around Sun-like stars
We have observed nearly 200 FGK stars at 24 and 70 microns with the Spitzer
Space Telescope. We identify excess infrared emission, including a number of
cases where the observed flux is more than 10 times brighter than the predicted
photospheric flux, and interpret these signatures as evidence of debris disks
in those systems. We combine this sample of FGK stars with similar published
results to produce a sample of more than 350 main sequence AFGKM stars. The
incidence of debris disks is 4.2% (+2.0/-1.1) at 24 microns for a sample of 213
Sun-like (FG) stars and 16.4% (+2.8/-2.9) at 70 microns for 225 Sun-like (FG)
stars. We find that the excess rates for A, F, G, and K stars are statistically
indistinguishable, but with a suggestion of decreasing excess rate toward the
later spectral types; this may be an age effect. The lack of strong trend among
FGK stars of comparable ages is surprising, given the factor of 50 change in
stellar luminosity across this spectral range. We also find that the incidence
of debris disks declines very slowly beyond ages of 1 billion years.Comment: ApJ, in pres
HST/NICMOS Imaging of Disks and Envelopes Around Very Young Stars
We present HST/NICMOS observations with 0.1" (15 AU) resolution of six young
stellar objects in the Taurus star-formation region. The targets of our survey
are three Class I IRAS sources (IRAS 04016+2610, IRAS 04248+2612, and IRAS
04302+2247) and three low-luminosity stars (DG Tau B, Haro 6-5B, and CoKu
Tau/1) associated with Herbig Haro jets. The broad-band images show that the
near-infrared radiation from these sources is dominated by light scattered from
dusty circumstellar material distributed in a region 10 - 15 times the size of
our solar system. Although the detailed morphologies of the individual objects
are unique, the observed young stellar objects share common features. All of
the circumstellar reflection nebulae are crossed by dark lanes from 500 - 900
AU in extent and from less than 50 to 350 AU in apparent thickness. The
absorption lanes extend perpendicular to known optical and millimeter outflows
in these sources. We interpret the dark lanes as optically thick circumstellar
disks seen in silhouette against bright reflection nebulosity. The bipolar
reflection nebulae extending perpendicular to the dust lanes appear to be
produced by scattering from the upper and lower surfaces of the disks and from
dusty material within or on the walls of the outflow cavities. Out of five
objects in which the central source is directly detected, two are found to be
subarcsecond binaries. This mini-survey is the highest resolution near-infrared
study to date of circumstellar environments around solar-type stars with age <=
1 Myr.Comment: 34 pages, 4 figures; also available at
http://spider.ipac.caltech.edu/staff/brandner/topics/disks/disks.html ;
accepted for publication in AJ (March 1999 issue
Hyperfine-Structure-Induced Depolarization of Impulsively Aligned Molecules
A moderately intense fs laser pulse is used to create rotational wave
packets in gas phase molecules. The ensuing time-dependent
alignment, measured by Coulomb explosion imaging with a delayed probe pulse,
exhibits the characteristic revival structures expected for rotational wave
packets but also a complex non-periodic substructure and decreasing mean
alignment not observed before. A quantum mechanical model attributes the
phenomena to coupling between the rotational angular momenta and the nuclear
spins through the electric quadrupole interaction. The calculated alignment
trace agrees very well with the experimental results.Comment: 6 pages, 4 figures, and Supplementary Information. This article has
been accepted for publication in Physical Review Letter
Control and femtosecond time-resolved imaging of torsion in a chiral molecule
We study how the combination of long and short laser pulses, can be used to
induce torsion in an axially chiral biphenyl derivative
(3,5-difluoro-3',5'-dibromo-4'-cyanobiphenyl). A long, with respect to the
molecular rotational periods, elliptically polarized laser pulse produces 3D
alignment of the molecules, and a linearly polarized short pulse initiates
torsion about the stereogenic axis. The torsional motion is monitored in
real-time by measuring the dihedral angle using femtosecond time-resolved
Coulomb explosion imaging. Within the first 4 picoseconds, torsion occurs with
a period of 1.25 picoseconds and an amplitude of 3 degrees in excellent
agreement with theoretical calculations. At larger times the quantum states of
the molecules describing the torsional motion dephase and an almost isotropic
distribution of the dihedral angle is measured. We demonstrate an original
application of covariance analysis of two-dimensional ion images to reveal
strong correlations between specific ejected ionic fragments from Coulomb
explosion. This technique strengthens our interpretation of the experimental
data.Comment: 11 pages, 9 figure
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