155 research outputs found
Continuous and Discontinuous Quantum Phase Transitions in a Model Two-Dimensional Magnet
The Shastry-Sutherland model, which consists of a set of spin 1/2 dimers on a
2-dimensional square lattice, is simple and soluble, but captures a central
theme of condensed matter physics by sitting precariously on the quantum edge
between isolated, gapped excitations and collective, ordered ground states. We
compress the model Shastry-Sutherland material, SrCu2(BO3)2, in a diamond anvil
cell at cryogenic temperatures to continuously tune the coupling energies and
induce changes in state. High-resolution x-ray measurements exploit what
emerges as a remarkably strong spin-lattice coupling to both monitor the
magnetic behavior and the absence or presence of structural discontinuities. In
the low-pressure spin-singlet regime, the onset of magnetism results in an
expansion of the lattice with decreasing temperature, which permits a
determination of the pressure dependent energy gap and the almost isotropic
spin-lattice coupling energies. The singlet-triplet gap energy is suppressed
continuously with increasing pressure, vanishing completely by 2 GPa. This
continuous quantum phase transition is followed by a structural distortion at
higher pressure.Comment: 16 pages, 4 figures. Accepted for publication in PNA
Orbital ordering transition in CaRuO observed with resonant x-ray diffraction
Resonant x-ray diffraction performed at the and
absorption edges of Ru has been used to investigate the magnetic and orbital
ordering in CaRuO single crystals. A large resonant enhancement due to
electric dipole transitions is observed at the wave-vector
characteristic of antiferromagnetic ordering. Besides the previously known
antiferromagnetic phase transition at K, an additional phase
transition, between two paramagnetic phases, is observed around 260 K. Based on
the polarization and azimuthal angle dependence of the diffraction signal, this
transition can be attributed to orbital ordering of the Ru electrons.
The propagation vector of the orbital order is inconsistent with some
theoretical predictions for the orbital state of CaRuO.Comment: to appear in PR
Recommended from our members
A comparison of an elliptical multipole wiggler and crystal optics for the production of circularly polarized x-rays
Recently, there has been a great deal of interest in polarization modulated x-ray diffraction and spectroscopy techniques. In particular, the importance of photon helicity in spin-dependent magnetic interactions has expanded the need for high quality circularly polarized x-ray sources with fast switching capabilities. Because circularly polarized photons couple differently with the magnetic moment of an atom than do neutrons, they are able to provide unique magnetic information not accessible by neutron techniques. The development of experiments utilizing circularly polarized x-rays, however, has been hampered by the lack of efficient sources. Two different approaches for the production of circularly polarized x-rays have attracted the most attention; (i) employing specialized insertion devices, and (ii) utilizing x-ray phase retarders based on perfect crystal optics. For soft x-rays (0.1--3.0 keV), source development has centered primarily on insertion devices because there are currently no crystal or multilayer polarizing optics available that cover that full energy range. For harder x-rays (>3.0 keV), however, phase retarding optics have been demonstrated, but whether these optics or insertion devices provide the most efficient circularly polarized x-ray source in this energy regime has remained a matter of contention. Advocates of each method have made qualitative statements about their advantages, i.e., insertion devices provide a larger flux and phase retarders provide a higher degree of circular polarization, yet a detailed quantitative comparison has been lacking. In this paper, we attempt to provide such a comparison by examining the efficiencies of an elliptical multipole wiggler (EMW) and a standard undulator followed by phase retarding crystal optics
Chromium at High Pressures: Weak Coupling and Strong Fluctuations in an Itinerant Antiferromagnet
The spin- and charge-density-wave order parameters of the itinerant
antiferromagnet chromium are measured directly with non-resonant x-ray
diffraction as the system is driven towards its quantum critical point with
high pressure using a diamond anvil cell. The exponential decrease of the spin
and charge diffraction intensities with pressure confirms the harmonic scaling
of spin and charge, while the evolution of the incommensurate ordering vector
provides important insight into the difference between pressure and chemical
doping as means of driving quantum phase transitions. Measurement of the charge
density wave over more than two orders of magnitude of diffraction intensity
provides the clearest demonstration to date of a weakly-coupled, BCS-like
ground state. Evidence for the coexistence of this weakly-coupled ground state
with high-energy excitations and pseudogap formation above the ordering
temperature in chromium, the charge-ordered perovskite manganites, and the blue
bronzes, among other such systems, raises fundamental questions about the
distinctions between weak and strong coupling.Comment: 11 pages, 9 figures (8 in color
Iterated Moire Maps and Braiding of Chiral Polymer Crystals
In the hexagonal columnar phase of chiral polymers a bias towards cholesteric
twist competes with braiding along an average direction. When the chirality is
strong, screw dislocations proliferate, leading to either a tilt grain boundary
phase or a new "moire state" with twisted bond order. Polymer trajectories in
the plane perpendicular to their average direction are described by iterated
moire maps of remarkable complexity.Comment: 10 pages (plain tex) 3 figures uufiled and appende
Magnetic Structure Of Sm2 Ir In8 Determined By X-ray Resonant Magnetic Scattering
The magnetic structure of the intermetallic antiferromagnet Sm2 Ir In8 was determined using x-ray resonant magnetic scattering. Below TN =14.2 K, Sm2 Ir In8 has a commensurate antiferromagnetic structure with a propagation vector η = (12,0,0). The Sm magnetic moments lie in the ab plane and are rotated roughly 18° away from the a axis. The magnetic structure of this compound was obtained by measuring the strong dipolar resonant peak whose enhancement was of over 2 orders of magnitude at the L2 edge. At the L3 edge, both quadrupolar and dipolar features were observed in the energy line shape. The magnetic structure and properties of Sm2 Ir In8 are found to be consistent with the general trend already seen for the Nd-, Tb-, and the Ce-based compounds from the Rm Mn In3m+2n family (R=rare earth; M=Rh or Ir; m=1,2; n=0,1), where the crystalline electrical field effects determine the direction of magnetic moments and the TN evolution in the series. The measured Néel temperature for Sm2 Ir In8 is slightly suppressed when compared to the TN of the parent cubic compound Sm In3. © 2007 The American Physical Society.7610Hegger, H., Petrovic, C., Moshopoulou, E.G., Hundley, M.F., Sarrao, J.L., Fisk, Z., Thompson, J.D., (2000) Phys. Rev. Lett., 84, p. 4986. , PRLTAO 0031-9007 10.1103/PhysRevLett.84.4986Petrovic, C., Movshovich, R., Jaime, M., Pagliuso, P.G., Hundley, M.F., Sarrao, J.L., Thompson, J.D., Fisk, Z., (2001) Europhys. Lett., 354-359, p. 4986. , EULEEJ 0295-5075Petrovic, C., Pagliuso, P.G., Hundley, M.F., Movshovich, R., Sarrao, J.L., Thompson, J.D., Fisk, Z., Monthoux, P., (2001) J. Phys.: Condens. Matter, 13, p. 337. , JCOMEL 0953-8984 10.1088/0953-8984/13/17/103Thompson, J.D., (2001) J. Magn. Magn. Mater., 226-230, p. 5. , JMMMDC 0304-8853Pagliuso, P.G., Thompson, J.D., Hundley, M.F., Sarrao, J.L., Fisk, Z., (2001) Phys. Rev. B, 63, p. 054426. , PRBMDO 0163-1829 10.1103/PhysRevB.63.054426Pagliuso, P.G., Thompson, J.D., Hundley, M.F., Sarrao, J.L., (2000) Phys. Rev. B, 62, p. 12266. , PRBMDO 0163-1829 10.1103/PhysRevB.62.12266Lora-Serrano, R., Giles, C., Granado, E., Garcia, D.J., Miranda, E., Agüero, O., Mendonça Ferreira, L., Pagliuso, P.G., (2006) Phys. Rev. B, 74, p. 214404. , PRBMDO 0163-1829 10.1103/PhysRevB.74.214404Chen, G., Ohara, S., Hedo, M., Uwatoko, Y., Saito, K., Sorai, M., Sakamoto, I., (2002) J. Phys. Soc. Jpn., 71, p. 2836. , JUPSAU 0031-9015 10.1143/JPSJ.71.2836Moshopoulou, E.G., Fisk, Z., Sarrao, J.L., Thompson, J.D., (2001) J. Solid State Chem., 158, p. 25. , JSSCBI 0022-4596 10.1006/jssc.2000.9052Moshopoulou, E.G., Ibberson, R.M., Sarrao, J.L., Thompson, J.D., Fisk, Z., (2006) Acta Crystallogr., Sect. B: Struct. Sci., 62, p. 173. , ASBSDK 0108-7681Buschow, K.H.J., De Wijn, H.W., Van Diepen, A.M., (1969) J. Chem. Phys., 50, p. 137. , JCPSA6 0021-9606 10.1063/1.1670771Pagliuso, P.G., Petrovic, C., Movshovich, R., Hall, D., Hundley, M.F., Sarrao, J.L., Thompson, J.D., Fisk, Z., (2001) Phys. Rev. B, 64, p. 100503. , PRBMDO 0163-1829 10.1103/PhysRevB.64.100503Pagliuso, P.G., Movshovich, R., Bianchi, A.D., Nicklas, M., Thompson, J.D., Hundley, M.F., Sarrao, J.L., Fisk, Z., (2002) Physica B, 312-313, p. 129. , PHYBE3 0921-4526Pham, L.D., Park, T., Maquilon, S., Thompson, J.D., Fisk, Z., (2006) Phys. Rev. Lett., 97, p. 056404. , PRLTAO 0031-9007 10.1103/PhysRevLett.97.056404Zapf, V.S., Freeman, E.J., Bauer, E.D., Petricka, J., Sirvent, C., Frederick, N.A., Dickey, R.P., Maple, M.B., (2001) Phys. Rev. B, 65, p. 014506. , PRBMDO 0163-1829 10.1103/PhysRevB.65.014506Park, T., Ronning, F., Yuan, H.Q., Salamon, M.B., Movshovich, R., Sarrao, J.L., Thompson, J.D., (2006) Nature (London), 440, p. 65. , NATUAS 0028-0836 10.1038/nature04571Sidorov, V.A., Nicklas, M., Pagliuso, P.G., Sarrao, J.L., Bang, Y., Balatsky, A.V., Thompson, J.D., (2002) Phys. Rev. Lett., 89, p. 157004. , PRLTAO 0031-9007 10.1103/PhysRevLett.89.157004Bianchi, A., Movshovich, R., Vekhter, I., Pagliuso, P.G., Sarrao, J.L., (2003) Phys. Rev. Lett., 91, p. 257001. , PRLTAO 0031-9007 10.1103/PhysRevLett.91.257001Bauer, E.D., Capan, C., Ronning, F., Movshovich, R., Thompson, J.D., Sarrao, J.L., (2005) Phys. Rev. Lett., 94, p. 047001. , PRLTAO 0031-9007 10.1103/PhysRevLett.94.047001Paglione, J., Tanatar, M.A., Hawthorn, D.G., Boaknin, E., Hill, R.W., Ronning, F., Sutherland, M., Canfield, P.C., (2003) Phys. Rev. Lett., 91, p. 246405. , PRLTAO 0031-9007 10.1103/PhysRevLett.91.246405Kumar, R.S., Cornelius, A.L., Sarrao, J.L., (2004) Phys. Rev. B, 70, p. 214526. , PRBMDO 0163-1829 10.1103/PhysRevB.70.214526Oeschler, N., Gegenwart, P., Lang, M., Movshovich, R., Sarrao, J.L., Thompson, J.D., Steglich, F., (2003) Phys. Rev. Lett., 91, p. 076402. , PRLTAO 0031-9007 10.1103/PhysRevLett.91.076402Christianson, A.D., (2004) Phys. Rev. B, 70, p. 134505. , PRBMDO 0163-1829 10.1103/PhysRevB.70.134505Harrison, N., (2004) Phys. Rev. Lett., 93, p. 186405. , PRLTAO 0031-9007 10.1103/PhysRevLett.93.186405Raj, S., (2005) Phys. Rev. B, 71, p. 224516. , PRBMDO 0163-1829 10.1103/PhysRevB.71.224516Hall, D., Palm, E.C., Murphy, T.P., Tozer, S.W., Fisk, Z., Alver, U., Goodrich, R.G., Ebihara, T., (2001) Phys. Rev. B, 64, p. 212508. , PRBMDO 0163-1829 10.1103/PhysRevB.64.212508Hall, D., (2001) Phys. Rev. B, 64, p. 064506. , PRBMDO 0163-1829 10.1103/PhysRevB.64.064506Costa-Quintana, J., López-Aguilar, F., (2003) Phys. Rev. B, 67, p. 132507. , PRBMDO 0163-1829 10.1103/PhysRevB.67.132507Sarrao, J.L., Morales, L.A., Thompson, J.D., Scott, B.L., Stewart, G.R., Wastin, F., Rebizant, J., Lander, G.H., (2002) Nature (London), 420, p. 297. , NATUAS 0028-0836 10.1038/nature01212Bauer, E.D., (2004) Phys. Rev. Lett., 93, p. 147005. , PRLTAO 0031-9007 10.1103/PhysRevLett.93.147005Christianson, A.D., (2005) Phys. Rev. Lett., 95, p. 217002. , PRLTAO 0031-9007 10.1103/PhysRevLett.95.217002Lora-Serrano, R., Mendonça Ferreira, L., Garcia, D.J., Miranda, E., Giles, C., Duque, J.G.S., Granado, E., Pagliuso, P.G., (2006) Physica B, 384, p. 326. , PHYBE3 0921-4526 10.1016/j.physb.2006.06.035Hieu, N.V., (2006) J. Phys. Soc. Jpn., 75, p. 074708. , JUPSAU 0031-9015Malinowski, A., Hundley, M.F., Moreno, N.O., Pagliuso, P.G., Sarrao, J.L., Thompson, J.D., (2003) Phys. Rev. B, 68, p. 184419. , PRBMDO 0163-1829 10.1103/PhysRevB.68.184419Correa, V.F., Tung, L., Hollen, S.M., Pagliuso, P.G., Moreno, N.O., Lashley, J.C., Sarrao, J.L., Lacerda, A.H., (2004) Phys. Rev. B, 69, p. 174424. , PRBMDO 0163-1829 10.1103/PhysRevB.69.174424Granado, E., Pagliuso, P.G., Giles, C., Lora-Serrano, R., Yokaichiya, F., Sarrao, J.L., (2004) Phys. Rev. B, 69, p. 144411. , PRBMDO 0163-1829 10.1103/PhysRevB.69.144411Pagliuso, P.G., (2006) J. Appl. Phys., 99, pp. 08P703. , JAPIAU 0021-8979 10.1063/1.2176109Bao, W., Pagliuso, P.G., Sarrao, J.L., Thompson, J.D., Fisk, Z., Lynn, J.W., Erwin, R.W., (2000) Phys. Rev. B, 62, p. 14621. , PRBMDO 0163-1829 10.1103/PhysRevB.62.R14621Bao, W., Pagliuso, P.G., Sarrao, J.L., Thompson, J.D., Fisk, Z., Lynn, J.W., Erwin, R.W., (2001) Phys. Rev. B, 63, p. 219901. , PRBMDO 0163-1829 10.1103/PhysRevB.63.219901Bao, W., Pagliuso, P.G., Sarrao, J.L., Thompson, J.D., Fisk, Z., Lynn, J.W., (2001) Phys. Rev. B, 64, p. 020401. , PRBMDO 0163-1829 10.1103/PhysRevB.64.020401Chang, S., Pagliuso, P.G., Bao, W., Gardner, J.S., Swainson, I.P., Sarrao, J.L., Nakotte, H., (2002) Phys. Rev. B, 66, p. 132417. , PRBMDO 0163-1829 10.1103/PhysRevB.66.132417Granado, E., Uchoa, B., Malachias, A., Lora-Serrano, R., Pagliuso, P.G., Westfahl Jr., H., (2006) Phys. Rev. B, 74, p. 214428. , PRBMDO 0163-1829 10.1103/PhysRevB.74.214428Kasaya, M., Liu, B., Sera, M., Kasuya, T., Endoh, D., Goto, T., Fujimura, F., (1985) J. Magn. Magn. Mater., 52, p. 289. , JMMMDC 0304-8853 10.1016/0304-8853(85)90282-3Endoh, D., Goto, T., Tamaki, A., Liu, B., Kasaya, M., Fujimura, T., Kasuya, T., (1989) J. Phys. Soc. Jpn., 58, p. 940. , JUPSAU 0031-9015Kletowski, Z., (1998) J. Magn. Magn. Mater., 186, p. 7. , JMMMDC 0304-8853Stunault, A., Dumesnil, K., Dufour, C., Vettier, C., Bernhoeft, N., (2002) Phys. Rev. B, 65, p. 064436. , PRBMDO 0163-1829 10.1103/PhysRevB.65.064436Fisk, Z., Remeika, J.P., (1989) Handbook on the Physics and Chemistry of Rare Earths, 12, p. 53. , edited by J. K. A. Geschneider and E. L. Eyring (Elsevier, Amsterdam/ North-Holland, AmsterdamPaolasini, L., (2007) J. Synchrotron Radiat., 14, p. 301. , JSYRES 0909-0495Hill, J.P., McMorrow, D.F., (1996) Acta Crystallogr., Sect. A: Found. Crystallogr., 52, p. 236. , ACACEQ 0108-7673 10.1107/S0108767395012670Zheludev, A., Hill, J.P., Buttrey, D.J., (1996) Phys. Rev. B, 54, p. 7216. , PRBMDO 0163-1829 10.1103/PhysRevB.54.7216Hill, J.P., Vigliante, A., Gibbs, D., Peng, J.L., Greene, R.L., (1995) Phys. Rev. B, 52, p. 6575. , PRBMDO 0163-1829 10.1103/PhysRevB.52.6575Detlefs, C., Islam, A.H.M.Z., Goldman, A.I., Stassis, C., Canfield, P.C., Hill, J.P., Gibbs, D., (1997) Phys. Rev. B, 55, p. 680. , PRBMDO 0163-1829 10.1103/PhysRevB.55.R680Hannon, J.P., Trammell, G.T., Blume, M., Gibbs, D., (1988) Phys. Rev. Lett., 61, p. 1245. , PRLTAO 0031-9007 10.1103/PhysRevLett.61.1245Blume, M., Gibbs, D., (1988) Phys. Rev. B, 37, p. 1779. , PRBMDO 0163-1829 10.1103/PhysRevB.37.1779Kubo, K., Hotta, T., (2006) J. Phys. Soc. Jpn., 75, p. 083702. , JUPSAU 0031-9015 10.1143/JPSJ.75.083702Tsuchida, T., Wallace, W.E., (1965) J. Chem. Phys., 43, p. 3811. , JCPSA6 0021-9606 10.1063/1.169656
A 4-unit-cell superstructure in optimally doped YBa2Cu3O6.92 superconductor
Using high-energy diffraction we show that a 4-unit-cell superstructure,
q0=(1/4,0,0), along the shorter Cu-Cu bonds coexists with superconductivity in
optimally doped YBCO. A complex set of anisotropic atomic displacements on
neighboring CuO chain planes, BaO planes, and CuO2 planes, respectively,
correlated over ~3-6 unit cells gives rise to diffuse superlattice peaks. Our
observations are consistent with the presence of Ortho-IV nanodomains
containing these displacements.Comment: Corrected typo in abstrac
- …