Spin wave stiffness and exchange stiffness of doped permalloy via ab-initio calculation

The way doping affects the spin wave stiffness and the exchange stiffness of permalloy (Py) is investigated via ab-initio calculations, using the Korringa-Kohn-Rostoker (KKR) Green function formalism. By considering various types of dopants of different nature (V, Gd, and Pt), we are able to draw general conclusions. To describe the trends of the stiffness with doping is it sufficient to account for the exchange coupling between nearest neighbors. The polarizability of the impurities is not an important factor for the spin wave stiffness. Rather, the decisive factor is the hybridization between the impurity and the host states as reflected by changes in the Bloch spectral function. Our theoretical results agree well with earlier experiments.Comment: 8 figures, 5 table

The challenges of change:Exploring the dynamics of police reform in Scotland

Despite a long tradition of pessimism regarding the scope for meaningful change in police practices, recent structural reforms to police organizations in several European countries suggest that significant change in policing is possible. Drawing on recent research into the establishment and consequences of a national police force in Scotland, this article uses instrumental, cultural and myth perspectives taken from organization theory to examine how change happened and with what effects. It highlights how police reform involves a complex interplay between the strategic aims of government, the cultural norms of police organizations and the importance of alignment with wider views about the nature of the public sector. The article concludes by identifying a set of wider lessons from the experience of organizational change in policing

Single 3dd transition metal atoms on multi-layer graphene systems: electronic configurations, bonding mechanisms and role of the substrate

The electronic configurations of Fe, Co, Ni, and Cu adatoms on graphene and graphite have been studied by x-ray magnetic circular dichroism and charge transfer multiplet theory. A delicate interplay between long-range interactions and local chemical bonding is found to influence the adatom equilibrium distance and magnetic moment. The results for Fe and Co are consistent with purely physisorbed species having, however, different 3$d$-shell occupancies on graphene and graphite ($d^{n+1}$ and $d^n$, respectively). On the other hand, for the late 3$d$ metals Ni and Cu a trend towards chemisorption is found, which strongly quenches the magnetic moment on both substrates.Comment: 7 pages, 4 figure

Nonequilibrium Josephson-like effects in wide mesoscopic S-N-S junctions

Mesoscopic superconducting-normal-metal-superconducting (S-N-S) junctions with a large separation between the superconducting electrodes (i.e. wide junctions) exhibit nonequilibrium supercurrents, even at temperatures for which the equilibrium Josephson effect is exponentially small. The second harmonic of the Josephson frequency dominates these currents, as observed in recent experiments. A simple description of these effects, in the spirit of the Resistively-Shunted-Junction model, is suggested here. It is used to calculate dc I-V characteristics, and to examine the effects of various types of noise and of external microwave radiation (Shapiro steps). It is found that the nonequilibrium supercurrents are excited when the junction is driven by a dc bias or an ac bias, or even by external noise. In the case of junctions which are also long in the direction perpendicular to the current flow, thermodynamic phase fluctuations (thermal noise) alone can drive the quasiparticles out of local equilibrium. Magnetic flux is then predicted to be trapped in units of Phi_0 /2 = hc/4e.Comment: 10 pages, to appear in a special issue of Superlattices & Microstructure

Proximity Effect, Andreev Reflections, and Charge Transport in Mesoscopic Superconducting-Semiconducting Heterostructures

In the quasi-twodimensional (Q2D) electron gas of an InAs channel between an AlSb substrate and superconducting Niobium layers the proximity effect induces a pair potential so that a Q2D mesoscopic superconducting-normal-superconducting (SNS) junction forms in the channel. The pair potential is calculated with quasiclassical Green's functions in the clean limit. For such a junction alternating Josephson currents and current-voltage characteristics (CVCs) are computed, using the non-equilibrium quasiparticle wavefunctions which solve the time-dependent Bogoliubov-de Gennes Equations. The CVCs exhibit features found experimentally by the Kroemer group: A steep rise of the current at small voltages ("foot") changes at a "corner current" to a much slower increase of current with higher voltages, and the zero-bias differential resistance increases with temperature. Phase-coherent multiple Andreev reflections and the associated Cooper pair transfers are the physical mechanisms responsible for the oscillating Josephson currents and the CVCs. Additional experimental findings not reproduced by the theory require model improvements, especially a consideration of the external current leads which should give rise to hybrid quasiparticle/collective mode excitations.Comment: 8 pages, 4 figures (consisting of 5 .ps-files), added referenc

Finite-temperature magnetism of Fex_xPd1−x_{1-x} and Cox_xPt1−x_{1-x} alloys

The finite-temperature magnetic properties of Fe$_x$Pd$_{1-x}$ and Co$_x$Pt$_{1-x}$ alloys have been investigated. It is shown that the temperature-dependent magnetic behaviour of alloys, composed of originally magnetic and non-magnetic elements, cannot be described properly unless the coupling between magnetic moments at magnetic atoms (Fe,Co) mediated through the interactions with induced magnetic moments of non-magnetic atoms (Pd,Pt) is included. A scheme for the calculation of the Curie temperature ($T_C$) for this type of systems is presented which is based on the extended Heisenberg Hamiltonian with the appropriate exchange parameters $J_{ij}$ obtained from {\em ab-initio} electronic structure calculations. Within the present study the KKR Green's function method has been used to calculate the $J_{ij}$ parameters. A comparison of the obtained Curie temperatures for Fe$_x$Pd$_{1-x}$ and Co$_x$Pt$_{1-x}$ alloys with experimental data shows rather good agreement.Comment: 10 pages, 12 figure

Assessing different approaches to ab initio calculations of spin wave stiffness

Ab initio calculations of the spin wave stiffness constant $D$ for elemental Fe and Ni performed by different groups in the past have led to values with a considerable spread of 50-100 %. We present results for the stiffness constant $D$ of Fe, Ni, and permalloy Fe$_{0.19}$Ni$_{0.81}$ obtained by three different approaches: (i) by finding the quadratic term coefficient of the power expansion of the spin wave energy dispersion, (ii) by a damped real-space summation of weighted exchange coupling constants, and (iii) by integrating the appropriate expression in reciprocal space. All approaches are implemented by means of the same Korringa-Kohn-Rostoker (KKR) Green function formalism. We demonstrate that if properly converged, all procedures yield comparable values, with uncertainties of 5-10 % remaining. By a careful analysis of the influence of various technical parameters we estimate the margin of errors for the stiffness constants evaluated by different approaches and suggest procedures to minimize the risk of getting incorrect results.Comment: 11 pages, 7 figures, 12 table