1 research outputs found
Large Magnetoresistance and Jahn Teller effect in SrFeCoO
Neutron diffraction measurement on the spin glass double perovskite
SrFeCoO reveals site disorder as well as Co intermediate spin
state. In addition, multiple valence states of Fe and Co are confirmed through
M\"{o}ssbauer and X-ray photoelectron spectroscopy. The structural disorder and
multiple valence lead to competing ferromagnetic and antiferromagnetic
interactions and subsequently to a spin glass state, which is reflected in the
form of an additional -linear contribution at low temperatures in specific
heat. A clear evidence of Jahn-Teller distortion at the Co-O complex
is observed and incorporating the physics of Jahn-Teller effect, the presence
of localized magnetic moment is shown. A large, negative and anomalous
magnetoresistance of 63% at 14K in 12T applied field is observed for
SrFeCoO. The observed magnetoresistance could be explained by applying
a semi-empirical fit consisting of a negative and a positive contribution and
show that the negative magnetoresistance is due to spin scattering of carriers
by localized magnetic moments in the spin glass phase