Characterization of atmospheric aerosol optical properties based on the combined use of a ground-based Raman lidar and an airborne optical particle counter in the framework of the Hydrological Cycle in the Mediterranean Experiment – Special Observation Period 1

Abstract. Vertical profiles of the particle backscattering coefficient at 355, 532 and 1064 nm measured by the University of Basilicata Raman lidar system (BASIL) have been compared with simulated particle backscatter profiles obtained through a Mie scattering code based on the use of simultaneous and almost co-located profiles provided by an airborne optical particle counter. Measurements were carried out during dedicated flights of the French research aircraft ATR42 in the framework of the European Facility for Airborne Research (EUFAR) project "WaLiTemp", as part of the Hydrological Cycle in the Mediterranean Experiment – Special Observation Period 1 (HyMeX-SOP1). Results from two selected case studies are reported and discussed in the paper, and a dedicated analysis approach is illustrated and applied to the dataset. Results reveal a good agreement between measured and simulated multi-wavelength particle backscattering profiles. Specifically, simulated and measured particle backscattering profiles at 355 and 532 nm for the second case study are found to deviate less than 15 % (mean value =5.9 %) and 50 % (mean value =25.9 %), respectively, when considering the presence of a continental–urban aerosol component, while slightly larger deviation values are found for the first study. The reported good agreement between measured and simulated multi-wavelength particle backscatter profiles testifies to the ability of multi-wavelength Raman lidar systems to infer aerosol types at different altitudes

Clear-air lidar dark band

This paper illustrates measurements carried out by the Raman lidar BASIL in the frame of HOPE, revealing the presence of a clear-air dark band phenomenon (i.e. the appearance of a minimum in lidar backscatter echoes) in the upper portion of the convective boundary layer. The phenomenon is clearly distinguishable in the lidar backscatter echoes at 1064 nm. This phenomenon is attributed to the presence of lignite aerosol particles advected from the surrounding open pit mines in the vicinity of the measuring site

Clear-air lidar dark band

Abstract. This paper illustrates measurements carried out by the Raman lidar BASIL in the frame of the HD(CP)2 Observational Prototype Experiment (HOPE), revealing the presence of a clear-air dark band phenomenon (i.e. a minimum in lidar backscatter echoes) in the upper portion of the convective boundary layer. The phenomenon is clearly distinguishable in the lidar backscatter echoes at 532 and 1064 nm, as well as in the particle depolarisation data. This phenomenon is attributed to the presence of lignite aerosol particles advected from the surrounding open pit mines in the vicinity of the measuring site. The paper provides evidence of the phenomenon and illustrates possible interpretations for its occurrence

Characterisation of boundary layer turbulent processes by the Raman lidar BASIL in the frame of HD(CP) 2 Observational Prototype Experiment

Abstract. Measurements carried out by the University of Basilicata Raman lidar system (BASIL) are reported to demonstrate the capability of this instrument to characterise turbulent processes within the convective boundary layer (CBL). In order to resolve the vertical profiles of turbulent variables, high-resolution water vapour and temperature measurements, with a temporal resolution of 10 s and vertical resolutions of 90 and 30 m, respectively, are considered. Measurements of higher-order moments of the turbulent fluctuations of water vapour mixing ratio and temperature are obtained based on the application of autocovariance analyses to the water vapour mixing ratio and temperature time series. The algorithms are applied to a case study (11:30–13:30 UTC, 20 April 2013) from the High Definition Clouds and Precipitation for Climate Prediction (HD(CP)2) Observational Prototype Experiment (HOPE), held in western Germany in the spring 2013. A new correction scheme for the removal of the elastic signal crosstalk into the low quantum number rotational Raman signal is applied. The noise errors are small enough to derive up to fourth-order moments for both water vapour mixing ratio and temperature fluctuations.To the best of our knowledge, BASIL is the first Raman lidar with a demonstrated capability to simultaneously retrieve daytime profiles of water vapour turbulent fluctuations up to the fourth order throughout the atmospheric CBL. This is combined with the capability of measuring daytime profiles of temperature fluctuations up to the fourth order. These measurements, in combination with measurements from other lidar and in situ systems, are important for verifying and possibly improving turbulence and convection parameterisation in weather and climate models at different scales down to the grey zone (grid increment  ∼  1 km; Wulfmeyer et al., 2016).For the considered case study, which represents a well-mixed and quasi-stationary CBL, the mean boundary layer height is found to be 1290 ± 75 m above ground level (a.g.l.). Values of the integral scale for water vapour and temperature fluctuations at the top of the CBL are in the range of 70–125 and 75–225 s, respectively; these values are much larger than the temporal resolution of the measurements (10 s), which testifies that the temporal resolution considered for the measurements is sufficiently high to resolve turbulent processes down to the inertial subrange and, consequently, to resolve the major part of the turbulent fluctuations. Peak values of all moments are found in the interfacial layer in the proximity of the top of the CBL. Specifically, water vapour and temperature second-order moments (variance) have maximum values of 0.29 g2 kg−2 and 0.26 K2; water vapour and temperature third-order moments have peak values of 0.156 g3 kg−3 and −0.067 K3, while water vapour and temperature fourth-order moments have maximum values of 0.28 g4 kg−4 and 0.24 K4. Water vapour and temperature kurtosis have values of  ∼  3 in the upper portion of the CBL, which indicate normally distributed humidity and temperature fluctuations. Reported values of the higher-order moments are in good agreement with previous measurements at different locations, thus providing confidence in the possibility of using these measurements for turbulence parameterisation in weather and climate models.In the determination of the temperature profiles, particular care was dedicated to minimise potential effects associated with elastic signal crosstalk on the rotational Raman signals. For this purpose, a specific algorithm was defined and tested to identify and remove the elastic signal crosstalk and to assess the residual systematic uncertainty affecting temperature measurements after correction. The application of this approach confirms that, for the present Raman lidar system, the crosstalk factor remains constant with time; consequently an appropriate assessment of its constant value allows for a complete removal of the leaking elastic signal from the rotational Raman lidar signals at any time (with a residual error on temperature measurements after correction not exceeding 0.18 K)

Comparison of Antarctic polar stratospheric cloud observations by ground-based and space-borne lidar and relevance for chemistry–climate models

Abstract. A comparison of polar stratospheric cloud (PSC) occurrence from 2006 to 2010 is presented, as observed from the ground-based lidar station at McMurdo (Antarctica) and by the satellite-borne CALIOP lidar (Cloud-Aerosol Lidar with Orthogonal Polarization) measuring over McMurdo. McMurdo (Antarctica) is one of the primary lidar stations for aerosol measurements of the NDACC (Network for Detection of Atmospheric Climate Change). The ground-based observations have been classified with an algorithm derived from the recent v2 detection and classification scheme, used to classify PSCs observed by CALIOP. A statistical approach has been used to compare ground-based and satellite-based observations, since point-to-point comparison is often troublesome due to the intrinsic differences in the observation geometries and the imperfect overlap of the observed areas. A comparison of space-borne lidar observations and a selection of simulations obtained from chemistry–climate models (CCMs) has been made by using a series of quantitative diagnostics based on the statistical occurrence of different PSC types. The distribution of PSCs over Antarctica, calculated by several CCMVal-2 and CCMI chemistry–climate models has been compared with the PSC coverage observed by the satellite-borne CALIOP lidar. The use of several diagnostic tools, including the temperature dependence of the PSC occurrences, evidences the merits and flaws of the different models. The diagnostic methods have been defined to overcome (at least partially) the possible differences due to the resolution of the models and to identify differences due to microphysics (e.g., the dependence of PSC occurrence on T−TNAT). A significant temperature bias of most models has been observed, as well as a limited ability to reproduce the longitudinal variations in PSC occurrences observed by CALIOP. In particular, a strong temperature bias has been observed in CCMVal-2 models with a strong impact on PSC formation. The WACCM-CCMI (Whole Atmosphere Community Climate Model – Chemistry-Climate Model Initiative) model compares rather well with the CALIOP observations, although a temperature bias is still present

Misure di profili verticali di umidità e backscattering aerosolico nel centro urbano di Roma in orario diurno e notturno mediante tecnica LIDAR

Nella tesi viene illustrata la progettazione di un LIDAR (LIght Detection And Ranging) Raman- Elastico, ne verranno descritte le componenti e l’assemblaggio, saranno mostrati i test dei canali, e saranno presi in considerazione dei casi studio. Lo scopo di questo studio è quello di fornire uno strumento per l’osservazione del planetary boundary layer (PBL) e degli effetti atmosferici ad esso correlato all’interno del centro abitato di Roma. In particolare è interessante dal punto di vista scientifico ed è utile dal punto di vista pratico studiare l’effetto dell’isola di calore urbano. Accade infatti che il fenomeno di urbanizzazione tenda a modificare il clima locale e a causare effetti che abbiano ricadute anche sulla qualità della vita delle persone che abitano in quella regione: viene amplificata la presenza delle ondate di caldo e di inquinanti poiché al riscaldamento dovuto alla radiazione solare incidente, si somma il calore generato da fonti antropogeniche.Inoltre l’alta densità di abitanti per kilometro, tipica dei centri urbani, richiede una produzione maggiore rispetto a quella che è necessaria nelle zone circostanti, di energia elettrica e meccanica che determina un aumento del rilascio dei gas serra. L’oggetto centrale di questa tesi è lo strumento LIDAR Raman-Elastico: i prodotti forniti da questo strumento sono i profili verticali di due parametri essenziali per lo studio del PBL come umidità e quantitativo di aerosol. Il carattere innovativo della ricerca risiede nel fatto che per la prima volta si rende possibile l’acquisizione in un’area urbana di profili verticali di vapore acqueo ad alta risoluzione sia verticale che temporale durante le ore diurne in cui si ha il massimo sviluppo del PBL e in cui si innestano i processi convettivi che rimescolano l’atmosfera nei primi strati. Inoltre questo studio è inquadrato in un progetto più ampio in cui è coinvolta l’ESA (European Space Agency). Tale progetto prevede l’allestimento di strumentazione per osservazioni atmosferiche concentrate in un grande supersite denominato BAQUNIN (Boundary layer Air Quality-analysis Using Network of INstruments): il sito è situato all’interno della zona urbana di Roma (l’edificio Fermi del dipartimento di Fisica, luogo dove ho svolto la mia attività di dottorato). Sempre in questo ambito vi è anche la collaborazione con il CNR – ISAC che gestisce il supersite CIRAS (CNR Isac Rome Atmospheric Supersite) a Tor Vergata. Nell’immediato futuro, il carattere urbano e semirurale dei due siti renderà possibile effettuare studi riguardo l’influenza sui parametri atmosferici da parte dell’azione antropologica ed inoltre sarà possibile caratterizzare i due supersite come centri di calibrazione e validazione di dati acquisiti da satellite. La tesi si svilupperà su sei capitoli di cui ora verrà data una breve descrizione:  Nel primo si presenteranno i fenomeni atmosferici che si vogliono studiare e si daranno le motivazioni per le quali è importante intraprendere questa ricerca.  Nel secondo capitolo si descriveranno i principi di funzionamento di un LIDAR Raman- Elastico, si simuleranno i segnali che si vorrebbero acquisire dal sistema e si descriverà il sistema LIDAR presente in laboratorio prima dell’inizio del lavoro di tesi mettendone in risalto le inadeguatezze ad effettuare le misure che ci si propone di fare in questo contesto.  Nel terzo capitolo verranno dimensionati i parametri usati per simulare i segnali nel capitolo precedente in base alle componenti utilizzate, si giustificheranno le scelte delle componenti del sistema LIDAR e solo dopo una breve descrizione dell’assemblaggio, verranno simulati di nuovo i segnali aspettati inserendo i nuovi parametri.Il quarto capitolo sarà il capitolo dei test infatti verranno messi a confronto i segnali simulati con quelli realmente misurati e verranno messe in luce le prestazioni dello strumento, ma anche i limiti.  Il quinto capitolo sarà dedicato all’analisi dati, alla descrizione dei software che permettono il retrieval dei profili verticali di vapore acqueo. In questo capitolo verranno anche discusse le approssimazioni utilizzate e la bontà del dato.  Nel sesto capitolo verranno presentati due casi studio particolari con l’intenzione di mostrare le prime considerazioni preliminari sul lavoro sinergico del LIDAR con gli altri strumenti operativi in BAQUNIN e sui confronti tra le misure ottenute dai due siti

Clear-air lidar dark band

This paper illustrates measurements carried out by the Raman lidar BASIL in the frame of HOPE, revealing the presence of a clear-air dark band phenomenon (i.e. the appearance of a minimum in lidar backscatter echoes) in the upper portion of the convective boundary layer. The phenomenon is clearly distinguishable in the lidar backscatter echoes at 1064 nm. This phenomenon is attributed to the presence of lignite aerosol particles advected from the surrounding open pit mines in the vicinity of the measuring site

Characterization of Turbulent Processes by the Raman Lidar System Basil in the Frame of the HD(CP)2 Observational Prototype Experiment-Hope

Measurements carried out by the Raman lidar system BASIL are reported to demonstrate the capability of this instrument to characterize turbulent processes within the Convective Boundary Layer (CBL). In order to resolve the vertical profiles of turbulent variables, high resolution water vapour and temperature measurements, with a temporal resolution of 10 sec and a vertical resolution of 90 and 210 m, respectively, are considered. Measurements of higher-order moments of the turbulent fluctuations of water vapour mixing ratio and temperature are obtained based on the application of spectral and auto-covariance analyses to the water vapour mixing ratio and temperature time series. The algorithms are applied to a case study (IOP 5, 20 April 2013) from the HD(CP)2 Observational Prototype Experiment (HOPE), held in Central Germany in the spring 2013. The noise errors are demonstrated to be small enough to allow the derivation of up to fourth-order moments for both water vapour mixing ratio and temperature fluctuations with sufficient accuracy

Characterization of Water Vapor Fluxes by the Raman Lidar System Basil and the Univeristy of Cologne Wind Lidar in the Frame of the HD(CP)2 Observational Prototype Experiment-Hope

Measurements carried out by the Raman lidar system BASIL and the University of Cologne wind lidar are reported to demonstrate the capability of these instruments to characterize water vapour fluxes within the Convective Boundary Layer (CBL). In order to determine the water vapour flux vertical profiles, high resolution water vapour and vertical wind speed measurements, with a temporal resolution of 1 sec and a vertical resolution of 15-90, are considered. Measurements of water vapour flux profiles are based on the application of covariance approach to the water vapour mixing ratio and vertical wind speed time series. The algorithms are applied to a case study (IOP 11, 04 May 2013) from the HD(CP)2 Observational Prototype Experiment (HOPE), held in Central Germany in the spring 2013. For this case study, the water vapour flux profile is characterized by increasing values throughout the CBL with lager values (around 0.1 g/kg m/s) in the entrainment region. The noise errors are demonstrated to be small enough to allow the derivation of water vapour flux profiles with sufficient accuracy

Characterization of Water Vapor Fluxes by the Raman Lidar System Basil and the Univeristy of Cologne Wind Lidar in the Frame of the HD(CP)2 Observational Prototype Experiment – Hope

Measurements carried out by the Raman lidar system BASIL and the University of Cologne wind lidar are reported to demonstrate the capability of these instruments to characterize water vapour fluxes within the Convective Boundary Layer (CBL). In order to determine the water vapour flux vertical profiles, high resolution water vapour and vertical wind speed measurements, with a temporal resolution of 1 sec and a vertical resolution of 15-90, are considered. Measurements of water vapour flux profiles are based on the application of covariance approach to the water vapour mixing ratio and vertical wind speed time series. The algorithms are applied to a case study (IOP 11, 04 May 2013) from the HD(CP)2 Observational Prototype Experiment (HOPE), held in Central Germany in the spring 2013. For this case study, the water vapour flux profile is characterized by increasing values throughout the CBL with lager values (around 0.1 g/kg m/s) in the entrainment region. The noise errors are demonstrated to be small enough to allow the derivation of water vapour flux profiles with sufficient accuracy