120 research outputs found
Characterization of strong light-matter coupling in semiconductor quantum-dot microcavities via photon-statistics spectroscopy
It is shown that spectrally resolved photon-statistics measurements of the
resonance fluorescence from realistic semiconductor quantum-dot systems allow
for high contrast identification of the two-photon strong-coupling states.
Using a microscopic theory, the second-rung resonance is analyzed and optimum
excitation conditions are determined. The computed photon-statistics spectrum
displays gigantic, experimentally robust resonances at the energetic positions
of the second-rung emission.Comment: 4 pages, 2 figure
Observation of Coulomb-Assisted Dipole-Forbidden Intraexciton Transitions in Semiconductors
We use terahertz pulses to induce resonant transitions between the
eigenstates of optically generated exciton populations in a high-quality
semiconductor quantum-well sample. Monitoring the excitonic photoluminescence,
we observe transient quenching of the exciton emission, which we attribute
to the terahertz-induced -to- excitation. Simultaneously, a pronounced
enhancement of the -exciton emission is observed, despite the -to-
transition being dipole forbidden. A microscopic many-body theory explains the
experimental observations as a Coulomb-scattering mixing of the 2 and 2
states, yielding an effective terahertz transition between the 1 and 2
populations.Comment: 5 pages, 3 figure
Palaeoenvironmental variability and carbon cycle perturbations during the Smithian-Spathian (Early Triassic) in Central Spitsbergen
The Early Triassic Smithian and Spathian time intervals are characterized by perturbations in the global carbon cycle, fluctuations in sea surface temperature, high turnover rates of marine nekton, and a change in terrestrial vegetation. Despite the importance of this time interval, comprehensive multiproxy investigations from Early Triassic high and middle latitude regions remain scarce due to the difficulty in accessing sections. The
objective of this study is to increase our understanding of regional and local palaeoenvironmental and carbon cycle perturbations from a middle Smithian to late Spathian middle latitude section from Central Spitsbergen. Geochemical analyses show an increase in phosphorus and nitrogen just at and above the Smithian–Spathian boundary (SSB). High primary productivity led to increasingly anoxic conditions in bottom waters
during the middle and late Spathian, enhancing the preservation of organic matter in the sediments. Anoxic conditions restrain phosphorus remineralization, allowing it to be recycled within the water column. This increase in anoxia is consistent with observations in other Arctic basins, demonstrating larger regional similarities in palaeoenvironmental conditions. The fluctuations in isostatic and eustatic sea levels affected organic
carbon sequestration by regulating organic matter mineral interactions via the control of grain size within the sediment. This study demonstrates that local organic carbon sequestration in the Barents Sea shelf during the Spathian was influenced by a multitude of factors, including sedimentology, redox conditions, nutrient availability, and primary productivity.
□ Vikinghøgda Formation, bulk rock geochemistry, particulate organic matter, extinction recovery, carbon isotopes, Stensiöfjellet Franziska R. Blattmann ✉ [[email protected]], Zoneibe A.S. Luz [[email protected]] and Torsten W. Vennemann [[email protected]], Institute
of Earth Surface Dynamics, University of Lausanne, Quartier UNIL-Mouline, 1015 Lausanne, Switzerland; Elke Schneebeli-Hermann [[email protected]] and Hugo F.R. Bucher [[email protected]], Department of Palaeontology, University of
Zürich, Karl-Schmid-Strasse 4, 8006 Zürich, Switzerland; Thierry Adatte [[email protected]], Institute of Earth Sciences, University of Lausanne, Quartier UNIL-Mouline, CH-1015 Lausanne, Switzerland; Christian Vérard [[email protected]], Section of Earth and Environmental Sciences, University of Geneva, Rue des Maraîchers 13, CH-1205 Geneva, Switzerland; Øyvind Hammer [[email protected]], Natural History Museum, University of Oslo, Pb. 1172 Blindern, 0318 Oslo, Norway; manuscript received on 08/08/2023; manuscript accepted on 02/02/2024; manuscript published on 20/06/2024 in Lethaia 57(2)
Highly Conducting pi-Conjugated Molecular Junctions Covalently Bonded to Gold Electrodes
We measure electronic conductance through single conjugated molecules bonded
to Au metal electrodes with direct Au-C covalent bonds using the scanning
tunneling microscope based break-junction technique. We start with molecules
terminated with trimethyltin end groups that cleave off in situ resulting in
formation of a direct covalent sigma bond between the carbon backbone and the
gold metal electrodes. The molecular carbon backbone used in this study consist
of a conjugated pi-system that has one terminal methylene group on each end,
which bonds to the electrodes, achieving large electronic coupling of the
electrodes to the pi-system. The junctions formed with the prototypical example
of 1,4-dimethylenebenzene show a conductance approaching one conductance
quantum (G0 = 2e2/h). Junctions formed with methylene terminated oligophenyls
with two to four phenyl units show a hundred-fold increase in conductance
compared with junctions formed with amine-linked oligophenyls. The conduction
mechanism for these longer oligophenyls is tunneling as they exhibit an
exponential dependence of conductance with oligomer length. In addition,
density functional theory based calculations for the Au-xylylene-Au junction
show near-resonant transmission with a cross-over to tunneling for the longer
oligomers.Comment: Accepted to the Journal of the American Chemical Society as a
Communication
Observation of squeezed light from one atom excited with two photons
Single quantum emitters like atoms are well-known as non-classical light
sources which can produce photons one by one at given times, with reduced
intensity noise. However, the light field emitted by a single atom can exhibit
much richer dynamics. A prominent example is the predicted ability for a single
atom to produce quadrature-squeezed light, with sub-shot-noise amplitude or
phase fluctuations. It has long been foreseen, though, that such squeezing
would be "at least an order of magnitude more difficult" to observe than the
emission of single photons. Squeezed beams have been generated using
macroscopic and mesoscopic media down to a few tens of atoms, but despite
experimental efforts, single-atom squeezing has so far escaped observation.
Here we generate squeezed light with a single atom in a high-finesse optical
resonator. The strong coupling of the atom to the cavity field induces a
genuine quantum mechanical nonlinearity, several orders of magnitude larger
than for usual macroscopic media. This produces observable quadrature squeezing
with an excitation beam containing on average only two photons per system
lifetime. In sharp contrast to the emission of single photons, the squeezed
light stems from the quantum coherence of photon pairs emitted from the system.
The ability of a single atom to induce strong coherent interactions between
propagating photons opens up new perspectives for photonic quantum logic with
single emittersComment: Main paper (4 pages, 3 figures) + Supplementary information (5 pages,
2 figures). Revised versio
Sensitivity of the stress response function to packing preparation
A granular assembly composed of a collection of identical grains may pack
under different microscopic configurations with microscopic features that are
sensitive to the preparation history. A given configuration may also change in
response to external actions such as compression, shearing etc. We show using a
mechanical response function method developed experimentally and numerically,
that the macroscopic stress profiles are strongly dependent on these
preparation procedures. These results were obtained for both two and three
dimensions. The method reveals that, under a given preparation history, the
macroscopic symmetries of the granular material is affected and in most cases
significant departures from isotropy should be observed. This suggests a new
path toward a non-intrusive test of granular material constitutive properties.Comment: 15 pages, 11 figures, some numerical data corrected, to appear in J.
Phys. Cond. Mat. special issue on Granular Materials (M. Nicodemi Editor
The MEG detector for decay search
The MEG (Mu to Electron Gamma) experiment has been running at the Paul
Scherrer Institut (PSI), Switzerland since 2008 to search for the decay \meg\
by using one of the most intense continuous beams in the world. This
paper presents the MEG components: the positron spectrometer, including a thin
target, a superconducting magnet, a set of drift chambers for measuring the
muon decay vertex and the positron momentum, a timing counter for measuring the
positron time, and a liquid xenon detector for measuring the photon energy,
position and time. The trigger system, the read-out electronics and the data
acquisition system are also presented in detail. The paper is completed with a
description of the equipment and techniques developed for the calibration in
time and energy and the simulation of the whole apparatus.Comment: 59 pages, 90 figure
The Influence of Molecular Adsorption on Elongating Gold Nanowires
Using molecular dynamics simulations, we study the impact of physisorbing
adsorbates on the structural and mechanical evolution of gold nanowires (AuNWs)
undergoing elongation. We used various adsorbate models in our simulations,
with each model giving rise to a different surface coverage and mobility of the
adsorbed phase. We find that the local structure and mobility of the adsorbed
phase remains relatively uniform across all segments of an elongating AuNW,
except for the thinning region of the wire where the high mobility of Au atoms
disrupts the monolayer structure, giving rise to higher solvent mobility. We
analyzed the AuNW trajectories by measuring the ductile elongation of the wires
and detecting the presence of characteristic structural motifs that appeared
during elongation. Our findings indicate that adsorbates facilitate the
formation of high-energy structural motifs and lead to significantly higher
ductile elongations. In particular, our simulations result in a large number of
monatomic chains and helical structures possessing mechanical stability in
excess of what we observe in vacuum. Conversely, we find that a molecular
species that interacts weakly (i.e., does not adsorb) with AuNWs worsens the
mechanical stability of monatomic chains.Comment: To appear in Journal of Physical Chemistry
- …