59 research outputs found
Dynamics of the Destruction and Rebuilding of a Dipole Gap in Glasses
After a strong electric bias field was applied to a glass sample at
temperatures in the millikelvin range its AC-dielectric constant increases and
then decays logarithmically with time. For the polyester glass mylar we have
observed the relaxation of the dielectric constant back to its initial value
for several temperatures and histories of the bias field. Starting from the
dipole gap theory we have developed a model suggesting that the change of the
dielectric constant after transient application of a bias field is only partly
due to relaxational processes. In addition, non-adiabatic driving of tunneling
states (TSs) by applied electric fields causes long lasting changes in the
dielectric constant. Moreover, our observations indicate that at temperatures
below 50 mK the relaxation of TSs is caused primarily by interactions between
TSs.Comment: 4 pages, 4 figures, submitted to PR
Correlated Persistent Tunneling Currents in Glasses
Low temperature properties of glasses are derived within a generalized
tunneling model, considering the motion of charged particles on a closed path
in a double-well potential. The presence of a magnetic induction field B
violates the time reversal invariance due to the Aharonov-Bohm phase, and leads
to flux periodic energy levels. At low temperature, this effect is shown to be
strongly enhanced by dipole-dipole and elastic interactions between tunneling
systems and becomes measurable. Thus, the recently observed strong sensitivity
of the electric permittivity to weak magnetic fields can be explained. In
addition, superimposed oscillations as a function of the magnetic field are
predicted.Comment: 4 page
Dynamics of Highly Supercooled Liquids:Heterogeneity, Rheology, and Diffusion
Highly supercooled liquids with soft-core potentials are studied via
molecular dynamics simulations in two and three dimensions in quiescent and
sheared conditions.We may define bonds between neighboring particle pairs
unambiguously owing to the sharpness of the first peak of the pair correlation
functions. Upon structural rearrangements, they break collectively in the form
of clusters whose sizes grow with lowering the temperature . The bond life
time , which depends on and the shear rate \gdot, is on the order
of the usual structural or relaxation time in weak
shear \gdot \tau_{\alpha} \ll 1, while it decreases as 1/\gdot in strong
shear \gdot\tau_{\alpha} \gg 1 due to shear-induced cage breakage.
Accumulated broken bonds in a time interval () closely
resemble the critical fluctuations of Ising spin systems. For example, their
structure factor is well fitted to the Ornstein-Zernike form, which yields the
correlation length representing the maximum size of the clusters composed
of broken bonds. We also find a dynamical scaling relation, , valid for any and \gdot with in two dimensions and
in three dimensions. The viscosity is of order for any and
\gdot, so marked shear-thinning behavior emerges. The shear stress is close
to a limiting stress in a wide shear region. We also examine motion of tagged
particles in shear in three dimensions. The diffusion constant is found to be
of order with for any and \gdot, so
it is much enhanced in strong shear compared with its value at zero shear. This
indicates breakdown of the Einstein-Stokes relation in accord with experiments.
Some possible experiments are also proposed.Comment: 20pages (including figures
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