59 research outputs found
Anisotropic conductivity of Nd_{1.85}Ce_{0.15}CuO_{4-\delta} films at submillimeter wavelengths
The anisotropic conductivity of thin NdCeCuO
films was measured in the frequency range 8 cm 40 cm and
for temperatures 4 K K. A tilted sample geometry allowed to extract
both, in-plane and c-axis properties. The in-plane quasiparticle scattering
rate remains unchanged as the sample becomes superconducting. The temperature
dependence of the in-plane conductivity is reasonably well described using the
Born limit for a d-wave superconductor. Below T_{{\rm C}%} the c-axis
dielectric constant changes sign at the screened c-axis plasma
frequency. The temperature dependence of the c-axis conductivity closely
follows the linear in T behavior within the plane.Comment: 4 pages, 4 figure
Microwave Electrodynamics of Electron-Doped Cuprate Superconductors
We report microwave cavity perturbation measurements of the temperature
dependence of the penetration depth, lambda(T), and conductivity, sigma(T) of
Pr_{2-x}Ce_{x}CuO_{4-delta} (PCCO) crystals, as well as parallel-plate
resonator measurements of lambda(T) in PCCO thin films. Penetration depth
measurements are also presented for a Nd_{2-x}Ce_{x}CuO_{4-delta} (NCCO)
crystal. We find that delta-lambda(T) has a power-law behavior for T<T_c/3, and
conclude that the electron-doped cuprate superconductors have nodes in the
superconducting gap. Furthermore, using the surface impedance, we have derived
the real part of the conductivity, sigma_1(T), below T_c and found a behavior
similar to that observed in hole-doped cuprates.Comment: 4 pages, 4 figures, 1 table. Submitted to Physical Review Letters
revised version: new figures, sample characteristics added to table, general
clarification give
Nonmonotonic d_{x^2-y^2} Superconducting Order Parameter in Nd_{2-x}Ce_xCuO_4
Low energy polarized electronic Raman scattering of the electron doped
superconductor Nd_1.85Ce_0.15CuO_4 (T_c=22 K) has revealed a nonmonotonic
d_{x^2-y^2} superconducting order parameter. It has a maximum gap of 4.4 k_BT_c
at Fermi surface intersections with antiferromagnetic Brillouin zone (the ``hot
spots'') and a smaller gap of 3.3 k_BT_c at fermionic Brillouin zone
boundaries. The gap enhancement in the vicinity of the ``hot spots'' emphasizes
role of antiferromagnetic fluctuations and similarity in the origin of
superconductivity for electron- and hole-doped cuprates.Comment: 4 pages, 4 figure
Aesthetics and Psychological Effects of Fractal Based Design
21 pagesHighly prevalent in nature, fractal patterns possess self-similar components that repeat
at varying size scales. The perceptual experience of human-made environments can
be impacted with inclusion of these natural patterns. Previous work has demonstrated
consistent trends in preference for and complexity estimates of fractal patterns.
However, limited information has been gathered on the impact of other visual judgments.
Here we examine the aesthetic and perceptual experience of fractal ‘global-forest’
designs already installed in humanmade spaces and demonstrate how fractal pattern
components are associated with positive psychological experiences that can be
utilized to promote occupant wellbeing. These designs are composite fractal patterns
consisting of individual fractal ‘tree-seeds’ which combine to create a ‘global fractal
forest.’ The local ‘tree-seed’ patterns, global configuration of tree-seed locations, and
overall resulting ‘global-forest’ patterns have fractal qualities. These designs span
multiple mediums yet are all intended to lower occupant stress without detracting
from the function and overall design of the space. In this series of studies, we
first establish divergent relationships between various visual attributes, with pattern
complexity, preference, and engagement ratings increasing with fractal complexity
compared to ratings of refreshment and relaxation which stay the same or decrease
with complexity. Subsequently, we determine that the local constituent fractal (‘treeseed’)
patterns contribute to the perception of the overall fractal design, and address
how to balance aesthetic and psychological effects (such as individual experiences
of perceived engagement and relaxation) in fractal design installations. This set of
studies demonstrates that fractal preference is driven by a balance between increased
arousal (desire for engagement and complexity) and decreased tension (desire for
relaxation or refreshment). Installations of these composite mid-high complexity ‘globalforest’
patterns consisting of ‘tree-seed’ components balance these contrasting needs,
and can serve as a practical implementation of biophilic patterns in human-made
environments to promote occupant wellbeing
Electron Dynamics in NdCeCuO: Evidence for the Pseudogap State and Unconventional c-axis Response
Infrared reflectance measurements were made with light polarized along the a-
and c-axis of both superconducting and antiferromagnetic phases of electron
doped NdCeCuO. The results are compared to
characteristic features of the electromagnetic response in hole doped cuprates.
Within the CuO planes the frequency dependent scattering rate,
1/, is depressed below 650 cm; this behavior is a
hallmark of the pseudogap state. While in several hole doped compounds the
energy scales associated with the pseudogap and superconducting states are
quite close, we are able to show that in NdCeCuO
the two scales differ by more than one order of magnitude. Another feature of
the in-plane charge response is a peak in the real part of the conductivity,
, at 50-110 cm which is in sharp contrast with the
Drude-like response where is centered at . This
latter effect is similar to what is found in disordered hole doped cuprates and
is discussed in the context of carrier localization. Examination of the c-axis
conductivity gives evidence for an anomalously broad frequency range from which
the interlayer superfluid is accumulated. Compelling evidence for the pseudogap
state as well as other characteristics of the charge dynamics in
NdCeCuO signal global similarities of the cuprate
phase diagram with respect to electron and hole doping.Comment: Submitted to PR
Multiband model of high Tc superconductors
We propose an extension to other high T_{c } compounds of a model introduced
earlier for YBCO. In the ''self-doped'' compounds we assume that the doping
part (namely the BiO, HgO, TlO planes in BSCCO, HBCCO, TBCCO respectively) is
metallic, which leads to a multiband model. This assumption is supported by
band structure calculations. Taking a repulsive pairing interaction between
these doping bands and the CuO_{2} bands leads to opposite signs for the order
parameter on these bands and to nodes whenever the Fermi surfaces of these
bands cross. We show that in BSCCO the low temperature dependence of the
penetration depth is reasonably accounted for. In this case the nodes are not
located near the 45^{o} direction, which makes the experimental determination
of the node locations an important test for our model. The situation in HBCCO
and TBCCO is rather analogous to BSCCO. We consider the indications given by
NMR and find that they rather favor a metallic character for the doping bands.
Finally we discuss the cases of NCCO and LSCO which are not ''self-doped'' and
where our model does not give nodes.Comment: 11 pages, revtex, 1 figure
Carrier relaxation, pseudogap, and superconducting gap in high-Tc cuprates: A Raman scattering study
We describe results of electronic Raman-scattering experiments in differently
doped single crystals of Y-123 and Bi-2212. The comparison of AF insulating and
metallic samples suggests that at least the low-energy part of the spectra
originates predominantly from excitations of free carriers. We therefore
propose an analysis of the data in terms of a memory function approach.
Dynamical scattering rates and mass-enhancement factors for the carriers are
obtained. In B2g symmetry the Raman data compare well to the results obtained
from ordinary and optical transport. For underdoped materials the dc scattering
rates in B1g symmetry become temperature independent and considerably larger
than in B2g symmetry. This increasing anisotropy is accompanied by a loss of
spectral weight in B2g symmetry in the range between the superconducting
transition at Tc and a characteristic temperature T* of order room temperature
which compares well with the pseudogap temperature found in other experiments.
The energy range affected by the pseudogap is doping and temperature
independent. The integrated spectral loss is approximately 25% in underdoped
samples and becomes much weaker towards higher carrier concentration. In
underdoped samples, superconductivity related features in the spectra can be
observed only in B2g symmetry. The peak frequencies scale with Tc. We do not
find a direct relation between the pseudogap and the superconducting gap.Comment: RevTeX, 21 pages, 24 gif figures. For PostScript with embedded eps
figures, see http://www.wmi.badw-muenchen.de/~opel/k2.htm
Inelastic Light Scattering From Correlated Electrons
Inelastic light scattering is an intensively used tool in the study of
electronic properties of solids. Triggered by the discovery of high temperature
superconductivity in the cuprates and by new developments in instrumentation,
light scattering both in the visible (Raman effect) and the X-ray part of the
electromagnetic spectrum has become a method complementary to optical
(infrared) spectroscopy while providing additional and relevant information.
The main purpose of the review is to position Raman scattering with regard to
single-particle methods like angle-resolved photoemission spectroscopy (ARPES),
and other transport and thermodynamic measurements in correlated materials.
Particular focus will be placed on photon polarizations and the role of
symmetry to elucidate the dynamics of electrons in different regions of the
Brillouin zone. This advantage over conventional transport (usually measuring
averaged properties) indeed provides new insights into anisotropic and complex
many-body behavior of electrons in various systems. We review recent
developments in the theory of electronic Raman scattering in correlated systems
and experimental results in paradigmatic materials such as the A15
superconductors, magnetic and paramagnetic insulators, compounds with competing
orders, as well as the cuprates with high superconducting transition
temperatures. We present an overview of the manifestations of complexity in the
Raman response due to the impact of correlations and developing competing
orders. In a variety of materials we discuss which observations may be
understood and summarize important open questions that pave the way to a
detailed understanding of correlated electron systems.Comment: 62 pages, 48 figures, to appear in Rev. Mod. Phys. High-resolution
pdf file available at http://onceler.uwaterloo.ca/~tpd/RMP.pd
Up scalable ITO free organic light emitting diodes based on embedded inkjet printed copper grids
We report on ITO-free OLEDS with a transparent hybrid Cu nanoparticle grid/PEDOT:PSS electrode processed in ambient conditions. An experimentally based methodology was implemented, where studies on alternative PEDOT:PSS derivatives and Cu grid design were performed, to gradually increase the efficiency of lab scale ITO-free OLEDs. To further increase electrode performance, inkjet-printed (IJP) Cu-grids are embedded to flatten the electrode, reduce leakage current and enhance homogeneity and efficiency. Finally, embedded Cu based ITO-free OLEDs showed current and power efficiencies comparable to reference ITO-based OLEDs. Methods to manufacture large area flat embedded IJP Cu-electrodes on glass and flexible substrates are presented and upscaling prospects of the proposed ITO-free electrode are discussed
Angle-resolved photoemission spectroscopy of the cuprate superconductors
This paper reviews the most recent ARPES results on the cuprate
superconductors and their insulating parent and sister compounds, with the
purpose of providing an updated summary of the extensive literature in this
field. The low energy excitations are discussed with emphasis on some of the
most relevant issues, such as the Fermi surface and remnant Fermi surface, the
superconducting gap, the pseudogap and d-wave-like dispersion, evidence of
electronic inhomogeneity and nano-scale phase separation, the emergence of
coherent quasiparticles through the superconducting transition, and many-body
effects in the one-particle spectral function due to the interaction of the
charge with magnetic and/or lattice degrees of freedom. The first part of the
paper introduces photoemission spectroscopy in the context of strongly
interacting systems, along with an update on the state-of-the-art
instrumentation. The second part provides a brief overview of the scientific
issues relevant to the investigation of the low energy electronic structure by
ARPES. The rest of the paper is devoted to the review of experimental results
from the cuprates and the discussion is organized along conceptual lines:
normal-state electronic structure, interlayer interaction, superconducting gap,
coherent superconducting peak, pseudogap, electron self energy and collective
modes. Within each topic, ARPES data from the various copper oxides are
presented.Comment: Reviews of Modern Physics, in press. A HIGH-QUALITY pdf file is
available at http://www.physics.ubc.ca/~damascel/RMP_ARPES.pd
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