3,483 research outputs found
Detection of antiferromagnetic ordering in heavily doped LaFeAsO1-xHx pnictide superconductors using nuclear-magnetic-resonance techniques
We studied double superconducting (SC) domes in LaFeAsO1-xHx by using 75As-
and 1H-nuclear magnetic resonance techniques, and unexpectedly discovered that
a new antiferromagnetic (AF) phase follows the double SC domes on further H
doping, forming a symmetric alignment of AF and SC phases in the electronic
phase diagram. We demonstrated that the new AF ordering originates from the
nesting between electron pockets, unlike the nesting between electron and hole
pockets as seen in the majority of undoped pnictides. The new AF ordering is
derived from the features common to high-Tc pnictides: however, it has not been
reported so far for other high-Tc pnictides because of their poor electron
doping capability.Comment: 5 figures, in press in PR
Quantum critical behavior in heavily doped LaFeAsOH pnictide superconductors analyzed using nuclear magnetic resonance
We studied the quantum critical behavior of the second antiferromagnetic (AF)
phase in the heavily electron-doped high- pnictide, LaFeAsOH
by using As and H nuclear-magnetic-resonance (NMR) technique. In
the second AF phase, we observed a spatially modulated spin-density-wave-like
state up to =0.6 from the NMR spectral lineshape and detected a low-energy
excitation gap from the nuclear relaxation time of As. The
excitation gap closes at the AF quantum critical point (QCP) at . The superconducting (SC) phase in a lower-doping regime contacts the
second AF phase only at the AF QCP, and both phases are segregated from each
other. The absence of AF critical fluctuations and the enhancement of the
in-plane electric anisotropy are key factors for the development of
superconductivity.Comment: accepted in Phys. Rev.
Scaling theory of DNA confined in nanochannels and nanoslits
A scaling analysis is presented of the statistics of long DNA confined in
nanochannels and nanoslits. It is argued that there are several regimes in
between the de Gennes and Odijk limits introduced long ago. The DNA chain folds
back on itself giving rise to a global persistence length which may be very
large owing to entropic deflection. Moreover, there is an orientational
excluded-volume effect between the DNA segments imposed solely by the
nanoconfinement. These two effects cause the chain statistics to be intricate
leading to nontrivial power laws for the chain extension in the intermediate
regimes. It is stressed that DNA confinement within nanochannels differs from
that in nanoslits because the respective orientational excluded-volume effects
are not the same.Comment: 5 pages, 1 figure Several corrections, some minor changes in the text
and replacement of one referenc
Diffusion-limited loop formation of semiflexible polymers: Kramers theory and the intertwined time scales of chain relaxation and closing
We show that Kramers rate theory gives a straightforward, accurate estimate
of the closing time of a semiflexible polymer that is valid in cases
of physical interest. The calculation also reveals how the time scales of chain
relaxation and closing are intertwined, illuminating an apparent conflict
between two ways of calculating in the flexible limit.Comment: Europhys. Lett., 2003 (in press). 8 pages, 3 figures. See also,
physics/0101087 for physicist's approach to and the importance of
semiflexible polymer looping, in DNA replicatio
Shapes of Semiflexible Polymers in Confined Spaces
We investigate the conformations of a semiflexible polymer confined to a
square box. Results of Monte Carlo simulations show the existence of a shape
transition when the persistence length of the polymer becomes comparable to the
dimensions of box. An order parameter is introduced to quantify this behavior.
A simple mean-field model is constructed to study the effect of the shape
transition on the effective persistence length of the polymer.Comment: 8 pages, 20 figure
A general theory of DNA-mediated and other valence-limited interactions
We present a general theory for predicting the interaction potentials between
DNA-coated colloids, and more broadly, any particles that interact via
valence-limited ligand-receptor binding. Our theory correctly incorporates the
configurational and combinatorial entropic factors that play a key role in
valence-limited interactions. By rigorously enforcing self-consistency, it
achieves near-quantitative accuracy with respect to detailed Monte Carlo
calculations. With suitable approximations and in particular geometries, our
theory reduces to previous successful treatments, which are now united in a
common and extensible framework. We expect our tools to be useful to other
researchers investigating ligand-mediated interactions. A complete and
well-documented Python implementation is freely available at
http://github.com/patvarilly/DNACC .Comment: 18 pages, 10 figure
Radial distribution function of semiflexible polymers
We calculate the distribution function of the end--to--end distance of a
semiflexible polymer with large bending rigidity. This quantity is directly
observable in experiments on single semiflexible polymers (e.g., DNA, actin)
and relevant to their interpretation. It is also an important starting point
for analyzing the behavior of more complex systems such as networks and
solutions of semiflexible polymers. To estimate the validity of the obtained
analytical expressions, we also determine the distribution function numerically
using Monte Carlo simulation and find good quantitative agreement.Comment: RevTeX, 4 pages, 1 figure. Also available at
http://www.cip.physik.tu-muenchen.de/tumphy/d/T34/Mitarbeiter/frey.htm
Orientational order and glassy states in networks of semiflexible polymers
Motivated by the structure of networks of cross-linked cytoskeletal
biopolymers, we study the orientationally ordered phases in two-dimensional
networks of randomly cross-linked semiflexible polymers. We consider permanent
cross-links which prescribe a finite angle and treat them as quenched disorder
in a semi-microscopic replica field theory. Starting from a fluid of
un-cross-linked polymers and small polymer clusters (sol) and increasing the
cross-link density, a continuous gelation transition occurs. In the resulting
gel, the semiflexible chains either display long range orientational order or
are frozen in random directions depending on the value of the crossing angle,
the crosslink concentration and the stiffness of the polymers. A crossing angle
leads to long range -fold orientational order, e.g.,
"hexatic" or "tetratic" for or , respectively.
The transition is discontinuous and the critical cross-link density depends on
the bending stiffness of the polymers and the cross-link geometry: the higher
the stiffness and the lower , the lower the critical number of cross-links.
In between the sol and the long range ordered state, we always observe a gel
which is a statistically isotropic amorphous solid (SIAS) with random
positional and random orientational localization of the participating polymers.Comment: 20 pages, added references, minor changes, final version as published
in PR
- …