Dynamic criticality in glass-forming liquids

We propose that the dynamics of supercooled liquids and the formation of glasses can be understood from the existence of a zero temperature dynamical critical point. To support our proposal, we derive from simple physical assumptions a dynamic field theory for supercooled liquids, which we study using the renormalization group (RG). Its long time behaviour is dominated by a zero temperature critical point, which for dimensions d > 2 belongs to the directed percolation universality class. Molecular dynamics simulations confirm the existence of dynamic scaling behaviour consistent with the RG predictions.Comment: 4 pages, 2 figure

Electron Spin Resonance of defects in the Haldane System Y(2)BaNiO(5)

We calculate the electron paramagnetic resonance (EPR) spectra of the antiferromagnetic spin-1 chain compound Y(2)BaNi(1-x)Mg(x)O(5) for different values of x and temperature T much lower than the Haldane gap (~100K). The low-energy spectrum of an anisotropic Heisenberg Hamiltonian, with all parameters determined from experiment, has been solved using DMRG. The observed EPR spectra are quantitatively reproduced by this model. The presence of end-chain S=1/2 states is clearly observed as the main peak in the spectrum and the remaining structure is completely understood.Comment: 5 pages, 4 figures include

Edge states in Open Antiferromagnetic Heisenberg Chains

In this letter we report our results in investigating edge effects of open antiferromagnetic Heisenberg spin chains with spin magnitudes $S=1/2, 1,3/2,2$ using the density-matrix renormalization group (DMRG) method initiated by White. For integer spin chains, we find that edge states with spin magnitude $S_{edge}=S/2$ exist, in agreement with Valence-Bond-Solid model picture. For half-integer spin chains, we find that no edge states exist for $S=1/2$ spin chain, but edge state exists in $S=3/2$ spin chain with $S_{edge}=1/2$, in agreement with previous conjecture by Ng. Strong finite size effects associated with spin dimmerization in half-integer spin chains will also be discussed.Comment: 4 pages, RevTeX 3.0, 5 figures in a separate uuencoded postscript file. Replaced once to enlarge the acknowlegement

Large-Scale Numerical Evidence for Bose Condensation in the S=1 Antiferromagnetic Chain in a Strong Field

Using the recently proposed density matrix renormalization group technique we show that the magnons in the S=1 antiferromagnetic Heisenberg chain effectively behaves as bosons that condense at a critical field h_c.Comment: 12 pages, REVTEX 3.0, 3 postscript figures appended, UBCTP-93-00

The Haldane gap for the S=2 antiferromagnetic Heisenberg chain revisited

Using the density matrix renormalization group (DMRG) technique, we carry out a large scale numerical calculation for the S=2 antiferromagnetic Heisenberg chain. Performing systematic scaling analysis for both the chain length $L$ and the number of optimal states kept in the iterations $m$, the Haldane gap $\Delta (2)$ is estimated accurately as $(0.0876\pm0.0013)J$. Our systematic analysis for the S=2 chains not only ends the controversies arising from various DMRG calculations and Monte Carlo simulations, but also sheds light on how to obtain reliable results from the DMRG calculations for other complicated systems.Comment: 4 pages and 1 figur

Distribution of exchange energy in a bond-alternating S=1 quantum spin chain

The quasi-one-dimensional bond-alternating S=1 quantum antiferromagnet NTENP is studied by single crystal inelastic neutron scattering. Parameters of the measured dispersion relation for magnetic excitations are compared to existing numerical results and used to determine the magnitude of bond-strength alternation. The measured neutron scattering intensities are also analyzed using the 1st-moment sum rules for the magnetic dynamic structure factor, to directly determine the modulation of ground state exchange energies. These independently determined modulation parameters characterize the level of spin dimerization in NTENP. First-principle DMRG calculations are used to study the relation between these two quantities.Comment: 10 pages, 10 figure

Levy flights from a continuous-time process

The Levy-flight dynamics can stem from simple random walks in a system whose operational time (number of steps n) typically grows superlinearly with physical time t. Thus, this processes is a kind of continuous-time random walks (CTRW), dual to usual Scher-Montroll model, in which $n$ grows sublinearly with t. The models in which Levy-flights emerge due to a temporal subordination let easily discuss the response of a random walker to a weak outer force, which is shown to be nonlinear. On the other hand, the relaxation of en ensemble of such walkers in a harmonic potential follows a simple exponential pattern and leads to a normal Boltzmann distribution. The mixed models, describing normal CTRW in superlinear operational time and Levy-flights under the operational time of subdiffusive CTRW lead to paradoxical diffusive behavior, similar to the one found in transport on polymer chains. The relaxation to the Boltzmann distribution in such models is slow and asymptotically follows a power-law

Thermodynamics of the bilinear-biquadratic spin one Heisenberg chain

The magnetic susceptibility and specific heat of the one-dimensional S=1 bilinear-biquadratic Heisenberg model are calculated using the transfer matrix renormalization group. By comparing the results with the experimental data of ${\rm LiVGe_2O_6}$ measured by Millet et al. (Phys. Rev. Lett. {\bf 83}, 4176 (1999)), we find that the susceptibility data of this material, after subtracting the impurity contribution, can be quantitatively explained with this model. The biquadratic exchange interaction in this material is found to be ferromagnetic, i.e. with a positive coupling constant.Comment: 4 pages, 4 postscript figure

Magnetization profiles and NMR spectra of doped Haldane chains at finite temperatures

Open segments of S=1 antiferromagnetic spin chains are studied at finite temperatures and fields using continuous time Quantum Monte Carlo techniques. By calculating the resulting magnetization profiles for a large range of chain lengths with fixed field and temperature we reconstruct the experimentally measured NMR spectrum of impurity doped Y$_2$BaNi$_{1-x}$Mg$_x$O$_5$. For temperatures above the gap the calculated NMR spectra are in excellent agreement with the experimental results, confirming the existence of $S=1/2$ excitations at the end of open S=1 chain segments. At temperatures below the gap, neglecting inter chain couplings, we still find well defined peaks in the calculated NMR spectra corresponding to the $S=1/2$ chain end excitations. At low temperatures, inter chain couplings could be important, resulting in a more complicated phase.Comment: 7 pages, 5 figures, minor correction

The Haldane Energy Gap of A Doped Linear-Chain Heisenberg Antiferromagnet

Using the valence-bond-solid (VBS) approach and the Schwinger boson mean field approximation, we study the dependence of the Haldane gap of a spin-1 linear chain Heisenberg antiferromagnet on impurity doping with different spins. The impurity spins affect the singlet pairing order parameter $\Delta$ and the constraint factor $\lambda$. As a result, the Haldane gap is reduced by a factor $\sim n_i^{2/3}$, with $n_i$ as the impurity concentration, and eventually collapses at $n_i \sim 1/\xi$ with $\xi$ as the VBS correlation length. This theoretical prediction can be verified by neutron scattering experiments.Comment: REVTEX, 12 pages, no figure