3 research outputs found
Calculation of pure dephasing for excitons in quantum dots
Pure dephasing of an exciton in a small quantum dot by optical and acoustic
phonons is calculated using the ``independent boson model''. Considering the
case of zero temperature the dephasing is shown to be only partial which
manifests itself in the polarization decaying to a finite value. Typical
dephasing times can be assigned even though the spectra exhibits strongly
non-Lorentzian line shapes. We show that the dephasing from LO phonon
scattering, occurs on a much larger time scale than that of dephasing due to
acoustic phonons which for low temperatures are also a more efficient dephasing
mechanism. The typical dephasing time is shown to strongly depend on the
quantum dot size whereas the electron phonon ``coupling strength'' and external
electric fields tend mostly to effect the residual coherence. The relevance of
the dephasing times for current quantum information processing implementation
schemes in quantum dots is discussed
Electron-phonon interaction effects in semiconductor quantum dots: a non-perturbative approach
Multiphonon processes in a model quantum dot (QD) containing two electronic states and several optical phonon modes are considered by taking into account both intra- and nterlevel terms. The Hamiltonian is exactly diagonalized, including a finite number of multiphonon processes large enough to guarantee that the result can be considered exact in the physically important energy region. The physical properties are studied by
calculating the electronic Green’s function and the QD dielectric function. When both the intra- and interlevel interactions are included, the calculated spectra allow several previously published experimental results obtained for spherical and self-assembled QD’s, such as enhanced two-LO-phonon replica in absorption spectra and up-converted photoluminescence to be explained. An explicit calculation of the spectral line shape due to intralevel interaction with a continuum of acoustic phonons is presented, where the multiphonon processes also are shown to be important. It is pointed out that such an interaction, under certain conditions, can lead to relaxation in the otherwise stationary polaron system.Fundação para a Ciência e a Tecnologia (FCT
Carrier relaxation with LO phonon decay in semiconductor quantum dots
Abstract Analysis of an exactly soluble model of phonons coupled to a carrier in a quantum dot provides a clear illustration of a phonon bottleneck to relaxation. The introduction of three-phonon interactions leads to a broad window for relaxation by the processes of LO phonon scattering and decay.