23 research outputs found
Iron Behaving Badly: Inappropriate Iron Chelation as a Major Contributor to the Aetiology of Vascular and Other Progressive Inflammatory and Degenerative Diseases
- Author
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- The Long-Term Intervention with Pravastatin in Ischaemic Disease (LIPID) Study Group
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- ZZ Chong
- Publication venue
- Publication date
- 09/08/2008
- Field of study
The production of peroxide and superoxide is an inevitable consequence of
aerobic metabolism, and while these particular "reactive oxygen species" (ROSs)
can exhibit a number of biological effects, they are not of themselves
excessively reactive and thus they are not especially damaging at physiological
concentrations. However, their reactions with poorly liganded iron species can
lead to the catalytic production of the very reactive and dangerous hydroxyl
radical, which is exceptionally damaging, and a major cause of chronic
inflammation. We review the considerable and wide-ranging evidence for the
involvement of this combination of (su)peroxide and poorly liganded iron in a
large number of physiological and indeed pathological processes and
inflammatory disorders, especially those involving the progressive degradation
of cellular and organismal performance. These diseases share a great many
similarities and thus might be considered to have a common cause (i.e.
iron-catalysed free radical and especially hydroxyl radical generation). The
studies reviewed include those focused on a series of cardiovascular, metabolic
and neurological diseases, where iron can be found at the sites of plaques and
lesions, as well as studies showing the significance of iron to aging and
longevity. The effective chelation of iron by natural or synthetic ligands is
thus of major physiological (and potentially therapeutic) importance. As
systems properties, we need to recognise that physiological observables have
multiple molecular causes, and studying them in isolation leads to inconsistent
patterns of apparent causality when it is the simultaneous combination of
multiple factors that is responsible. This explains, for instance, the
decidedly mixed effects of antioxidants that have been observed, etc...Comment: 159 pages, including 9 Figs and 2184 reference
ATTITUDES OF ALLIED HEALTH STUDENTS TOWARD WRITING IN COMMUNITY COLLEGE SCIENCE COURSES
- Author
- Publication venue
- 'Informa UK Limited'
- Publication date
- Field of study
State and concentration of selenium in copper refinery electrolyte
- Author
- Publication venue
- 'Springer Science and Business Media LLC'
- Publication date
- Field of study
The Interaction of Serotonin, Norepinephrine, Epinephrine, and Angiotensin II During Pregnancy
- Author
- Publication venue
- 'Informa UK Limited'
- Publication date
- Field of study
Effect of Atriopeptin on Production of Cerebrospinal Fluid
- Author
- Publication venue
- 'Springer Science and Business Media LLC'
- Publication date
- Field of study
Surface and Passive Monitoring for Asbestos in an Industrial Facility
- Author
- Publication venue
- 'SAGE Publications'
- Publication date
- Field of study
From Bhopal to Cold Fusion: A Case-Study Approach to Writing Assignments in Honors General Chemistry
- Author
- Publication venue
- 'American Chemical Society (ACS)'
- Publication date
- Field of study
A comparison of the reactions of the oxide radical anion (o−.) with simple aromatic compounds at atmospheric and at reduced pressure conditions
- Author
- Publication venue
- 'Elsevier BV'
- Publication date
- Field of study
Influence of the leaving group on the dynamics of a gas-phase SN2 reaction
- Author
- AA Viggiano
- Aditya H. Kelkar
- AJ Orr-Ewing
- AP Bento
- ATJB Eppink
- DR Lide
- Eduardo Carrascosa
- Gábor Czakó
- I Fernández
- I Szabó
- I Szabó
- István Szabó
- J Mikosch
- J Mikosch
- J Xie
- J Xie
- J Zhang
- Jennifer Meyer
- JK Laerdahl
- JM Garver
- JM Garver
- JSM Anderson
- KPC Vollhardt
- LA Angel
- Martin A. Kainz
- Martin Stei
- ML Chabinyc
- P Jaramillo
- R Kretschmer
- R Otto
- R Sun
- R Wester
- Roland Wester
- S Liu
- S Schmatz
- S Thallmair
- SL Vanorden
- SS Shaik
- T Su
- T Su
- VF DeTuri
- WL Hase
- WN Olmstead
- Publication venue
- 'Springer Science and Business Media LLC'
- Publication date
- 01/01/2016
- Field of study
In addition to nucleophile and solvent, the leaving group has a significant
influence on nucleophilic substitution (SN2) reactions. Its role is frequently
discussed with respect to reactivity, but its influence on the reaction
dynamics remains obscured. Here, we uncover the influence of the leaving group
on the gas phase dynamics of SN2 reactions in a combined approach of
crossed-beam imaging and dynamics simulations. We have studied the reaction F-
+ CH3Cl and compared it to F- + CH3I. For the two leaving groups Cl and I we
find very similar structures and energetics, but the dynamics show
qualitatively different features. Simple scaling of the leaving group mass does
not explain these differences. Instead, the relevant impact parameters for the
reaction mechanisms are found to be crucial, which is attributed to the
relative orientation of the approaching reactants. This effect occurs on short
time scales and may also prevail under solution phase conditions
Effects of nitrogen oxides, sulfur dioxide, and ferric ions on the corrosion of mild steel in concentrated sulfuric acid
- Author
- Publication venue
- 'Springer Science and Business Media LLC'
- Publication date
- Field of study