9 research outputs found

    Anthropogenic, detritic and atmospheric soil-derived sources of lead in an alpine poor fen in northeast China

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    Ombrotrophic bogs are faithful archive of atmospheric metal deposition, but the potential for fens to reconstruct environmental change is often underestimated. In this study, some new data on the Pb depositional history in northeast China were provided using two ~(210)Pb-dated peat sequences from a poor fen in the Fenghuang Mountain of Heilongjiang province. Anthropogenic, detritic and atmospheric soil sources were discriminated using a two-step sequential digestion (weak acid leaching to liberate mobile Pb which is often regarded as anthropogenic Pb, especially for recent samples) and a ratio of unsupported ~(210)Pb and supported ~(210)Pb with the logic of that the 214Pb mainly represents the residual detritus (constant throughout the core) and the unsupported ~(210)Pb arises from atmospheric fallout. A higher ~(210)Pb/214Pb suggests more contributions from atmospheric deposition to the Pb content in the peat, and a ratio of 10 was defined to indicate the boundary between detritic input and atmospheric deposition. The detritic Pb was estimated to be 10–13 mg·kg~(–1), the anthropogenic Pb ranged from 10–80 mg·kg~(–1), and the atmospheric soil-derived Pb ranged from < 5 mg·kg~(–1) to 30 mg·kg~(–1). The history of anthropogenic Pb pollution over the last 150 years was reconstructed, and the calculated Pb deposition rate (AR Pb) ranged from 5 to 56 mg·m-2·yr-1. Using Ti as a reliable reference, the enrichment factor of Pb (EF Pb) relative to the upper continental crust was calculated. Both AR Pb and EF Pb increased with time, especially after the foundation of the People's Republic of China. This is consistent with increasing industrialization and coal burning in the last 60 years in northeast China. The present record of anthropogenic Pb deposition was consistent with the previous reports and an increasing trend of environmental pollution due to anthropogenic activities, in contrasts to Europe and North America which have experienced a major environmental cleanup. For the first time, this work estimates atmospheric Pb deposition via a minerotrophic peat core in China. This will enhance the use of peat archives for studies of environmental change

    Do Cross-Latitude and Local Studies Give Similar Predictions of Phytoplankton Responses to Warming? An Analysis of Monitoring Data from 504 Danish Lakes

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    Cross-latitude studies on lakes have a potential to predict how global warming may cause major changes in phytoplankton biomass and composition, e.g., the development of favourable conditions for cyanobacteria dominance. However, results from these studies may be influenced by biogeographical factors, and the conclusions may, therefore, not hold when considering local response patterns. We used monthly monitoring data from 504 lakes in Denmark—a small and homogeneous geographical region—to establish empirical relationships between key phytoplankton groups and a set of explanatory variables including total phosphorus (TP), total nitrogen (TN), lake mean depth (DEP) and water temperature (TEMP). All variables had strong effects on phytoplankton biomass and composition, but their contributions varied over the seasons, with TEMP being particularly important in June–October. We found dominance of cyanobacteria in terms of biomass and also an increase in dinophytes biomass at higher TEMP, while diatoms and chlorophytes became less important. In May, however, the TEMP effect on total phytoplankton biomass was negative, likely reflecting intensified zooplankton grazing. Our results suggest that biogeographical effects are of minor importance for the response patterns of phytoplankton to temperature and that substantial concentration reductions of TN and TP are needed in eutrophic lakes to counteract the effect of the climate change-induced increase in TEMP

    Do Cross-Latitude and Local Studies Give Similar Predictions of Phytoplankton Responses to Warming? An Analysis of Monitoring Data from 504 Danish Lakes

    No full text
    Cross-latitude studies on lakes have a potential to predict how global warming may cause major changes in phytoplankton biomass and composition, e.g., the development of favourable conditions for cyanobacteria dominance. However, results from these studies may be influenced by biogeographical factors, and the conclusions may, therefore, not hold when considering local response patterns. We used monthly monitoring data from 504 lakes in Denmark&mdash;a small and homogeneous geographical region&mdash;to establish empirical relationships between key phytoplankton groups and a set of explanatory variables including total phosphorus (TP), total nitrogen (TN), lake mean depth (DEP) and water temperature (TEMP). All variables had strong effects on phytoplankton biomass and composition, but their contributions varied over the seasons, with TEMP being particularly important in June&ndash;October. We found dominance of cyanobacteria in terms of biomass and also an increase in dinophytes biomass at higher TEMP, while diatoms and chlorophytes became less important. In May, however, the TEMP effect on total phytoplankton biomass was negative, likely reflecting intensified zooplankton grazing. Our results suggest that biogeographical effects are of minor importance for the response patterns of phytoplankton to temperature and that substantial concentration reductions of TN and TP are needed in eutrophic lakes to counteract the effect of the climate change-induced increase in TEMP

    A New Humic Acid Preparation with Addition of Silver Nanoparticles

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    Toward predicting climate change effects on lakes: a comparison of 1656 shallow lakes from Florida and Denmark reveals substantial differences in nutrient dynamics, metabolism, trophic structure, and top-down control

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    Rapid climate changes may potentially have strong impacts on the ecosystem structure and nutrient dynamics of lakes as well as implications for water quality. We used a space-for-time approach to elucidate such possible effects by comparing data from 1656 shallow lakes (mean depth 100 mu g L-1) in the FL lakes, but coverage was higher in the DK lakes at low TP. We also found lower oxygen saturation in the nutrient-rich FL lakes than in the DK lakes, suggesting lower net ecosystem production in the FL lakes. We discuss our results within the framework of climate warming

    Complexation of Dissolved Organic Matter with Trace Metal Ions in Natural Waters

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