1,252 research outputs found
Low temperature behavior of the heavy Fermion Ce3Co4Sn13
The compound Ce3Co4Sn13 is an extremely heavy cubic heavy fermion system with
a low temperature electronic specific heat of order ~4 J/mol-K2. If the
compound is nonmagnetic, it would be one of the heaviest nonmagnetic Ce-based
heavy fermions reported to date and therefore would be expected to lie
extremely close to a quantum critical point. However, a broad peak of unknown
origin is observed at 0.8 K in the specific heat and magnetic susceptibility,
suggesting the possibility of antiferromagnetic order. We present neutron
diffraction data from polycrystalline samples which do not show any sign of
magnetic scattering below 0.8 K. In addition, we present inelastic neutron
scattering data from a single crystal sample which is consistent with the 1.2 K
energy scale for Kondo spin fluctuations determined from specific heat
measurements.Comment: 4 pages, 2 figures, submitted to J. Mag. Mag. Mater. for ICM 200
Raman scattering studies of spin, charge, and lattice dynamics in Ca_{2-x}Sr_{x}RuO_{4} (0 =< x < 0.2)
We use Raman scattering to study spin, charge, and lattice dynamics in
various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by
Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the
electron-phonon interaction strength, (2) an increased temperature-dependence
of the two-magnon energy and linewidth in the antiferromagnetic insulating
phase, and (3) evidence for charge gap development, and hysteresis associated
with the structural phase change, both of which are indicative of a first-order
metal-insulator transition (T_{MI}) and a coexistence of metallic and
insulating components for T < T_{MI}
Orbital Switching and the First-Order Insulator-Metal Transition in Paramagnetic V_2O_3
The first-order metal-insulator transition (MIT) in paramagnetic
is studied within the ab-initio scheme LDA+DMFT, which merges the local density
approximation (LDA) with dynamical mean field theory (DMFT). With a fixed value
of the Coulomb , we show how the abrupt pressure driven MIT is
understood in a new picture: pressure-induced decrease of the trigonal
distortion within the strong correlation scenario (which is not obtained within
LDA). We find good quantitative agreement with switch of the orbital
occupation of and the spin state S=1
across the MIT, thermodynamics and resistivity, and the
one-electron spectral function, within this new scenario.Comment: 4 pages, 4 figures, submitted to PR
First-Order Transition to Incommensurate Phase with Broken Lattice Rotation Symmetry in Frustrated Heisenberg Model
We study a finite-temperature phase transition in the two-dimensional
classical Heisenberg model on a triangular lattice with a ferromagnetic
nearest-neighbor interaction and an antiferromagnetic
third-nearest-neighbor interaction using a Monte Carlo method. Apart from
a trivial degeneracy corresponding to O(3) spin rotations,the ground state for
has a threefold degeneracy corresponding to 120 degree lattice
rotations. We find that this model exhibits a first-order phase transition with
the breaking of the threefold symmetry when the interaction ratio is
.Comment: 4pages,5figure
Anomalous spin density distribution on oxygen and Ru in CaSrRuO: A polarised neutron diffraction study
By means of polarized neutron diffraction in a magnetic field of 7.0 T at 1.6
K an anomalously large magnetization density is observed on the in-plane oxygen
in CaSrRuO. Field-induced moments of different ions are
determined by refinement on the flipping ratios, yielding =
0.346(11) , = 0.076(6) and = 0.009(6)
. The moment on the oxygen arises from the strong hybridization
between the Ru-4d and O-2p orbitals. %The maximum entropy method is used for
the %reconstruction of the magnetization density and reveals a strongly
anisotropic The maximum entropy magnetization density reconstruction reveals a
strongly anisotropic density at the Ru site, consistent with the distribution
of the {\it xy} ( band) {\it d}-orbitals.Comment: 4 pages 3 figure
Orbital Dependent Phase Control in Ca2-xSrxRuO4
We present first-principles studies on the orbital states of the layered
perovskites CaSrRuO. The crossover from antiferromagnetic (AF)
Mott insulator for to nearly ferromagnetic (FM) metal at is
characterized by the systematic change of the orbital occupation. For the
AF side (), we present firm evidence for the ferro-orbital
ordering. It is found that the degeneracy of (or ) states is
lifted robustly due to the two-dimensional (2D) crystal-structure, even without
the Jahn-Teller distortion of RuO. This effect dominates, and the
cooperative occupation of orbital is concluded. In contrast to recent
proposals, the resulting electronic structure explains well both the observed
X-ray absorption spectra and the double peak structure of optical conductivity.
For the FM side (), however, the orbital with half filling opens a
pseudo-gap in the FM state and contributes to the spin =1/2 moment (rather
than =1 for =0.0 case) dominantly, while states are itinerant
with very small spin polarization, explaining the recent neutron data
consistently.Comment: 17 pages, 5 figure
Orbital-selective Mass Enhancements in Multi-band CaSrRuO Systems Analyzed by the Extended Drude Model
We investigated optical spectra of quasi-two-dimensional multi-band CaSrRuO systems. The extended Drude model analysis on the
ab-plane optical conductivity spectra indicates that the effective mass should
be enhanced near . Based on the sum rule argument, we showed that the
orbital-selective Mott-gap opening for the bands, the widely
investigated picture, could not be the origin of the mass enhancement. We
exploited the multi-band effects in the extended Drude model analysis, and
demonstrated that the intriguing heavy mass state near should come from
the renormalization of the band.Comment: 4 figure
Structural and magnetic aspects of the metal insulator transition in CaSrRuO
The phase diagram of CaSrRuO has been studied by neutron
diffraction on powder and single-crystalline samples. The experiments reveal
antiferromagnetic order and structural distortions characterized by tilts and
rotations of the RuO-octahedra. There is strong evidence that the
structural details of the isovalent samples tune the magnetic as well as the
electronic behavior. In particular we observe for low Sr-concentration a metal
insulator transition associated with a structural change and magnetic ordering
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