227 research outputs found
Unusual Shubnikov-de Haas oscillations in BiTeCl
We report measurements of Shubnikov-de Haas (SdH) oscillations in single
crystals of BiTeCl at magnetic fields up to 31 T and at temperatures as low as
0.4 K. Two oscillation frequencies were resolved at the lowest temperatures,
Tesla and Tesla. We also measured the
infrared optical reflectance and Hall effect; we
propose that the two frequencies correspond respectively to the inner and outer
Fermi sheets of the Rashba spin-split bulk conduction band. The bulk carrier
concentration was cm and the effective
masses for the inner and for the
outer sheet. Surprisingly, despite its low effective mass, we found that the
amplitude of is very rapidly suppressed with increasing temperature,
being almost undetectable above K
The Role of Transport Agents in MoS2 Single Crystals
We report resistivity, thermoelectric power and thermal conductivity of MoS2
single crystals prepared by chemical vapour transport (CVT) method using I2,
Br2 and TeCl4 as transport agents. The material presents low-lying donor and
acceptor levels, which dominate the in-plane charge transport. Intercalates
into the Van der Waals gap strongly influence the inter-plane resistivity.
Thermoelectric power displays the characteristics of strong electron-phonon
interaction. Detailed theoretical model of thermal conductivity reveals the
presence of high number of defects in the MoS2 structure. We show that these
defects are inherent to CVT growth method, coming mostly from the transport
agent molecules inclusion as identified by Total Reflection X-ray Fluorescence
analysis (TXRF) and in-beam activation analysis (IBAA).Comment: 17 pages, 5 figure
Tunable Polaronic Conduction in Anatase TiO2
Oxygen vacancies created in anatase TiO2 by UV photons (80–130 eV) provide an effective electron-doping mechanism and induce a hitherto unobserved dispersive metallic state. Angle resolved photoemission reveals that the quasiparticles are large polarons. These results indicate that anatase can be tuned from an insulator to a polaron gas to a weakly correlated metal as a function of doping and clarify the nature of conductivity in this material.open1192sciescopu
Universal response of the type-II Weyl semimetals phase diagram
The discovery of Weyl semimetals represents a significant advance in
topological band theory. They paradigmatically enlarged the classification of
topological materials to gapless systems while simultaneously providing
experimental evidence for the long-sought Weyl fermions. Beyond fundamental
relevance, their high mobility, strong magnetoresistance, and the possible
existence of even more exotic effects, such as the chiral anomaly, make Weyl
semimetals a promising platform to develop radically new technology. Fully
exploiting their potential requires going beyond the mere identification of
materials and calls for a detailed characterization of their functional
response, which is severely complicated by the coexistence of surface- and
bulk-derived topologically protected quasiparticles, i.e., Fermi arcs and Weyl
points, respectively. Here, we focus on the type-II Weyl semimetal class where
we find a stoichiometry-dependent phase transition from a trivial to a
non-trivial regime. By exploring the two extreme cases of the phase diagram, we
demonstrate the existence of a universal response of both surface and bulk
states to perturbations. We show that quasi-particle interference patterns
originate from scattering events among surface arcs. Analysis reveals that
topologically non-trivial contributions are strongly suppressed by spin
texture. We also show that scattering at localized impurities generate
defect-induced quasiparticles sitting close to the Weyl point energy. These
give rise to strong peaks in the local density of states, which lift the Weyl
node significantly altering the pristine low-energy Weyl spectrum. Visualizing
the microscopic response to scattering has important consequences for
understanding the unusual transport properties of this class of materials.
Overall, our observations provide a unifying picture of the Weyl phase diagram
Spin excitations in the skymion host Cu2OSeO3
We have used inelastic neutron scattering to measure the magnetic excitation
spectrum along the high-symmetry directions of the first Brillouin zone of the
magnetic skyrmion hosting compound CuOSeO. The majority of our
scattering data are consistent with the expectations of a recently proposed
model for the magnetic excitations in CuOSeO, and we report best-fit
parameters for the dominant exchange interactions. Important differences exist,
however, between our experimental findings and the model expectations. These
include the identification of two energy scales that likely arise due to
neglected anisotropic interactions. This feature of our work suggests that
anisotropy should be considered in future theoretical work aimed at the full
microscopic understanding of the emergence of the skyrmion state in this
material.Comment: 5 pages, 6 figure
In situ control of the helical and skyrmion phases in Cu2OSeO3 using high-pressure helium gas up to 5 kbar
We report a small-angle neutron scattering study of the helical and skyrmion lattice order in single crystal Cu2OSeO3 under quasihydrostatic helium gas pressures up to 5 kbar. By using helium gas as the pressure-transmitting medium (PTM) we ensure pressure application with improved hydrostaticity at cryogenic temperatures compared with previous reports where liquid PTMs were used. For 5-kbar He gas pressure we observe modest changes of the ambient pressure phase diagram; the critical temperature Tc changes by +2.8(2)%, while in the low-T limit the helical propagation vector |q| changes by −0.5(2)%, the lower critical field Hc1 changes by +2.5(1.0)%, and the upper critical field Hc2 remains unchanged within uncertainty. The skyrmion phase also changes little under pressure; its largest T extent varies from Tc − 2.5(5) K at ambient pressure to Tc − 3.0(5) K at 5 kbar, and its location in the phase diagram follows the pressure-driven shift of Tc. The weak pressure dependences of the critical magnetic fields and skyrmion phase contrast strongly with much stronger pressure-driven changes reported from previous quasihydrostatic pressure studies. Taking into account the present results and those of other uniaxial pressure data, we suggest that the results of previous quasihydrostatic pressure studies were influenced by inadvertent directional stress pressure components. Overall, our study represents a high-pressure study of the chiral magnetism in Cu2OSeO3 under the most hydrostatic high-pressure conditions to date and serves also as a salient reminder of the sensitivity of chiral magnets to deviations from hydrostaticity in quasihydrostatic high-pressure studies
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