34 research outputs found
Microscopic model for Bose-Einstein condensation and quasiparticle decay
Sufficiently dimerized quantum antiferromagnets display elementary S=1
excitations, triplon quasiparticles, protected by a gap at low energies. At
higher energies, the triplons may decay into two or more triplons. A strong
enough magnetic field induces Bose-Einstein condensation of triplons. For both
phenomena the compound IPA-CuCl3 is an excellent model system. Nevertheless no
quantitative model was determined so far despite numerous studies. Recent
theoretical progress allows us to analyse data of inelastic neutron scattering
(INS) and of magnetic susceptibility to determine the four magnetic couplings
J1=-2.3meV, J2=1.2meV, J3=2.9meV and J4=-0.3meV. These couplings determine
IPA-CuCl3 as system of coupled asymmetric S=1/2 Heisenberg ladders
quantitatively. The magnetic field dependence of the lowest modes in the
condensed phase as well as the temperature dependence of the gap without
magnetic field corroborate this microscopic model.Comment: 6 pages, 5 figure
Adapted continuous unitary transformation to treat systems with quasiparticles of finite lifetime
An improved generator for continuous unitary transformations is introduced to
describe systems with unstable quasiparticles. Its general properties are
derived and discussed. To illustrate this approach we investigate the
asymmetric antiferromagnetic spin-1/2 Heisenberg ladder which allows for
spontaneous triplon decay. We present results for the low energy spectrum and
the momentum resolved spectral density of this system. In particular, we show
the resonance behavior of the decaying triplon explicitly.Comment: 40 pages, 12 figure
Hole Dispersions for Antiferromagnetic Spin-1/2 Two-Leg Ladders by Self-Similar Continuous Unitary Transformations
The hole-doped antiferromagnetic spin-1/2 two-leg ladder is an important
model system for the high- superconductors based on cuprates. Using the
technique of self-similar continuous unitary transformations we derive
effective Hamiltonians for the charge motion in these ladders. The key
advantage of this technique is that it provides effective models explicitly in
the thermodynamic limit. A real space restriction of the generator of the
transformation allows us to explore the experimentally relevant parameter
space. From the effective Hamiltonians we calculate the dispersions for single
holes. Further calculations will enable the calculation of the interaction of
two holes so that a handle of Cooper pair formation is within reach.Comment: 16 pages, 26 figure
From Gapped Excitons to Gapless Triplons in One Dimension
Often, exotic phases appear in the phase diagrams between conventional
phases. Their elementary excitations are of particular interest. Here, we
consider the example of the ionic Hubbard model in one dimension. This model is
a band insulator (BI) for weak interaction and a Mott insulator (MI) for strong
interaction. Inbetween, a spontaneously dimerized insulator (SDI) occurs which
is governed by energetically low-lying charge and spin degrees of freedom.
Applying a systematically controlled version of the continuous unitary
transformations (CUTs) we are able to determine the dispersions of the
elementary charge and spin excitations and of their most relevant bound states
on equal footing. The key idea is to start from an externally dimerized system
using the relative weak interdimer coupling as small expansion parameter which
finally is set to unity to recover the original model.Comment: 18 pages, 10 figure
Size-Selected Ag Nanoparticles with Five-Fold Symmetry
Silver nanoparticles were synthesized using the inert gas aggregation technique. We found the optimal experimental conditions to synthesize nanoparticles at different sizes: 1.3 ± 0.2, 1.7 ± 0.3, 2.5 ± 0.4, 3.7 ± 0.4, 4.5 ± 0.9, and 5.5 ± 0.3 nm. We were able to investigate the dependence of the size of the nanoparticles on the synthesis parameters. Our data suggest that the aggregation of clusters (dimers, trimer, etc.) into the active zone of the nanocluster source is the predominant physical mechanism for the formation of the nanoparticles. Our experiments were carried out in conditions that kept the density of nanoparticles low, and the formation of larges nanoparticles by coalescence processes was avoided. In order to preserve the structural and morphological properties, the impact energy of the clusters landing into the substrate was controlled, such that the acceleration energy of the nanoparticles was around 0.1 eV/atom, assuring a soft landing deposition. High-resolution transmission electron microscopy images showed that the nanoparticles were icosahedral in shape, preferentially oriented with a five-fold axis perpendicular to the substrate surface. Our results show that the synthesis by inert gas aggregation technique is a very promising alternative to produce metal nanoparticles when the control of both size and shape are critical for the development of practical applications
Softlanding and STM imaging of Ag (561) clusters on a C (60) monolayer
The low energy deposition of silver cluster cations with 561 (+/- 5) atoms on a cold fullerene covered gold surface has been studied both by scanning tunneling microscopy and molecular dynamics simulation. The special properties of the C-60/Au(111) surface result in a noticeable fixation of the clusters without a significant change of the cluster shape. Upon heating to room temperature we observe a flattening or shrinking of the cluster samples due to thermal activation. Similar changes were observed also for mass selected Ag clusters with other sizes. For comparison we also studied Ag islands of similar size, grown by low temperature deposition of Ag atoms and subsequent annealing. A completely different behavior is observed with much broader size distributions and a qualitatively different response to annealing