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Relating supercooling and glass-like arrest of kinetics for phase separated systems: studies on doped CeFe and (La,Pr,Ca)MnO
Coexisting ferromagnetic and antiferromagnetic phases over a range of
temperature as well as magnetic field have been reported in many materials of
current interest, showing disorder-broadened 1st order transitions. Anomalous
history effects observed in magnetization and resistivity are being explained
invoking the concepts of kinetic arrest akin to glass transitions. From
magnetization measurements traversing novel paths in field-temperature space,
we obtain the intriguing result that the regions of the sample which can be
supercooled to lower temperatures undergo kinetic-arrest at higher
temperatures, and vice versa. Our results are for two diverse systems viz. the
inter-metallic doped CeFe which has an antiferromagnetic ground state, and
the oxide La-Pr-Ca-Mn-O which has a ferromagnetic ground state, indicating the
possible universality of this effect of disorder on the widely encountered
phenomenon of glass-like arrest of kinetics
Studies on Magnetic-field induced first-order transitions
We shall discuss magnetization and transport measurements in materials
exhibiting a broad first-order transition. The phase transitions would be
caused by varying magnetic field as well as by varying temperature, and we
concentrate on ferromagnetic to antiferromagnetic transitions in magnetic
materials. We distinguish between metastable supercooled phases and metastable
glassy phase.Comment: 50th Golden Jubilee Solid State Physics Symposium during Dec.5-9
(2005) in Mumbai - manuscript of Invited tal
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