25 research outputs found
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Modeling planetary interiors in laser based experiments using shockless compression
X-ray diffraction is a widely used technique for measuring the crystal structure of a compressed material. Recently, short pulse x-ray sources have been used to measure the crystal structure in-situ while a sample is being dynamically loaded. To reach the ultra high pressures that are unattainable in static experiments at temperatures lower than using shock techniques, shockless quasi-isentropic compression is required. Shockless compression has been demonstrated as a successful means of accessing high pressures. The National Ignition Facility (NIF), which will begin doing high pressure material science in 2010, it should be possible to reach over 2 TPa quasi-isentropically. This paper outlines how x-ray diffraction could be used to study the crystal structure in laser driven, shocklessly compressed targets the same way it has been used in shock compressed samples. A simulation of a shockless laser driven iron is used to generate simulated diffraction signals. And recently experimental results are presented
Ultra-Lithium-Deficient Halo Stars and Blue Stragglers: A Common Origin?
We present data for four ultra-Li-deficient, warm, halo stars. The Li
deficiency of two of these is a new discovery. Three of the four stars have
effective temperatures Teff ~ 6300 K, in contrast to previously known
Li-deficient halo stars which spanned the temperature range of the Spite
Plateau. In this paper we propose that these, and previously known
ultra-Li-deficient halo stars, may have had their surface lithium abundances
reduced by the same mechanism as produces halo field blue stragglers. Even
though these stars have yet to reveal themselves as blue stragglers, they might
be regarded as "blue-stragglers-to-be." In our proposed scenario, the surface
abundance of Li in these stars could be destroyed (a) during the normal
pre-main-sequence single star evolution of their low mass precursors, (b)
during the post-main-sequence evolution of a evolved mass donor, and/or (c) via
mixing during a mass-transfer event or stellar merger. The warmest Li-deficient
stars at the turnoff would be regarded as emerging "canonical" blue stragglers,
whereas cooler ones represent sub-turnoff-mass "blue-stragglers-to-be." The
latter are presently hidden on the main sequence, Li depletion being possibly
the clearest signature of their past history and future significance.
Eventually, the main sequence turnoff will reach down to their mass, exposing
those Li-depleted stars as canonical blue stragglers when normal stars of that
mass evolve away. Arguing against this unified view is the observation that the
three Li-depleted stars at Teff ~ 6300 K are all binaries, whereas very few of
the cooler systems show evidence for binarity; it is thus possible that two
separate mechanisms are responsible for the production of Li-deficient
main-sequence halo stars.Comment: 23 pages including 3 figures. 2001, ApJ, 547, xxx (1 February
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High-pressure, High-strain-rate Materials Effects
A 3-year LDRD-ER project to study the response of shocked materials at high pressure and high strain rate has concluded. This project involved a coordinated effort to study single crystal samples that were shock loaded by direct laser irradiation, in-situ and post-recovery measurements, and molecular dynamics and continuum modeling. Laser-based shock experiments have been conducted to study the dynamic response of materials under shock loading materials at a high strain-rate. Experiments were conducted at pressures above the published Hugoniot Elastic Limit (HEL). The residual deformation present in recovered samples was characterized by transmission electron microscopy, and the response of the shocked lattice during shock loading was measured by in-situ x-ray diffraction. Static film and x-ray streak cameras recorded x-rays diffracted from lattice planes of Cu and Si both parallel and perpendicular to the shock direction. Experiments were also conducted using a wide-angle detector to record x-rays diffracted from multiple lattice planes simultaneously. This data showed uniaxial compression of Si (100) along the shock direction and 3-dimensional compression of Cu (100). In the case of the Si diffraction, there was a multiple wave structure observed. We present results of shocked Si and Cu obtained with a new large angle diffraction diagnostic, and discuss the results in the context of detailed molecular dynamics simulations and post-processing
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Material dynamics under extreme conditions of pressure and strain rate
Solid state experiments at extreme pressures (10-100 GPa) and strain rates ({approx}10{sup 6}-10{sup 8}s{sup -1}) are being developed on high-energy laser facilities, and offer the possibility for exploring new regimes of materials science. These extreme solid-state conditions can be accessed with either shock loading or with a quasi-isentropic ramped pressure drive. Velocity interferometer measurements establish the high pressure conditions. Constitutive models for solid-state strength under these conditions are tested by comparing 2D continuum simulations with experiments measuring perturbation growth due to the Rayleigh-Taylor instability in solid-state samples. Lattice compression, phase, and temperature are deduced from extended x-ray absorption fine structure (EXAFS) measurements, from which the shock-induced {alpha}-{omega} phase transition in Ti and the {alpha}-{var_epsilon} phase transition in Fe are inferred to occur on sub-nanosec time scales. Time resolved lattice response and phase can also be measured with dynamic x-ray diffraction measurements, where the elastic-plastic (1D-3D) lattice relaxation in shocked Cu is shown to occur promptly (< 1 ns). Subsequent large-scale molecular dynamics (MD) simulations elucidate the microscopic dynamics that underlie the 3D lattice relaxation. Deformation mechanisms are identified by examining the residual microstructure in recovered samples. The slip-twinning threshold in single-crystal Cu shocked along the [001] direction is shown to occur at shock strengths of {approx}20 GPa, whereas the corresponding transition for Cu shocked along the [134] direction occurs at higher shock strengths. This slip-twinning threshold also depends on the stacking fault energy (SFE), being lower for low SFE materials. Designs have been developed for achieving much higher pressures, P > 1000 GPa, in the solid state on the National Ignition Facility (NIF) laser
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DIRECT OBSERVATION OF THE ALPHA-EPSILON TRANSITION IN SHOCKED SINGLE CRYSTAL IRON
In-situ x-ray diffraction was used to study the response of single crystal iron under shock conditions. Measurements of the response of [001] iron showed a uniaxial compression of the initially bcc lattice along the shock direction by up to 6% at 13 GPa. Above this pressure, the lattice responded with a further collapse of the lattice by 15-18% and a transformation to a hcp structure. The in-situ measurements are discussed and results summarized
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PICOSECOND X-RAY DIFFRACTION FROM LASER-SHOCKED COPPER AND IRON
In situ X-ray diffraction allows the determination of the structure of transient states of matter. We have used laser-plasma generated X-rays to study how single crystals of metals (copper and iron) react to uniaxial shock compression. We find that copper, as a face-centered-cubic material, allows rapid generation and motion of dislocations, allowing close to hydrostatic conditions to be achieved on sub-nanosecond timescales. Detailed molecular dynamics calculations provide novel information about the process, and point towards methods whereby the dislocation density might be measured during the passage of the shock wave itself. We also report on recent experiments where we have obtained diffraction images from shock-compressed single-crystal iron. The single crystal sample transforms to the hcp phase above a critical pressure, below which it appears to be uniaxially compressed bcc, with no evidence of plasticity. Above the transition threshold, clear evidence for the hcp phase can be seen in the diffraction images, and via a mechanism that is also consistent with recent multi-million atom molecular dynamics simulations that use the Voter-Chen potential. We believe these data to be of import, in that they constitute the first conclusive in situ evidence of the transformed structure of iron during the passage of a shock wave
Picosecond X-ray diffraction from shock-compressed metals
In this thesis, Molecular Dynamics simulations of shocked single crystals of Copper and Iron are studied using simulated X-ray diffraction. Strains and volumetric compression in modeled Copper crystals shock-compressed on picosecond time-scales are found. By comparing the shifts in the second and fourth diffraction orders, the density of dislocations is calculated. In Iron, simulated X-ray diffraction is used to verify the modelling of the α-ε phase transition induced by shock-compression on picosecond time-scales. No plastic deformation of Iron is found in the studied pressure range of ~ 15-53 GPa. The results are then compared with data from in situ X-ray diffraction experiments of laser-shocked single crystals. Near-hydrostatic compression of shock-compressed Copper on nanosecond time-scales is confirmed using a new wide-angle film diagnostic capturing diffraction from multiple crystal planes. Also, the first in situ X-ray diffraction evidence of the onset of the α-ε phase transition in laser-shocked single crystal Iron is shown. No plastic yield of the crystal lattice is found, which is in agreement with the simulation results. Results from both the Molecular Dynamics simulations and experiments are used to suggest enhancements in computer modelling of shocked crystals, as well as future experimental studies. In particular, the need for a measurement of dislocation densities during the shock wave passage through a crystal is highlighted, and a method enabling such a measurement is proposed.</p
Picosecond X-ray diffraction from shock-compressed metals: experiments and computational analysis of molecular dynamics simulations
In this thesis, Molecular Dynamics simulations of shocked single crystals of Copper and Iron are studied using simulated X-ray diffraction. Strains and volumetric compression in modeled Copper crystals shock-compressed on picosecond time-scales are found. By comparing the shifts in the second and fourth diffraction orders, the density of dislocations is calculated. In Iron, simulated X-ray diffraction is used to verify the modelling of the α-ε phase transition induced by shock-compression on picosecond time-scales. No plastic deformation of Iron is found in the studied pressure range of ~ 15-53 GPa. The results are then compared with data from in situ X-ray diffraction experiments of laser-shocked single crystals. Near-hydrostatic compression of shock-compressed Copper on nanosecond time-scales is confirmed using a new wide-angle film diagnostic capturing diffraction from multiple crystal planes. Also, the first in situ X-ray diffraction evidence of the onset of the α-ε phase transition in laser-shocked single crystal Iron is shown. No plastic yield of the crystal lattice is found, which is in agreement with the simulation results. Results from both the Molecular Dynamics simulations and experiments are used to suggest enhancements in computer modelling of shocked crystals, as well as future experimental studies. In particular, the need for a measurement of dislocation densities during the shock wave passage through a crystal is highlighted, and a method enabling such a measurement is proposed
Measuring stacking fault densities in shock-compressed FCC crystals using in situ x-ray diffraction
A method is presented of in situ measurements of stacking fault densities in shocked face-centred-cubic (FCC) crystals using x-ray diffraction. Using results from both the second and fourth diffraction orders, wherein shifts in the Bragg peaks due to faulting are accounted for, we calculated fault densities present in a molecular dynamics (MD) simulation of shocked single crystal of copper. The results are in good quantitative agreement with dislocation density measurements inferred directly from the MD simulation. The x-ray diffraction method thus presents a real possibility for experimental determination in real time of dislocation densities in crystals during shock wave passage. © 2006 IOP Publishing Ltd