NMR detection with an atomic magnetometer

We demonstrate detection of NMR signals using a non-cryogenic atomic magnetometer and describe several novel applications of this technique. A water free induction decay (FID) signal in a 0.5 $\mu$T field is detected using a spin-exchange-relaxation-free K magnetometer and the possibility of using a multi-channel magnetometer for 3-D MRI requiring only a single FID signal is described. We also demonstrate detection of less than $10^{13}$ $^{129}$Xe atoms whose NMR signal is enhanced by a factor of 540 due to Fermi-contact interaction with K atoms. This technique allows detection of less than $10^{9}$ $^{129}$Xe spins in a flowing system suitable for remote NMR applications

High-Temperature Alkali Vapor Cells with Anti-Relaxation Surface Coatings

Antirelaxation surface coatings allow long spin relaxation times in alkali-metal cells without buffer gas, enabling faster diffusion of the alkali atoms throughout the cell and giving larger signals due to narrower optical linewidths. Effective coatings were previously unavailable for operation at temperatures above 80 C. We demonstrate that octadecyltrichlorosilane (OTS) can allow potassium or rubidium atoms to experience hundreds of collisions with the cell surface before depolarizing, and that an OTS coating remains effective up to about 170 C for both potassium and rubidium. We consider the experimental concerns of operating without buffer gas and with minimal quenching gas at high vapor density, studying the stricter need for effective quenching of excited atoms and deriving the optical rotation signal shape for atoms with resolved hyperfine structure in the spin-temperature regime. As an example of a high-temperature application of antirelaxation coated alkali vapor cells, we operate a spin-exchange relaxation-free atomic magnetometer with sensitivity of 6 fT/sqrt(Hz) and magnetic linewidth as narrow as 2 Hz.Comment: 8 pages, 5 figures. The following article appeared in Journal of Applied Physics and may be found at http://link.aip.org/link/?jap/106/11490

Calculation of Magnetic Field Noise from High-Permeability Magnetic Shields and Conducting Objects with Simple Geometry

High-permeability magnetic shields generate magnetic field noise that can limit the sensitivity of modern precision measurements. We show that calculations based on the fluctuation-dissipation theorem allow quantitative evaluation of magnetic field noise, either from current or magnetization fluctuations, inside enclosures made of high-permeability materials. Explicit analytical formulas for the noise are derived for a few axially symmetric geometries, which are compared with results of numerical finite element analysis. Comparison is made between noises caused by current and magnetization fluctuations inside a high-permeability shield and also between current-fluctuation-induced noises inside magnetic and non-magnetic conducting shells. A simple model is suggested to predict power-law decay of noise spectra beyond quasi-static regime. Our results can be used to assess noise from existing shields and to guide design of new shields for precision measurements.Comment: 10 page

Isotropic magnetometry with simultaneous excitation of orientation and alignment CPT resonances

Atomic magnetometers have very high absolute precision and sensitivity to magnetic fields but suffer from a fundamental problem: the vectorial or tensorial interaction of light with atoms leads to "dead zones", certain orientations of magnetic field where the magnetometer loses its sensitivity. We demonstrate a simple polarization modulation scheme that simultaneously creates coherent population trapping (CPT) in orientation and alignment, thereby eliminating dead zones. Using $^{87}$Rb in a 10 Torr buffer gas cell we measure narrow, high-contrast CPT transparency peaks in all orientations and also show absence of systematic effects associated with non-linear Zeeman splitting.Comment: 4 pages, 4 figure

New limit on Lorentz and CPT-violating neutron spin interactions

We performed a search for neutron spin coupling to a Lorentz and CPT-violating background field using a magnetometer with overlapping ensembles of K and $^3$He atoms. The co-magnetometer is mounted on a rotary platform for frequent reversal of its orientation. We measure sidereal oscillations in the signal to search for anomalous spin coupling of extra-solar origin. We determine the equatorial components of the background field interacting with the neutron spin to be $\widetilde{b}^n_X = (0.1 \pm 1.6) \times 10^{-33}$ GeV and $\widetilde{b}^n_Y = (2.5 \pm 1.6) \times 10^{-33}$ GeV, improving on the previous limit by a factor of 30. This measurement represents the highest energy resolution of any spin anisotropy experiment

Correlation function of spin noise due to atomic diffusion

We use paramagnetic Faraday rotation to study spin noise spectrum from unpolarized Rb vapor in a tightly focused probe beam in the presence of N$_2$ buffer gas. We derive an analytical form for the diffusion component of the spin noise time-correlation function in a Gaussian probe beam. We also obtain analytical forms for the frequency spectrum of the spin noise in the limit of a tightly focused or a collimated Gaussian beam in the presence of diffusion. In particular, we find that in a tightly focused probe beam the spectral lineshape can be independent of the buffer gas pressure. Experimentally, we find good agreement between the calculated and measured spin noise spectra for N$_2$ gas pressures ranging from 56 to 820 torr.Comment: 6 pages, 4 figure

Non-linear amplification of small spin precession using long range dipolar interactions

In measurements of small signals using spin precession the precession angle usually grows linearly in time. We show that non-linear interactions between particles can lead to an exponentially growing spin precession angle, resulting in an amplification of small signals and raising them above the noise level of a detection system. We demonstrate amplification by a factor of greater than 8 of a spin precession signal due to a small magnetic field gradient in a spherical cell filled with hyperpolarized liquid $^{129}$Xe. This technique can improve the sensitivity in many measurements that are limited by the noise of the detection system, rather then the fundamental spin-projection noise.Comment: 4 pages, 4 figure