Polydispersity Effects in the Dynamics and Stability of Bubbling Flows

The occurrence of swarms of small bubbles in a variety of industrial systems enhances their performance. However, the effects that size polydispersity may produce on the stability of kinematic waves, the gain factor, mean bubble velocity, kinematic and dynamic wave velocities is, to our knowledge, not yet well established. We found that size polydispersity enhances the stability of a bubble column by a factor of about 23% as a function of frequency and for a particular type of bubble column. In this way our model predicts effects that might be verified experimentally but this, however, remain to be assessed. Our results reinforce the point of view advocated in this work in the sense that a description of a bubble column based on the concept of randomness of a bubble cloud and average properties of the fluid motion, may be a useful approach that has not been exploited in engineering systems.Comment: 11 pages, 2 figures, presented at the 3rd NEXT-SigmaPhi International Conference, 13-18 August, 2005, Kolymbari, Cret

Momentum distributions of α\alpha-particles from decaying low-lying 12^{12}C-resonances

The complex scaled hyperspherical adiabatic expansion method is used to compute momentum and energy distributions of the three $\alpha$-particles emerging from the decay of low-lying $^{12}$C-resonances. The large distance continuum properties of the wave functions are crucial and must be accurately calculated. We discuss separately decays of natural parity states: two $0^+$, one $1^{-}$, three $2^+$, one $3^-$, two $4^+$, one $6^+$, and one of each of unnatural parity, $1^{+}$, $2^-$, $3^+$, $4^-$. The lowest natural parity state of each $J^{\pi}$ decays predominantly sequentially via the $^{8}$Be ground state whereas other states including unnatural parity states predominantly decay directly to the continuum. We present Dalitz plots and systematic detailed momentum correlations of the emerging $\alpha$-particles.Comment: 11 pages, 7 figures, accepted for publication in Physical Review

Non-gaussianity from the second-order cosmological perturbation

Several conserved and/or gauge invariant quantities described as the second-order curvature perturbation have been given in the literature. We revisit various scenarios for the generation of second-order non-gaussianity in the primordial curvature perturbation \zeta, employing for the first time a unified notation and focusing on the normalisation f_{NL} of the bispectrum. When the classical curvature perturbation first appears a few Hubble times after horizon exit, |f_{NL}| is much less than 1 and is, therefore, negligible. Thereafter \zeta (and hence f_{NL}) is conserved as long as the pressure is a unique function of energy density (adiabatic pressure). Non-adiabatic pressure comes presumably only from the effect of fields, other than the one pointing along the inflationary trajectory, which are light during inflation (`light non-inflaton fields'). During single-component inflation f_{NL} is constant, but multi-component inflation might generate |f_{NL}| \sim 1 or bigger. Preheating can affect f_{NL} only in atypical scenarios where it involves light non-inflaton fields. The curvaton scenario typically gives f_{NL} \ll -1 or f_{NL} = +5/4. The inhomogeneous reheating scenario can give a wide range of values for f_{NL}. Unless there is a detection, observation can eventually provide a limit |f_{NL}| \lsim 1, at which level it will be crucial to calculate the precise observational limit using second order theory.Comment: Latex file in Revtex style. 13 pages, 1 figure. v2: minor changes. Discussion in Subsection VI-A enlarged. References added. Conclusions unchanged. v3: minor typographic changes. Correlated and uncorrelated \chi^2 non-gaussianity concepts and consequences introduced. Section VI-A enlarged. Small change in Table I. References updated and added. Conclusions unchanged. Version to appear in Physical Review

Polyradical character and spin frustration in fullerene molecules: An ab initio non-collinear Hartree--Fock study

Most {\em ab initio} calculations on fullerene molecules have been carried out based on the paradigm of the H\"uckel model. This is consistent with the restricted nature of the independent-particle model underlying such calculations, even in single-reference-based correlated approaches. On the other hand, previous works on some of these molecules using model Hamiltonians have clearly indicated the importance of short-range inter-atomic spin-spin correlations. In this work, we consider {\em ab initio} non-collinear Hartree--Fock (HF) solutions for representative fullerene systems: the bowl, cage, ring, and pentagon isomers of C$_{20}$, and the larger C$_{30}$, C$_{36}$, C$_{60}$, C$_{70}$, and C$_{84}$ fullerene cages. In all cases but the ring we find that the HF minimum corresponds to a truly non-collinear solution with a torsional spin density wave. Optimized geometries at the generalized HF (GHF) level lead to fully symmetric structures, even in those cases where Jahn-Teller distortions have been previously considered. The nature of the GHF solutions is consistent with the $\pi$-electron space becoming polyradical in nature: each $p$-orbital remains effectively singly occupied. The spin frustration, induced by the pentagon rings in an otherwise anti-ferromagnetic background, is minimized at the HF level by aligning the spins in non-collinear arrangements. The long-range magnetic ordering observed is reminiscent of the character of broken symmetry HF solutions in polyacene systems.Comment: 16 figure