Atom-molecule dark states in a Bose-Einstein condensate

We have created a dark quantum superposition state of a Rb Bose-Einstein condensate (BEC) and a degenerate gas of Rb$_2$ ground state molecules in a specific ro-vibrational state using two-color photoassociation. As a signature for the decoupling of this coherent atom-molecule gas from the light field we observe a striking suppression of photoassociation loss. In our experiment the maximal molecule population in the dark state is limited to about 100 Rb$_2$ molecules due to laser induced decay. The experimental findings can be well described by a simple three mode model.Comment: 4 pages, 6 figure

Strong magnetic coupling of an ultracold gas to a superconducting waveguide cavity

Placing an ensemble of $10^6$ ultracold atoms in the near field of a superconducting coplanar waveguide resonator (CPWR) with $Q \sim 10^6$ one can achieve strong coupling between a single microwave photon in the CPWR and a collective hyperfine qubit state in the ensemble with $g_\textit{eff} / {2 \pi} \sim 40$ kHz larger than the cavity line width of ${\kappa}/{2 \pi} \sim 7$ kHz. Integrated on an atomchip such a system constitutes a hybrid quantum device, which also can be used to interconnect solid-state and atomic qubits, to study and control atomic motion via the microwave field, observe microwave super-radiance, build an integrated micro maser or even cool the resonator field via the atoms

Master Equation for the Motion of a Polarizable Particle in a Multimode Cavity

We derive a master equation for the motion of a polarizable particle weakly interacting with one or several strongly pumped cavity modes. We focus here on massive particles with complex internal structure such as large molecules and clusters, for which we assume a linear scalar polarizability mediating the particle-light interaction. The predicted friction and diffusion coefficients are in good agreement with former semiclassical calculations for atoms and small molecules in weakly pumped cavities, while the current rigorous quantum treatment and numerical assessment sheds a light on the feasibility of experiments that aim at optically manipulating beams of massive molecules with multimode cavities.Comment: 30 pages, 5 figure

Collective Electronic Excitation Coupling between Planar Optical Lattices using Ewald's Method

Using Ewald's summation method we investigate collective electronic excitations (excitons) of ultracold atoms in parallel planar optical lattices including long range interactions. The exciton dispersion relation can then be suitably rewritten and efficiently calculated for long range resonance dipole-dipole interactions. Such in-plane excitons resonantly couple for two identical optical lattices, with an energy transfer strength decreasing exponentially with the distance between the lattices. This allows a restriction of the transfer to neighboring planes and gives rise to excitons delocalized between the lattices. In general equivalent results will hold for any planar system containing lattice layers of optically active and dipolar materials.Comment: 6 pages, and 7 figure

Optical Properties of Collective Excitations for Finite Chains of Trapped Atoms

Resonant dipole-dipole interaction modifies the energy and decay rate of electronic excitations for finite one dimensional chains of ultracold atoms in an optical lattice. We show that collective excited states of the atomic chain can be divided into dark and bright modes, where a superradiant mode with an enhanced collective effective dipole dominates the optical scattering. Studying the generic case of two chain segments of different length and position exhibits an interaction blockade and spatially structured light emission. Ultimately, an extended system of several interfering segments models a long chain with randomly distributed defects of vacant sites. The corresponding emission pattern provides a sensitive tool to study structural and dynamical properties of the system.Comment: 8 pages, 12 figure

Prospects for the cavity-assisted laser cooling of molecules

Cooling of molecules via free-space dissipative scattering of photons is thought not to be practicable due to the inherently large number of Raman loss channels available to molecules and the prohibitive expense of building multiple repumping laser systems. The use of an optical cavity to enhance coherent Rayleigh scattering into a decaying cavity mode has been suggested as a potential method to mitigate Raman loss, thereby enabling the laser cooling of molecules to ultracold temperatures. We discuss the possibility of cavity-assisted laser cooling particles without closed transitions, identify conditions necessary to achieve efficient cooling, and suggest solutions given experimental constraints. Specifically, it is shown that cooperativities much greater than unity are required for cooling without loss, and that this could be achieved via the superradiant scattering associated with intracavity self-localization of the molecules. Particular emphasis is given to the polar hydroxyl radical (OH), cold samples of which are readily obtained from Stark deceleration.Comment: 18 pages, 10 figure

Role of electromagnetically induced transparency in resonant four-wave-mixing schemes.

Published versio

Phase-dependent spectra in a driven two-level atom

We propose a method to observe phase-dependent spectra in resonance fluorescence, employing a two-level atom driven by a strong coherent field and a weak, amplitude-fluctuating field. The spectra are similar to those which occur in a squeezed vacuum, but avoid the problem of achieving squeezing over a $4\pi$ solid angle. The system shows other interesting features, such as pronounced gain without population inversion.Comment: 4 pages and 4 figures. Submitted to Phys. Rev. Let

Dark resonances for ground state transfer of molecular quantum gases

One possible way to produce ultracold, high-phase-space-density quantum gases of molecules in the rovibronic ground state is given by molecule association from quantum-degenerate atomic gases on a Feshbach resonance and subsequent coherent optical multi-photon transfer into the rovibronic ground state. In ultracold samples of Cs_2 molecules, we observe two-photon dark resonances that connect the intermediate rovibrational level |v=73,J=2> with the rovibrational ground state |v=0,J=0> of the singlet $X^1\Sigma_g^+$ ground state potential. For precise dark resonance spectroscopy we exploit the fact that it is possible to efficiently populate the level |v=73,J=2> by two-photon transfer from the dissociation threshold with the stimulated Raman adiabatic passage (STIRAP) technique. We find that at least one of the two-photon resonances is sufficiently strong to allow future implementation of coherent STIRAP transfer of a molecular quantum gas to the rovibrational ground state |v=0,J=0>.Comment: 7 pages, 4 figure

Influence of a Feshbach resonance on the photoassociation of LiCs

We analyse the formation of ultracold 7Li133Cs molecules in the rovibrational ground state through photoassociation into the B1Pi state, which has recently been reported [J. Deiglmayr et al., Phys. Rev. Lett. 101, 133004 (2008)]. Absolute rate constants for photoassociation at large detunings from the atomic asymptote are determined and are found to be surprisingly large. The photoassociation process is modeled using a full coupled-channel calculation for the continuum state, taking all relevant hyperfine states into account. The enhancement of the photoassociation rate is found to be caused by an `echo' of the triplet component in the singlet component of the scattering wave function at the inner turning point of the lowest triplet a3Sigma+ potential. This perturbation can be ascribed to the existence of a broad Feshbach resonance at low scattering energies. Our results elucidate the important role of couplings in the scattering wave function for the formation of deeply bound ground state molecules via photoassociation.Comment: Added Erratum, 20 pages, 9 figure