44 research outputs found
Tunable Metasurface and Flat Optical Zoom Lens on a Stretchable Substrate
A mechanically reconfigurable metasurface
that can continuously tune the wavefront is demonstrated in the visible
frequency range by changing the lattice constant of a complex Au nanorod
array fabricated on a stretchable polydimethylsiloxane substrate.
It is shown that the anomalous refraction angle of visible light at
632.8 nm interacting with the tunable metasurface can be adjusted
from 11.4° to 14.9° by stretching the substrate by ∼30%.
An ultrathin flat 1.7× zoom lens whose focal length can continuously
be changed from 150 to 250 μm is realized, which also demonstrates
the potential of utilizing metasurfaces for reconfigurable flat optics
Factors used for assessing the annual incidence and 5-year period prevalence of chronic pulmonary aspergillosis (CPA) as a sequel to pulmonary tuberculosis.
<p>Factors used for assessing the annual incidence and 5-year period prevalence of chronic pulmonary aspergillosis (CPA) as a sequel to pulmonary tuberculosis.</p
Crystallographic Characterization of II–VI Semiconducting Nanostructures via Optical Second Harmonic Generation
We demonstrate the utility of optical
second harmonic generation (SHG) polarimetry to perform structural
characterization of noncentrosymmetric, single-crystalline II–VI
semiconducting nanowires, nanobelts, and nanoflakes. By analyzing
anisotropic SHG polarimetric patterns, we distinguish between wurtzite
and zincblende II–VI semiconducting crystal structures and
determine their growth orientation. The crystallography of these nanostructures
was then confirmed via transmission electron microscopy measurements
performed on the same system. In addition, we show that some intrinsic
material properties such as nonlinear coefficients and geometry-dependent
optical in-coupling coefficients can also be determined from the SHG
experiments in WZ nanobelts. The ability to perform SHG-based structural
characterization and crystallographic study of II–VI semiconducting
single-crystalline nanomaterials will be useful to correlate structure–property
relationships of nanodevices on which transmission electron microscopy
measurements cannot be typically performed
Pulmonary tuberculosis (TB) estimates in the Indian population.
<p>CPA: chronic pulmonary aspergillosis.</p><p>Pulmonary tuberculosis (TB) estimates in the Indian population.</p
Estimated burden of allergic bronchopulmonary aspergillosis (ABPA) and severe asthma with fungal sensitization (SAFS) in adult Indian population with different rates of prevalence of ABPA in adult (≧15 years) asthmatic patients.
<p>Estimated burden of allergic bronchopulmonary aspergillosis (ABPA) and severe asthma with fungal sensitization (SAFS) in adult Indian population with different rates of prevalence of ABPA in adult (≧15 years) asthmatic patients.</p
Studies of Hot Photoluminescence in Plasmonically Coupled Silicon via Variable Energy Excitation and Temperature-Dependent Spectroscopy
By integrating silicon
nanowires (∼150 nm diameter, 20 μm
length) with an Ω-shaped plasmonic nanocavity, we are able to
generate broadband visible luminescence, which is induced by high
order hybrid nanocavity-surface plasmon modes. The nature of this
super bandgap emission is explored via photoluminescence spectroscopy
studies performed with variable laser excitation energies (1.959 to
2.708 eV) and finite difference time domain simulations. Furthermore,
temperature-dependent photoluminescence spectroscopy shows that the
observed emission corresponds to radiative recombination of unthermalized
(hot) carriers as opposed to a resonant Raman process
Nanotwin Detection and Domain Polarity Determination via Optical Second Harmonic Generation Polarimetry
We demonstrate that
optical second harmonic generation (SHG) can be utilized to determine
the exact nature of nanotwins in noncentrosymmetric crystals, which
is challenging to resolve via conventional transmission electron or
scanned probe microscopies. Using single-crystalline nanotwinned CdTe
nanobelts and nanowires as a model system, we show that SHG polarimetry
can distinguish between upright (Cd–Te bonds) and inverted
(Cd–Cd or Te–Te bonds) twin boundaries in the system.
Inverted twin boundaries are generally not reported in nanowires due
to the lack of techniques and complexity associated with the study
of the nature of such defects. Precise characterization of the nature
of defects in nanocrystals is required for deeper understanding of
their growth and physical properties to enable their application in
future devices
Strain-Induced Large Exciton Energy Shifts in Buckled CdS Nanowires
Strain
engineering can be utilized to tune the fundamental properties of
semiconductor materials for applications in advanced electronic and
photonic devices. Recently, the effects of large strain on the properties
of nanostructures are being intensely investigated to further expand
our insights into the physics and applications of such materials.
In this Letter, we present results on controllable buckled cadmium-sulfide
(CdS) optical nanowires (NWs), which show extremely large energy bandgap
tuning by >250 meV with applied strains within the elastic deformation
limit. Polarization and spatially resolved optical measurements reveal
characteristics related to both compressive and tensile regimes, while
microreflectance
spectroscopy clearly demonstrates the effect of strain on the different
types of excitons in CdS. Our results may enable strained NWs-based
optoelectronic devices with tunable optical responses
Uniform Bimetallic Nanocrystals by High-Temperature Seed-Mediated Colloidal Synthesis and Their Catalytic Properties for Semiconducting Nanowire Growth
A general
procedure to prepare uniform gold-based bimetallic nanocrystals
(NCs) is reported. The method relies on a seed-mediated approach in
which deposition and <i>in-situ</i> alloying of a second
metal (Ag, Pt, Hg, Sn, Cd) onto monodisperse Au seeds are performed
at relatively high temperatures, giving access to bimetallic NCs of
tunable compositions and properties. The position of the plasmon resonance
in the original Au NCs is tunable over a wide range (∼300–520
nm) of the electromagnetic spectrum. We demonstrate the catalytic
properties of these monodisperse NCs for growing single-crystalline
semiconductor nanowires of uniform, small diameter (∼15–30
nm) via a vapor–liquid–solid (VLS) mechanism at low
temperatures. This seeded-mediated approach is not restricted to Au
but can be extended to several other combinations, making this procedure
a straightforward method to prepare highly monodisperse and controllable
multimetallic nanocrystals for optical and catalytic applications