3,318 research outputs found
Pressure-induced phase transition and bi-polaronic sliding in a hole-doped Cu_2O_3 ladder system
We study a hole-doped two-leg ladder system including metal ions, oxygen, and
electron-lattice interaction, as a model for Sr_{14-x}Ca_xCu_{24}O_{41-\delta}.
Single- and bi-polaronic states at 1/4-hole doping are modeled as functions of
pressure by applying an unrestricted Hartree-Fock approximation to a multiband
Peierls-Hubbard Hamiltonian. We find evidence for a pressure-induced phase
transition between single-polaron and bi-polaron states. The electronic and
phononic excitations in those states, including distinctive local lattice
vibrational modes, are calculated by means of a direct-space Random Phase
approximation. Finally, as a function of pressure, we identify a transition
between site- and bond-centered bi-polarons, accompanied by a soft mode and a
low-energy charge-sliding mode. We suggest comparisons with available
experimented data
Raman scattering from the CaC6 superconductor in the presence of disorder
Polarized Raman scattering has been performed on CaC6 superconductor. We
identify two of the three Raman active Eg phonon modes at 440 and 1508 cm-1
expected for the R-3m space group of CaC6. These first order scattering modes
appear along with the D and G bands around 1300 cm-1 and 1600 cm-1 that are
similar in origin to the corresponding bands in plain graphite. The intensities
of the D and G bands in CaC6 correlate with degree of disorder. The D band
arises from the double resonant Raman scattering process; its frequency shifts
as a function of excitation energy with approximately 35 cm-1/eV. The double
resonant Raman scattering probes phonon excitations with finite wave vector q.
We estimate the characteristic spacing of structural defects to be on the scale
of about 100 Angstrom by comparing the intensity of the D band and the 1508
cm-1 Eg mode in CaC6 to calibrated intensity ratio of analogous bands in
disordered graphites. A sharp superconducting coherence peak at 24 cm-1 is
observed below Tc.Comment: 10 pages, 5 figure
Nonmonotonic d_{x^2-y^2} Superconducting Order Parameter in Nd_{2-x}Ce_xCuO_4
Low energy polarized electronic Raman scattering of the electron doped
superconductor Nd_1.85Ce_0.15CuO_4 (T_c=22 K) has revealed a nonmonotonic
d_{x^2-y^2} superconducting order parameter. It has a maximum gap of 4.4 k_BT_c
at Fermi surface intersections with antiferromagnetic Brillouin zone (the ``hot
spots'') and a smaller gap of 3.3 k_BT_c at fermionic Brillouin zone
boundaries. The gap enhancement in the vicinity of the ``hot spots'' emphasizes
role of antiferromagnetic fluctuations and similarity in the origin of
superconductivity for electron- and hole-doped cuprates.Comment: 4 pages, 4 figure
Observation of a 500meV Collective Mode in LaSrCuO and NdCuO
Utilizing resonant inelastic x-ray scattering, we report a previously
unobserved mode in the excitation spectrum of LaSrCuO at 500
meV. The mode is peaked around the (,0) point in reciprocal space and is
observed to soften, and broaden, away from this point. Samples with x=0, 0.01,
0.05, and 0.17 were studied. The new mode is found to be rapidly suppressed
with increasing Sr content and is absent at =0.17, where it is replaced by a
continuum of excitations. The peak is only observed when the incident x-ray
polarization is normal to the CuO planes and is also present in NdCuO.
We suggest possible explanations for this excitation.Comment: 5 pages, 5 figure
Developing customized stepwise MIRU-VNTR typing for tuberculosis surveillance in Georgia
INTRODUCTION: Mycobacterial Interspersed Repetitive Units-Variable Tandem Repeats (MIRU-VNTR) typing has been widely used for molecular epidemiological studies of tuberculosis (TB). However, genotyping tools for Mycobacterium tuberculosis (Mtb) may be limiting in some settings due to high cost and workload. In this study developed a customized stepwise MIRU-VNTR typing that prioritizes high discriminatory loci and validated this method using penitentiary system cohort in the country of Georgia. METHODS: We used a previously generated MIRU-VNTR dataset from recurrent TB cases (32 cases) in Georgia and a new dataset of TB cases from the penitentiary system (102 cases) recruited from 2014 to 2015. A Hunter-Gaston Discriminatory Index (HGDI) was calculated utilizing a 24 standard loci panel, to select high discriminatory power loci, subsequently defined as the customized Georgia-specific set of loci for initial typing. The remaining loci were scored and hierarchically grouped for second and third step typing of the cohort. We then compared the processing time and costs of the customized stepwise method to the standard 24-loci method. RESULTS: For the customized Georgia-specific set that was used for initial typing, 10 loci were selected with a minimum value of 0.32 to the highest HGDI score locus. Customized 10 loci (step 1) typing of 102 Mtb patient isolates revealed 35.7% clustered cases. This proportion was reduced to 19.5% after hierarchical application of 2nd and 3rd step typing with the corresponding groups of loci. Our customized stepwise MIRU-VNTR genotyping approach reduced the quantity of samples to be typed and therefore overall processing time and costs by 42.6% each. CONCLUSION: Our study shows that our customized stepwise MIRU-VNTR typing approach is a valid alternative of standard MIRI-VNTR typing panels for molecular epidemiological investigation in Georgia that saves time, workload and costs. Similar approaches could be developed for other settings
Coccidioidomycosis Transmission Through Organ Transplantation: A Report of the OPTN Ad Hoc Disease Transmission Advisory Committee
Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/134822/1/ajt13950.pdfhttp://deepblue.lib.umich.edu/bitstream/2027.42/134822/2/ajt13950_am.pd
Evolution of Superconductivity in Electron-Doped Cuprates: Magneto-Raman Spectroscopy
The electron-doped cuprates Pr_{2-x}Ce_xCuO_4 and Nd_{2-x}Ce_xCuO_4 have been
studied by electronic Raman spectroscopy across the entire region of the
superconducting (SC) phase diagram. The SC pairing strength is found to be
consistent with a weak-coupling regime except in the under-doped region where
we observe an in-gap collective mode at 4.5 k_{B}T_c while the maximum
amplitude of the SC gap is ~8 k_{B}T_{c}. In the normal state, doped carriers
divide into coherent quasi-particles (QPs) and carriers that remain incoherent.
The coherent QPs mainly reside in the vicinity of (\pi/2, \pi/2) regions of the
Brillouin zone (BZ). We find that only coherent QPs contribute to the
superfluid density in the B_{2g} channel. The persistence of SC coherence peaks
in the B_{2g} channel for all dopings implies that superconductivity is mainly
governed by interactions between the hole-like coherent QPs in the vicinity of
(\pi/2, \pi/2) regions of the BZ. We establish that superconductivity in the
electron-doped cuprates occurs primarily due to pairing and condensation of
hole-like carriers. We have also studied the excitations across the SC gap by
Raman spectroscopy as a function of temperature (T) and magnetic field (H) for
several different cerium dopings (x). Effective upper critical field lines
H*_{c2}(T, x) at which the superfluid stiffness vanishes and
H^{2\Delta}_{c2}(T, x) at which the SC gap amplitude is suppressed by field
have been determined; H^{2\Delta}_{c2}(T, x) is larger than H*_{c2}(T, x) for
all doping concentrations. The difference between the two quantities suggests
the presence of phase fluctuations that increase for x< 0.15. It is found that
the magnetic field suppresses the magnitude of the SC gap linearly at
surprisingly small fields.Comment: 13 pages, 8 figures; submitted to Phys. Rev.
Reply to Comment on:"Nonmonotonic d_{x^2-y^2} Superconducting Order Parameter in Nd_{2-x}Ce_xCuO_4"
We confirm that all the results of scanning SQUID, tunneling, ARPES,
penetration depth and Raman experiments are consistent with a nonmonotonic
d_{x^2-y^2} superconducting order parameter proposed in Phys. Rev. Lett., 88,
107002 (2002).Comment: Reply to Comment by F. Venturini, R. Hackl, and U. Michelucci
cond-mat/020541
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