3,687 research outputs found
Tunneling splitting of magnetic levels in Fe8 detected by 1H NMR cross relaxation
Measurements of proton NMR and the spin lattice relaxation rate 1/T1 in the
octanuclear iron (III) cluster [Fe8(N3C6H15)6O2(OH)12][Br8 9H2O], in short Fe8,
have been performed at 1.5 K in a powder sample aligned along the main
anisotropy z axis, as a function of a transverse magnetic field (i.e.,
perpendicular to the main easy axis z). A big enhancement of 1/T1 is observed
over a wide range of fields (2.5-5 T), which can be attributed to the tunneling
dynamics; in fact, when the tunneling splitting of the pairwise degenerate
m=+-10 states of the Fe8 molecule becomes equal to the proton Larmor frequency
a very effective spin lattice relaxation channel for the nuclei is opened. The
experimental results are explained satisfactorily by considering the
distribution of tunneling splitting resulting from the distribution of the
angles in the hard xy plane for the aligned powder, and the results of the
direct diagonalization of the model Hamiltonian.Comment: J. Appl. Phys., in pres
Magnetisation of hole-doped CuO2 spin chains in Sr14-xCaxCu24O41
We report on magnetisation measurements of Sr14-xCaxCu24O41, with 0 <= x <=
12, in magnetic fields up to 16 T. The low temperature magnetic response of the
CuO2 spin chains changes strongly upon doping. For x = 0, the ground state with
nearly independent dimers is confirmed. Reduction of the number of holes in the
chains through Ca-doping leads to an additional contribution to the
magnetisation, which depends linearly on the magnetic field. Remarkably, the
slope of this linear contribution increases with the Ca content. We argue that
antiferromagnetic spin chains do not account for this behaviour but that the
hole dynamics might be involved.Comment: In v2, spelling of author names has been change
Anomalous pressure effect on the remanent lattice striction of a (La,Pr)SrMnO bilayered manganite single crystal
We have studied the pressure effect on magnetostriction, both in the
-plane and along the c-axis, of a (La,Pr)SrMnO
bilayered manganite single crystal over the temperature region where the
field-induced ferromagnetic metal (FMM) transition takes place. For comparison,
we have also examined the pressure dependence of magnetization curves at the
corresponding temperatures. The applied pressure reduces the critical field of
the FMM transition and it enhances the remanent magnetostriction. An anomalous
pressure effect on the remanent lattice relaxation is observed and is similar
to the pressure effect on the remanent magnetization along the c-axis. These
findings are understood from the view point that the double-exchange
interaction driven FMM state is strengthened by application of pressure.Comment: 7 pages,7 figure
Inhomogeneous electronic structure probed by spin-echo experiments in the electron doped high-Tc superconductor Pr_{1.85}Ce_{0.15}CuO_{4-y}
63Cu nuclear magnetic resonance (NMR) spin-echo decay rate (T_2^{-1})
measurements are reported for the normal and superconducting states of a single
crystal of Pr_{1.85}Ce_{0.15}CuO_{4-y} (PCCO) in a magnetic field B_0=9T over
the temperature range 2K<T<200K. The spin-echo decay rate is
temperature-dependent for T<55K, and has a substantial dependence on the radio
frequency (rf) pulse parameters below T~25K. This dependence indicates that
T_2^{-1} is strongly effected by a local magnetic field distribution that can
be modified by the rf pulses, including ones that are not at the nuclear Larmor
frequency. The low-temperature results are consistent with the formation of a
static inhomogeneous electronic structure that couples to the rf fields of the
pulses.Comment: 4 pages, 4 figure
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Steplike Lattice Deformation of Single Crystalline (LaPr)SrMnO Bilayered Manganite
We report a steplike lattice transformation of single crystalline
(LaPr)SrMnObilayered manganite
accompanied by both magnetization and magnetoresistive jumps, and examine the
ultrasharp nature of the field-induced first-order transition from a
paramagnetic insulator to a ferromagnetic metal phase accompanied by a huge
decrease in resistance. Our findings support that the abrupt magnetostriction
is closely related to an orbital frustration existing in the inhomogeneous
paramagnetic insulating phase rather than a martensitic scenario between
competing two phases.Comment: 5 pages,4figures, v4: figures are changed, in press in Phys.Rev.Let
Possible Magnetic Chirality in Optically Chiral Magnet [Cr(CN)][Mn()-pnH(HO)](HO) Probed by Muon Spin Rotation and Relaxation
Local magnetic fields in a molecule-based optically chiral magnet
[Cr(CN)][Mn()-pnH(HO)](HO) (GN-S) and its enantiomer (GN-R) are
studied by means of muon spin rotation and relaxation (muSR). Detailed analysis
of muon precession signals under zero field observed below T_c supports the
average magnetic structure suggested by neutron powder diffraction. Moreover,
comparison of muSR spectra between GN-S and GN-R suggests that they are a pair
of complete optical isomers in terms of both crystallographic and magnetic
structure. Possibility of magnetic chirality in such a pair is discussed.Comment: 5 pages, 5 figures, submitted to J. Phys. Soc. Jp
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