Glauber dynamics in a single-chain magnet: From theory to real systems

The Glauber dynamics is studied in a single-chain magnet. As predicted, a single relaxation mode of the magnetization is found. Above 2.7 K, the thermally activated relaxation time is mainly governed by the effect of magnetic correlations and the energy barrier experienced by each magnetic unit. This result is in perfect agreement with independent thermodynamical measurements. Below 2.7 K, a crossover towards a relaxation regime is observed that is interpreted as the manifestation of finite-size effects. The temperature dependences of the relaxation time and of the magnetic susceptibility reveal the importance of the boundary conditions.Comment: Submitted to PRL 10 May 2003. Submitted to PRB 12 December 2003; published 15 April 200

Quantum nucleation in a single-chain magnet

The field sweep rate (v=dH/dt) and temperature (T) dependence of the magnetization reversal of a single-chain magnet (SCM) is studied at low temperatures. As expected for a thermally activated process, the nucleation field (H_n) increases with decreasing T and increasing v. The set of H_n(T,v) data is analyzed with a model of thermally activated nucleation of magnetization reversal. Below 1 K, H_n becomes temperature independent but remains strongly sweep rate dependent. In this temperature range, the reversal of the magnetization is induced by a quantum nucleation of a domain wall that then propagates due to the applied field.Comment: 5 pages, 4 figure

Effect of cation size variance on spin and orbital order in Eu1−x_{1-x}(La0.254_{0.254}Y0.746_{0.746})x_{x}VO3_3

We have investigated the $R$-ion ($R$ = rare earth or Y) size variance effect on spin/orbital order in Eu$_{1-x}$(La$_{0.254}$Y$_{0.746}$)$_{x}$VO$_3$. The size variance disturbs one-dimensional orbital correlation in $C$-type spin/$G$-type orbital ordered states and suppresses this spin/orbital order. In contrast, it stabilizes the other spin/orbital order. The results of neutron and resonant X-ray scattering denote that in the other ordered phase, the spin/orbital patterns are $G$-type/$C$-type, respectively.Comment: 4 pages, 4 figures, accepted to Rapid Communication in Physical Review

Comparative study of the effects of electron irradiation and natural disorder in single crystals of SrFe2_{2}(As1−x_{1-x}Px_x)2_2 (x=x=0.35) superconductor

London penetration depth, $\lambda(T)$, was measured in single crystals of SrFe$_2$(As$_{1-x}$P$_x$)$_2$ ($x=$0.35) iron - based superconductor. The influence of disorder on the transition temperature, $T_c$, and on $\lambda(T)$ was investigated. The effects of scattering controlled by the annealing of as-grown crystals was compared with the effects of artificial disorder introduced by 2.5~MeV electron irradiation. The low temperature behavior of $\lambda(T)$ can be described by a power-law function, $\Delta \lambda (T)=AT^n$, with the exponent $n$ close to one in pristine annealed samples, as expected for superconducting gap with line nodes. Upon $1.2 \times 10^{19}$ \ecm irradiation, the exponent $n$ increases rapidly exceeding a dirty limit value of $n=$ 2 implying that the nodes in the superconducting gap are accidental and can be lifted by the disorder. The variation of the exponent $n$ with $T_c$ is much stronger in the irradiated crystals compared to the crystals in which disorder was controlled by the annealing of the growth defects. We discuss the results in terms of different influence of different types of disorder on intra- and inter- band scattering

Universal observation of multiple order parameters in cuprate superconductors

The temperature dependence of the London penetration depth \lambda was measured for an untwined single crystal of YBa_2Cu_3O_{7-\delta} along the three principal crystallographic directions (a, b, and c). Both in-plane components (\lambda_a and \lambda_b) show an inflection point in their temperature dependence which is absent in the component along the c-direction (\lambda_c). The data provide convincing evidence that the in-plane superconducting order parameter is a mixture of s+d-wave symmetry whereas it is exclusively s-wave along the c-direction. In conjunction with previous results it is concluded that coupled s+d-order parameters are universal and intrinsic to cuprate superconductors.Comment: 5 pages, 3 figure