The effect of uniaxial pressure on the magnetic anisotropy of the Mn_{12}-Ac single-molecule magnet

We study the effect of uniaxial pressure on the magnetic hysteresis loops of the single-molecule magnet Mn_{12}-Ac. We find that the application of pressure along the easy axis increases the fields at which quantum tunneling of magnetization occurs. The observations are attributed to an increase in the molecule's magnetic anisotropy constant D of 0.142(1)%/kbar. The increase in D produces a small, but measurable increase in the effective energy barrier for magnetization reversal. Density-functional theory calculations also predict an increase in the barrier with applied pressure.Comment: version accepted by EPL; 6 pages, including 7 figures. Small changes and added reference

Partitioning Complex Networks via Size-constrained Clustering

The most commonly used method to tackle the graph partitioning problem in practice is the multilevel approach. During a coarsening phase, a multilevel graph partitioning algorithm reduces the graph size by iteratively contracting nodes and edges until the graph is small enough to be partitioned by some other algorithm. A partition of the input graph is then constructed by successively transferring the solution to the next finer graph and applying a local search algorithm to improve the current solution. In this paper, we describe a novel approach to partition graphs effectively especially if the networks have a highly irregular structure. More precisely, our algorithm provides graph coarsening by iteratively contracting size-constrained clusterings that are computed using a label propagation algorithm. The same algorithm that provides the size-constrained clusterings can also be used during uncoarsening as a fast and simple local search algorithm. Depending on the algorithm's configuration, we are able to compute partitions of very high quality outperforming all competitors, or partitions that are comparable to the best competitor in terms of quality, hMetis, while being nearly an order of magnitude faster on average. The fastest configuration partitions the largest graph available to us with 3.3 billion edges using a single machine in about ten minutes while cutting less than half of the edges than the fastest competitor, kMetis

Measurement of Magnetization Dynamics in Single-Molecule Magnets Induced by Pulsed Millimeter-Wave Radiation

We describe an experiment aimed at measuring the spin dynamics of the Fe8 single-molecule magnet in the presence of pulsed microwave radiation. In earlier work, heating was observed after a 0.2-ms pulse of intense radiation, indicating that the spin system and the lattice were out of thermal equilibrium at millisecond time scale [Bal et al., Europhys. Lett. 71, 110 (2005)]. In the current work, an inductive pick-up loop is used to probe the photon-induced magnetization dynamics between only two levels of the spin system at much shorter time scales (from ns to us). The relaxation time for the magnetization, induced by a pulse of radiation, is found to be on the order of 10 us.Comment: 3 RevTeX pages, including 3 eps figures. The paper will appear in the Journal of Applied Physics as MMM'05 conference proceeding

Radiation- and Phonon-Bottleneck-Induced Tunneling in the Fe8 Single-Molecule Magnet

We measure magnetization changes in a single crystal of the single-molecule magnet Fe8 when exposed to intense, short (<20 $\mu$s) pulses of microwave radiation resonant with the m = 10 to 9 transition. We find that radiation induces a phonon bottleneck in the system with a time scale of ~5 $\mu$s. The phonon bottleneck, in turn, drives the spin dynamics, allowing observation of thermally assisted resonant tunneling between spin states at the 100-ns time scale. Detailed numerical simulations quantitatively reproduce the data and yield a spin-phonon relaxation time of T1 ~ 40 ns.Comment: 6 RevTeX pages, including 4 EPS figures, version accepted for publicatio

Experimental Upper Bound on Superradiance Emission from Mn12 Acetate

We used a Josephson junction as a radiation detector to look for evidence of the emission of electromagnetic radiation during magnetization avalanches in a crystal assembly of Mn_12-Acetate. The crystal assembly exhibits avalanches at several magnetic fields in the temperature range from 1.8 to 2.6 K with durations of the order of 1 ms. Although a recent study shows evidence of electromagnetic radiation bursts during these avalanches [J. Tejada, et al., Appl. Phys. Lett. {\bf 84}, 2373 (2004)], we were unable to detect any significant radiation at well-defined frequencies. A control experiment with external radiation pulses allows us to determine that the energy released as radiation during an avalanche is less than 1 part in 10^4 of the total energy released. In addition, our avalanche data indicates that the magnetization reversal process does not occur uniformly throughout the sample.Comment: 4 RevTeX pages, 3 eps figure

All-Optical Switching Demonstration using Two-Photon Absorption and the Classical Zeno Effect

Low-contrast all-optical Zeno switching has been demonstrated in a silicon nitride microdisk resonator coupled to a hot atomic vapor. The device is based on the suppression of the field build-up within a microcavity due to non-degenerate two-photon absorption. This experiment used one beam in a resonator and one in free-space due to limitations related to device physics. These results suggest that a similar scheme with both beams resonant in the cavity would correspond to input power levels near 20 nW.Comment: 4 pages, 5 figure