964 research outputs found
Signature of Carrier-Induced Ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta}: Exchange Interaction Between High-Spin Co 2+ and the Ti 3d Conduction Band
X-ray photoemission spectroscopy measurements were performed on thin-film
samples of rutile Ti_{1-x}Co_{x}O_{2-delta} to reveal the electronic structure.
The Co 2p core level spectra indicate that the Co ions take the high-spin Co 2+
configuration, consistent with substitution on the Ti site. The high spin state
and the shift due to the exchange splitting of the conduction band suggest
strong hybridization between carriers in the Ti 3d t2g band and the t2g states
of the high-spin Co 2+. These observations support the argument that room
temperature ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta} is intrinsic.Comment: 4 pages, 5 figures. Accepted for publication in Physical Review
Letter
Anomalous Flux Flow Resistivity in Two Gap Superconductor MgB_2
The flux flow resistivity associated with purely viscous motion of vortices
in high-quality MgB_2 was measured by microwave surface impedance. Flux flow
resistivity exhibits unusual field dependence with strong enhancement at low
field, which is markedly different to conventional s-wave superconductors. A
crossover field which separates two distinct flux flow regimes having different
flux flow resistivity slopes was clearly observed in H//ab-plane. The unusual
H-dependence indicates that two very differently sized superconducting gaps in
MgB_2 manifest in the vortex dynamics and almost equally contribute to energy
dissipation. The carrier scattering rate in two different bands is also
discussed with the present results, compared to heat capacity and thermal
conductivity results.Comment: 4 pages, 3figure
Relation between the superconducting gap energy and the two-magnon Raman peak energy in Bi2Sr2Ca{1-x}YxCu2O{8+\delta}
The relation between the electronic excitation and the magnetic excitation
for the superconductivity in Bi2Sr2Ca{1-x}YxCu2O{8+\delta} was investigated by
wide-energy Raman spectroscopy. In the underdoping region the B1g scattering
intensity is depleted below the two-magnon peak energy due to the "hot spots"
effects. The depleted region decreases according to the decrease of the
two-magnon peak energy, as the carrier concentration ncreases. This two-magnon
peak energy also determines the B1g superconducting gap energy as
from under to overdoping hole concentration.Comment: 10 pages, 4 figure
Temperature-dependent Raman spectroscopy in BaRuO systems
We investigated the temperature-dependence of the Raman spectra of a
nine-layer BaRuO single crystal and a four-layer BaRuO epitaxial film,
which show pseudogap formations in their metallic states. From the polarized
and depolarized spectra, the observed phonon modes are assigned properly
according to the predictions of group theory analysis. In both compounds, with
decreasing temperature, while modes show a strong hardening, (or
) modes experience a softening or no significant shift. Their different
temperature-dependent behaviors could be related to a direct Ru metal-bonding
through the face-sharing of RuO. It is also observed that another
mode of the oxygen participating in the face-sharing becomes split at low
temperatures in the four layer BaRuO. And, the temperature-dependence of
the Raman continua between 250 600 cm is strongly correlated to
the square of the plasma frequency. Our observations imply that there should be
a structural instability in the face-shared structure, which could be closely
related to the pseudogap formation of BaRuO systems.Comment: 8 pages, 6 figures. to be published in Phys. Rev.
Mixed state properties of superconducting MgB2 single crystals
We report on measurements of the magnetic moment in superconducting MgB2
single crystals. We find \mu_0H_{c2}^c(0) = 3.2 T, \mu_0H_{c2}^{ab}(0) = 14.5
T, \gamma = 4.6, \mu_0H_c(0) = 0.28 T, and \kappa(T_c) = 4.7. The standard
Ginzburg-Landau and London model relations lead to a consistent data set and
indicate that MgB2 is a clean limit superconductor of intermediate coupling
strength with very pronounced anisotropy effects
Doping Dependence of the Pseudogap in La(2-x)Sr(x)CuO(4)
We report the results of Raman scattering experiments on single crystals of
La(2-x)Sr(x)CuO(4) that span the range from underdoped (x = 0.10) to overdoped
(x =0.22). The spectra are consistent with the existence of a strong
anisotropic quasiparticle interaction that results in a normal state depletion
of spectral weight from regions of the Fermi surface located near the zone
axes. The strength of the interaction decreases rapidly with increasing hole
concentration and the spectral evidence for the pseudogap vanishes when the
optimum doping level is reached. The results suggest that the pseudogap and
superconducting gap arise from different mechanisms.Comment: 7 pages, 6 eps figures, added new sections, figures, reference
Disorder induced collapse of the electron phonon coupling in MgB observed by Raman Spectroscopy
The Raman spectrum of the superconductor MgB has been measured as a
function of the Tc of the film. A striking correlation is observed between the
onset and the frequency of the mode. Analysis of the data with
the McMillan formula provides clear experimental evidence for the collapse of
the electron phonon coupling at the temperature predicted for the convergence
of two superconducting gaps into one observable gap. This gives indirect
evidence of the convergence of the two gaps and direct evidence of a transition
to an isotropic state at 19 K. The value of the electron phonon coupling
constant is found to be 1.22 for films with T 39K and 0.80 for films with
T19K.Comment: 5 pages, 4 figure
Evidence for High-frequency Phonon Mediated S-wave Superconductivity : 11B-NMR Study of Al-doped MgB2
We report B-NMR study on Al-doped MgB that addresses a possible
mechanism for a high superconducting (SC) transition temperature () of
K in recently discovered MgB. The result of nuclear spin lattice
relaxation rate in the SC state revealed that the size in the SC gap is
not changed by substituting Al for Mg. The reduction on by Al-doping is
shown to be due to the decrease of . According to the McMillan
equation, the experimental relation between and the relative change in
allowed us to estimate a characteristic phonon frequency K and an electron-phonon coupling constant . These
results suggest that the high- superconductivity in MgB is mediated by
the strong electron-phonon coupling with high-frequency phonons.Comment: 6pages, 3figure
Extreme Electron-Phonon Coupling in Boron-based Layered Superconductors
The phonon-mode decomposition of the electron-phonon coupling in the
MgB2-like system Li_{1-x}BC is explored using first principles calculations. It
is found that the high temperature superconductivity of such systems results
from extremely strong coupling to only ~2% of the phonon modes. Novel
characteristics of E_2g branches include (1) ``mode lambda'' values of 25 and
greater compared to a mean of for other modes, (2) a precipitous
Kohn anomaly, and (3) E_2g phonon linewidths within a factor of ~2 of the
frequency itself, indicating impending breakdown of linear electron-phonon
theory. This behavior in borne out by recent inelastic x-ray scattering studies
of MgB2 by Shukla et al.Comment: 4 two-column pages, 4 figures. Equations simplified. Figure 4
changed. Comparison with new data include
Hole concentration and phonon renormalization in Ca-doped YBa_2Cu_3O_y (6.76 < y < 7.00)
In order to access the overdoped regime of the YBa_2Cu_3O_y phase diagram, 2%
Ca is substituted for Y in YBa_2Cu_3O_y (y = 7.00,6.93,6.88,6.76). Raman
scattering studies have been carried out on these four single crystals.
Measurements of the superconductivity-induced renormalization in frequency
(Delta \omega) and linewidth (\Delta 2\gamma) of the 340 cm^{-1} B_{1g} phonon
demonstrate that the magnitude of the renormalization is directly related to
the hole concentration (p), and not simply the oxygen content. The changes in
\Delta \omega with p imply that the superconducting gap (\Delta_{max})
decreases monotonically with increasing hole concentration in the overdoped
regime, and \Delta \omega falls to zero in the underdoped regime. The linewidth
renormalization \Delta 2\gamma is negative in the underdoped regime, crossing
over at optimal doping to a positive value in the overdoped state.Comment: 18 pages; 5 figures; submitted to Phys. Rev. B Oct. 24, 2002 (BX8292
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