A Dynamic 'Double Slit' Experiment in a Single Atom

A single-atom 'double-slit' experiment is realized by photo-ionizing Rubidium atoms using two independent low power lasers. The photoelectron wave of well-defined energy recedes to the continuum either from the 5P or 6P states in the same atom, resulting in two-path interference imaged in the far field using a photoelectron detector. Even though the lasers are independent and not phase locked, the transitions within the atom impart the phase relationship necessary for interference. The experiment is designed so that either 5P or 6P states are excited by one laser, before ionization by the second beam. The measurement cannot determine which excitation path is taken, resulting in interference in wave-vector space analogous to Young's double-slit studies. As the lasers are tunable in both frequency and intensity, the individual excitation-ionization pathways can be varied, allowing dynamic control of the interference term. Since the electron wave recedes in the Coulomb potential of the residual ion, a quantum model is used to capture the dynamics. Excellent agreement is found between theory and experiment.Comment: 8 pages, 4 figures, accepted in Phys. Rev. Let

Natural & unnatural-parity contributions in electron-impact ionization of laser-aligned atoms

Differential cross section measurements from laser-aligned Mg atoms are compared to theoretical calculations using both time dependent and time-independent formalisms. It is found that both natural and unnatural parity contributions to the calculated cross sections are required to emulate the data when the state is aligned out of the scattering plane

Comparison of experiment and theory for superelastic electron-collision studies from laser-aligned magnesium

A combined experimental and theoretical study of superelastic electron collisions from laser-aligned magnesium atoms for a range of collision energies from 35 to 55 eV is presented. 24Mg atoms were excited from the 3 1S0 ground state to the 3 1P1 excited state using continuous-wave linearly polarized laser radiation at ∼285 nm. Electrons of well-defined energy Einc then deexcited the targets, and the superelastically scattered electrons emerging from the collision were detected as a function of scattering angle and laser polarization. Results for alignment of the target by the electron beam are presented for a range of scattering angles, for outgoing energies from Eout=35 to 55 eV. The agreement between the measurements and the results of the convergent close-coupling theory are encouraging, but some discrepancies remain