610 research outputs found
Double exchange magnets: Spin-dynamics in the paramagnetic phase
The electronic structure of perovskite manganese oxides is investigated in
terms of a Kondo lattice model with ferromagnetic Hund coupling and
antiferromagnetic exchange between -spins using a finite temperature
diagonalization technique. Results for the dynamic structure factor are
consistent with recent neutron scattering experiments for the bilayer manganite
LaSrMnO . The susceptibility shows Curie-Weiss
behaviour and is used to derive a phase diagram. In the paramagnetic phase
carriers are characterized as ferromagnetic polarons in an antiferromagnetic
spin liquid.Comment: Revtex, 4 pages with 5 postscript figures include
Spin excitations used to probe the nature of the exchange coupling in the magnetically ordered ground state of PrCaMnO
We have used time-of-flight inelastic neutron scattering to measure the spin
wave spectrum of the canonical half-doped manganite
PrCaMnO, in its magnetic and orbitally ordered phase. The
data, which cover multiple Brillouin zones and the entire energy range of the
excitations, are compared with several different models that are all consistent
with the CE-type magnetic order, but arise through different exchange coupling
schemes. The Goodenough model, i.e. an ordered state comprising strong nearest
neighbor ferromagnetic interactions along zig-zag chains with antiferromagnetic
inter-chain coupling, provides the best description of the data, provided that
further neighbor interactions along the chains are included. We are able to
rule out a coupling scheme involving formation of strongly bound ferromagnetic
dimers, i.e. Zener polarons, on the basis of gross features of the observed
spin wave spectrum. A model with weaker dimerization reproduces the observed
dispersion but can be ruled out on the basis of discrepancies between the
calculated and observed structure factors at certain positions in reciprocal
space. Adding further neighbor interactions results in almost no dimerization,
i.e. recovery of the Goodenough model. These results are consistent with
theoretical analysis of the degenerate double exchange model for half-doping,
and provide a recipe for how to interpret future measurements away from
half-doping, where degenerate double exchange models predict more complex
ground states.Comment: 14 pages, 11 figure
A Comparison of the High-Frequency Magnetic Fluctuations in Insulating and Superconducting La2-xSrxCuO4
Inelastic neutron scattering performed at a spallation source is used to make
absolute measurements of the dynamic susceptibility of insulating La2CuO4 and
superconducting La2-xSrxCuO4 over the energy range 15<EN<350 meV. The effect of
Sr doping on the magnetic excitations is to cause a large broadening in
wavevector and a substantial change in the spectrum of the local spin
fluctuations. Comparison of the two compositions reveals a new energy scale of
22 meV in La1.86Sr0.14CuO4.Comment: RevTex, 7 Pages, 4 postscript figure
HORACE: software for the analysis of data from single crystal spectroscopy experiments at time-of-flight neutron instruments
The HORACE suite of programs has been developed to work with large
multiple-measurement data sets collected from time-of-flight neutron
spectrometers equipped with arrays of position-sensitive detectors. The
software allows exploratory studies of the four dimensions of reciprocal space
and excitation energy to be undertaken, enabling multi-dimensional subsets to
be visualized, algebraically manipulated, and models for the scattering to
simulated or fitted to the data. The software is designed to be an extensible
framework, thus allowing user-customized operations to be performed on the
data. Examples of the use of its features are given for measurements exploring
the spin waves of the simple antiferromagnet RbMnF and ferromagnetic
iron, and the phonons in URuSi.Comment: 14 pages, 6 figure
Absence of strong magnetic fluctuations in the iron phosphide superconductors LaFePO and Sr2ScO3FeP
We report neutron inelastic scattering measurements on polycrystalline LaFePO
and Sr2ScO3FeP, two members of the iron phosphide families of superconductors.
No evidence is found for any magnetic fluctuations in the spectrum of either
material in the energy and wavevector ranges probed. Special attention is paid
to the wavevector at which spin-density-wave-like fluctuations are seen in
other iron-based superconductors. We estimate that the magnetic signal, if
present, is at least a factor of four (Sr2ScO3FeP) or seven (LaFePO) smaller
than in the related iron arsenide and chalcogenide superconductors. These
results suggest that magnetic fluctuations are not as influential on the
electronic properties of the iron phosphide systems as they are in other
iron-based superconductors.Comment: 7 pages, 5 figure
Spin wave spectrum of the quantum ferromagnet on the pyrochlore lattice Lu2V2O7
Neutron inelastic scattering has been used to probe the spin dynamics of the
quantum (S=1/2) ferromagnet on the pyrochlore lattice Lu2V2O7. Well-defined
spin waves are observed at all energies and wavevectors, allowing us to
determine the parameters of the Hamiltonian of the system. The data are found
to be in excellent overall agreement with a minimal model that includes a
nearest- neighbour Heisenberg exchange J = 8:22(2) meV and a
Dzyaloshinskii-Moriya interaction (DMI) D =1:5(1) meV. The large DMI term
revealed by our study is broadly consistent with the model developed by Onose
et al. to explain the magnon Hall effect they observed in Lu2V2O7 [1], although
our ratio of D=J = 0:18(1) is roughly half of their value and three times
larger than calculated by ab initio methods [2].Comment: 5 pages, 4 figure
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