51 research outputs found

    Long-range transfer of electron-phonon coupling in oxide superlattices

    Full text link
    The electron-phonon interaction is of central importance for the electrical and thermal properties of solids, and its influence on superconductivity, colossal magnetoresistance, and other many-body phenomena in correlated-electron materials is currently the subject of intense research. However, the non-local nature of the interactions between valence electrons and lattice ions, often compounded by a plethora of vibrational modes, present formidable challenges for attempts to experimentally control and theoretically describe the physical properties of complex materials. Here we report a Raman scattering study of the lattice dynamics in superlattices of the high-temperature superconductor YBa2Cu3O7\bf YBa_2 Cu_3 O_7 and the colossal-magnetoresistance compound La2/3Ca1/3MnO3\bf La_{2/3}Ca_{1/3}MnO_{3} that suggests a new approach to this problem. We find that a rotational mode of the MnO6_6 octahedra in La2/3Ca1/3MnO3\bf La_{2/3}Ca_{1/3}MnO_{3} experiences pronounced superconductivity-induced lineshape anomalies, which scale linearly with the thickness of the YBa2Cu3O7\bf YBa_2 Cu_3 O_7 layers over a remarkably long range of several tens of nanometers. The transfer of the electron-phonon coupling between superlattice layers can be understood as a consequence of long-range Coulomb forces in conjunction with an orbital reconstruction at the interface. The superlattice geometry thus provides new opportunities for controlled modification of the electron-phonon interaction in complex materials.Comment: 13 pages, 4 figures. Revised version to be published in Nature Material

    Relevance of tumor-infiltrating lymphocytes in breast cancer

    Full text link

    Orbital selective switching of ferromagnetism in an oxide quasi two-dimensional electron gas

    No full text
    Multi-orbital physics in quasi-two-dimensional electron gases (q2DEGs) triggers intriguing phenomena not observed in bulk materials, such as unconventional superconductivity and magnetism. Here, we investigate the mechanism of orbital selective switching of the spin-polarization in the oxide q2DEG formed at the (001) interface between the LaAlO3, EuTiO3 and SrTiO3 band insulators. By using density functional theory calculations, transport, magnetic and x-ray spectroscopy measurements, we find that the filling of titanium-bands with 3dxz/3dyz orbital character in the EuTiO3 layer and at the interface with SrTiO3 induces an antiferromagnetic to ferromagnetic switching of the exchange interaction between Eu-4f7 magnetic moments. The results explain the observation of the carrier density-dependent ferromagnetic correlations and anomalous Hall effect in this q2DEG, and demonstrate how combined theoretical and experimental approaches can lead to a deeper understanding of emerging electronic phases and serve as a guide for the materials design of advanced electronic applications

    Orbital selective switching of ferromagnetism in an oxide quasi two-dimensional electron gas

    Get PDF
    International audienceMulti-orbital physics in quasi-two-dimensional electron gases (q2DEGs) triggers unique phenomena not observed in bulk materials, such as unconventional superconductivity and magnetism. Here, we investigate the mechanism of orbital selective switching of the spin-polarization in the oxide q2DEG formed at the (001) interface between the LaAlO3_{3}, EuTiO3_{3} and SrTiO3_{3} band insulators. By using density functional theory calculations, transport, magnetic and x-ray spectroscopy measurements, we find that the filling of titanium-bands with 3dxz,yz_{xz,yz} orbital character in the EuTiO3 layer and at the interface with SrTiO3_{3} induces an antiferromagnetic to ferromagnetic switching of the exchange interaction between Eu-4f7^{7} magnetic moments. The results explain the observation of the carrier density dependent ferromagnetic correlations and anomalous Hall effect in this q2DEG, and demonstrate how combined theoretical and experimental approaches can lead to a deeper understanding of novel electronic phases and serve as a guide for the materials design for advanced electronic applications

    Orbital selective switching of ferromagnetism in an oxide quasi two-dimensional electron gas

    No full text
    International audienceMulti-orbital physics in quasi-two-dimensional electron gases (q2DEGs) triggers unique phenomena not observed in bulk materials, such as unconventional superconductivity and magnetism. Here, we investigate the mechanism of orbital selective switching of the spin-polarization in the oxide q2DEG formed at the (001) interface between the LaAlO3_{3}, EuTiO3_{3} and SrTiO3_{3} band insulators. By using density functional theory calculations, transport, magnetic and x-ray spectroscopy measurements, we find that the filling of titanium-bands with 3dxz,yz_{xz,yz} orbital character in the EuTiO3 layer and at the interface with SrTiO3_{3} induces an antiferromagnetic to ferromagnetic switching of the exchange interaction between Eu-4f7^{7} magnetic moments. The results explain the observation of the carrier density dependent ferromagnetic correlations and anomalous Hall effect in this q2DEG, and demonstrate how combined theoretical and experimental approaches can lead to a deeper understanding of novel electronic phases and serve as a guide for the materials design for advanced electronic applications

    Au and Cu Atoms on NaCl(001): a single-atom based memory device prototype?

    No full text
    We present a first-principle study of gold and copper atoms adsorbed in NaCl(001) surfaces. Motivated by a recent STM experiment on this subject, the electronic and magnetic properties of Au and Cu atoms are investigated, as well as the modifications in these properties under charge injection. Similarities of these systems and the corresponding isolated atom are exploited. A discussion about the possibility of applying the studied systems on high-density memory devices is addressed. Copyright EDP Sciences, SIF, Springer-Verlag Berlin Heidelberg 2010
    • …
    corecore