40 research outputs found
Simultaneous PIXE and RBS data analysis using Bayesian Inference with the DataFurnace code
The Rutherford Backscattering Spectroscopy (RBS) and Particle Induced X-ray
Emission (PIXE) techniques can be used to obtain complementary information
about the characteristics of a sample but, traditionally, a gap has separated
the available computer codes for analyzing data from each technique, being hard
to simultaneously analyze data from the same sample. The recent development of
a free and open source library, LibCPIXE, for PIXE simulation and analysis of
arbitrary multilayered samples, has permitted to integrate this technique into
the DataFurnace code which already handles many other IBA techniques such as
Rutherford and non-Rutherford backscattering, elastic recoil detection, and
non-resonant nuclear reaction analysis. The fitting capabilities of DataFurnace
can therefore now be applied to PIXE spectra as well, including the Bayesian
Inference analysis and the simultaneous and coherent fitting of multiple
spectra from different techniques. Various examples are presented in which the
simultaneous RBS and PIXE analysis allows us to obtain consistent results that
cannot be obtained by independent analysis of the data from each technique.Comment: 10 pages, 5 figures. Paper initially presented to IBA2005. Please
cite the published version (DOI:10.1016/j.nimb.2006.03.190
LibCPIXE: a PIXE simulation open-source library for multilayered samples
Most particle induced X-ray emission (PIXE) data analysis codes are not
focused on handling multilayered samples. We have developed an open-source
library called "LibCPIXE", for PIXE data analysis. It is written in standard C
and implements functions for simulating X-ray yields of PIXE spectra taken from
arbitrary samples, including multilayered targets. The library is designed to
be fast, portable, modular and scalable, as well as to facilitate its
incorporation into any existing program. In order to demonstrate the
capabilities of the library, a program called CPIXE was developed and used to
analyze various real samples involving both bulk and layered samples. Just as
the library, the CPIXE source code is freely available under the General Public
License. We demonstrate that it runs both under GNU/Linux systems as well as
under MS Windows. There is in principle no limitation to port it to other
platforms
On the traceably accurate voltage calibration of electrostatic accelerators
We describe in detail a calibration method for the terminal voltage of small accelerators used for ion beam analysis, with the elastic resonance of 16O(α,α)16O at 3038 keV as the intrinsic measurement standard. The beam energy relative to this resonance is determined with a precision around 300 eV and an evaluated reproducibility of 1.0 keV. We show that this method is both robust and convenient, and demonstrate consistency with calibration relative to three other independent methods: using radioactive sources and using the resonant 27Al(p,γ)28Si and non-resonant 16O(p,γ)17F direct capture reactions. We re-evaluate the literature and show that the peak in the cross-section function is at 3038.1 ± 2.3 keV. By comparing the results obtained with 16O(α,α)16O to the other calibration methods we show that this uncertainty can be reduced to 1.3 keV.</p
Structure of N22 and the N=14 subshell
One-neutron knockout data for N18-22 are analyzed in the eikonal approximation of the Glauber model. The role of the s-d shell and the crossing of the N=14 neutron subshell are discussed. Of particular interest is the nucleus N22, where the knockout data provide a sensitive experimental test for a possible halo structure of its ground state. The observation of a narrow momentum distribution of the N21 fragments, together with an essential 1s 1/2 contribution needed to describe the observed longitudinal- momentum distribution, allow the firm conclusion that the ground state of N22 is a well-developed nuclear halo. The results also show that the N=14 subshell in N22 is somewhat reduced as compared to that of O23. © 2011 American Physical Society.This work was supported by: GSI, via Hochschulzusammenarbeitsvereinbarungen under Contracts No. DA RICK, No. OF ELZ, and No. MZ KRAK; German BMBF; the DFG Cluster of Excellence, Origin and Structure of the Universe; FBR under Contract No. 08-02-012244; EC under Contract No. ERBCHGE-CT92-003; Ministerio de Ciencia e Innovacion under Project No. FPA2009-14604-602-01; ´ Ministerio de Educacion under Grant No. FPU-AP2005-3308, ´ and the Galician Conseller´ıa de Educacion e Ordenaci ´ on´ Universitaria, Consolidacion e Estructuraci ´ on de Unidades ´ Competitivas 2010/57.Peer Reviewe
Positron annihilation lifetime spectroscopy (PALS) as a characterization technique for nanostructured self-assembled amphiphile systems
Positron annihilation lifetime spectroscopy (PALS) has potential as a novel rapid characterization method for self-assembly amphiphile systems; however, a lack of systematic correlation of PALS parameters with structural attributes has limited its more widespread application. In this study, using the well-characterized phytantriol/ water and the phytantriol/vitamin E acetate/water self-assembly amphiphile systems, the impact of systematic structural changes controlled by changes in composition and temperature on PALS parameters has been studied. The PALS parameters (orthopositronium (oPs) lifetime and intensity signatures) were shown to be sensitive to the molecular packing and mobility of the self-assembled lipid molecules in various lyotropic liquid crystalline phases, enabling differentiation between liquid crystalline structures. The oPs lifetime, related to the molecular packing and mobility, is correlated with rheological properties of the individual mesophases. The oPs lifetime links the lipid chain packing and mobility in the various mesophases to resultant macroscopic properties, such as permeability, which is critical for the use of these mesophase structures as diffusioncontrolled release matrices for active liposoluble compounds
External Beam Total-IBA using DataFurnace
The self-consistent Ion Beam Analysis (IBA) of cultural heritage samples using the external beam is technically demanding. We report on the calibration of an analysis of glass samples from the Rosslyn Chapel where the interest will ultimately be in the full characterisation of the weathered glass. Such an analysis requires a comprehensive Total-IBA approach using p-PIGE and He-PIXE to obtain ”bulk” and surface Na, with H-PIXE/EBS for multielemental depth profiling to 10 μm and He-PIXE/EBS for higher depth resolution near the surface; also with two PIXE detectors as usual for the high and low energy parts of the spectrum. A revised NDF v.10 code capable of a self-consistent handling of all these signals at state-of-the-art accuracy is described, together with the calibration protocols required for such an analysis. Other capabilities of the NDF code not previously discussed are also reviewed