42,124 research outputs found
High-pressure study of the basal-plane anisotropy of the upper critical field of the topological superconductor SrxBi2Se3
We report a high-pressure transport study of the upper-critical field,
, of the topological superconductor SrBiSe ( K). was measured for magnetic fields directed along two
orthogonal directions, and , in the trigonal basal plane. While
superconductivity is rapidly suppressed at the critical pressure
GPa, the pronounced two-fold basal-plane anisotropy at K, recently reported at ambient pressure (Pan et al., 2016), is
reinforced and attains a value of at the highest pressure (2.2 GPa).
The data reveal that the unconventional superconducting state with broken
rotational symmetry is robust under pressure
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Highly Stable Luminous "snakes" from CsPbX3 Perovskite Nanocrystals Anchored on Amine-Coated Silica Nanowires
CsPbX3 (X = Cl, Br, and I) perovskite nanocrystals (NCs) are known for their exceptional optoelectronic properties, yet the material's instability toward polar solvents, heat, or UV irradiation greatly limits its further applications. Herein, an efficient in situ growing strategy has been developed to give highly stable perovskite NC composites (abbreviated CsPbX3@CA-SiO2) by anchoring CsPbX3 NCs onto silica nanowires (NWs), which effectively depresses the optical degradation of their photoluminescence (PL) and enhances stability. The preparation of surface-functionalized serpentine silica NWs is realized by a sol-gel process involving hydrolysis of a mixture of tetraethyl orthosilicate (TEOS), 3-aminopropyltriethoxysilane (APTES), and trimethoxy(octadecyl)silane (TMODS) in a water/oil emulsion. The serpentine NWs are formed via an anisotropic growth with lengths up to 8 μm. The free amino groups are employed as surface ligands for growing perovskite NCs, yielding distributed monodisperse NCs (∼8 nm) around the NW matrix. The emission wavelength is tunable by simple variation of the halide compositions (CsPbX3, X = Cl, Br, or I), and the composites demonstrate a high photoluminescence quantum yield (PLQY 32-69%). Additionally, we have demonstrated the composites CsPbX3@CA-SiO2 can be self-woven to form a porous 3D hierarchical NWs membrane, giving rise to a superhydrophobic surface with hierarchical micro/nano structural features. The resulting composites exhibit high stability toward water, heat, and UV irradiation. This work elucidates an effective strategy to incorporate perovskite nanocrystals onto functional matrices as multifunctional stable light sources
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On the exceptional damage-tolerance of gradient metallic materials
An experimental study is described on the fracture toughness and micro-mechanisms associated with the initiation and propagation of cracks in metallic nickel containing marked gradients in grain size, ranging from ∼30 nm to ∼4 μm. Specifically, cracks are grown in a gradient structured (GS) nickel with grain-size gradient ranging from the coarse macro-scale to nano-scale (CG → NG) and vice versa (NG → CG), with the measured crack-resistance R-curves compared to the corresponding behavior in uniform nano-grained (NG) and coarse-grained (CG) materials. It is found that the gradient structures display a much-improved combination of high strength and toughness compared to uniform grain-sized materials. However, based on J-integral measurements in the gradient materials, the crack-initiation toughness is far higher for cracks grown in the direction of the coarse-to-nano grained gradient than vice versa, a result which we ascribe primarily to excessive crack-tip blunting in the coarse-grained microstructure. Both gradient structures, however, display marked rising R-curve behavior with exceptional crack-growth toughnesses exceeding 200 MPa.m½
Microscopic origin of local moments in a zinc-doped high- superconductor
The formation of a local moment around a zinc impurity in the high-
cuprate superconductors is studied within the framework of the bosonic
resonating-valence-bond (RVB) description of the model. A topological
origin of the local moment has been shown based on the phase string effect in
the bosonic RVB theory. It is found that such an moment distributes
near the zinc in a form of staggered magnetic moments at the copper sites. The
corresponding magnetic properties, including NMR spin relaxation rate, uniform
spin susceptibility, and dynamic spin susceptibility, etc., calculated based on
the theory, are consistent with the experimental measurements. Our work
suggests that the zinc substitution in the cuprates provide an important
experimental evidence for the RVB nature of local physics in the original (zinc
free) state.Comment: The topological reason of local moment formation is given. One figure
is adde
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