362 research outputs found
Activity-controlled annealing of colloidal monolayers.
Molecular motors are essential to the living, generating fluctuations that boost transport and assist assembly. Active colloids, that consume energy to move, hold similar potential for man-made materials controlled by forces generated from within. Yet, their use as a powerhouse in materials science lacks. Here we show a massive acceleration of the annealing of a monolayer of passive beads by moderate addition of self-propelled microparticles. We rationalize our observations with a model of collisions that drive active fluctuations and activate the annealing. The experiment is quantitatively compared with Brownian dynamic simulations that further unveil a dynamical transition in the mechanism of annealing. Active dopants travel uniformly in the system or co-localize at the grain boundaries as a result of the persistence of their motion. Our findings uncover the potential of internal activity to control materials and lay the groundwork for the rise of materials science beyond equilibrium
Colloidal motility and pattern formation under rectified diffusiophoresis
In this letter, we characterize experimentally the diffusiophoretic motion of
colloids and lambda- DNA toward higher concentration of solutes, using
microfluidic technology to build spatially- and temporally-controlled
concentration gradients. We then demonstrate that segregation and spatial
patterning of the particles can be achieved from temporal variations of the
solute concentration profile. This segregation takes the form of a strong
trapping potential, stemming from an osmotically induced rectification
mechanism of the solute time-dependent variations. Depending on the spatial and
temporal symmetry of the solute signal, localization patterns with various
shapes can be achieved. These results highlight the role of solute contrasts in
out-of-equilibrium processes occuring in soft matter
Sedimentation of active colloidal suspensions
In this paper, we investigate experimentally the non-equilibrium steady state
of an active colloidal suspension under gravity field. The active particles are
made of chemically powered colloids, showing self propulsion in the presence of
an added fuel, here hydrogen peroxide. The active suspension is studied in a
dedicated microfluidic device, made of permeable gel microstructures. Both the
microdynamics of individual colloids and the global stationary state of the
suspension under gravity - density profiles, number fluctuations - are measured
with optical microscopy. This allows to connect the sedimentation length to the
individual self-propelled dynamics, suggesting that in the present dilute
regime the active colloids behave as 'hot' particles. Our work is a first step
in the experimental exploration of the out-of-equilibrium properties of
artificial active systems.Comment: 4 pages, 4 figure
Dynamic clustering in active colloidal suspensions with chemical signaling
In this paper, we explore experimentally the phase behavior of a dense active
suspension of self- propelled colloids. In addition to a solid-like and a
gas-like phase observed for high and low densities, a novel cluster phase is
reported at intermediate densities. This takes the form of a stationary
assembly of dense aggregates, with an average size which grows with activity as
a linear function of the self-propelling velocity. While different possible
scenarii can be considered to account for these observations - such as a
generic velocity weakening instability recently put forward -, we show that the
experimental results are reproduced by a chemotactic aggregation mechanism,
originally introduced to account for bacterial aggregation, and accounting here
for diffusiophoretic chemical interaction between colloidal swimmers.Comment: supplementary video :http://
www-lpmcn.univ-lyon1.fr/~lbocquet/Movie-Theurkauff-SI.av
Artificial Rheotaxis
Motility is a basic feature of living microorganisms, and how it works is
often determined by environmental cues. Recent efforts have focused on develop-
ing artificial systems that can mimic microorganisms, and in particular their
self-propulsion. Here, we report on the design and characterization of syn-
thetic self-propelled particles that migrate upstream, known as positive rheo-
taxis. This phenomenon results from a purely physical mechanism involving the
interplay between the polarity of the particles and their alignment by a
viscous torque. We show quantitative agreement between experimental data and a
simple model of an overdamped Brownian pendulum. The model no- tably predicts
the existence of a stagnation point in a diverging flow. We take advantage of
this property to demonstrate that our active particles can sense and
predictably organize in an imposed flow. Our colloidal system represents an
important step towards the realization of biomimetic micro-systems withthe
ability to sense and respond to environmental changesComment: Published in Science Advances [Open access journal of Science
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