Combined effect of coherent Z exchange and the hyperfine interaction in atomic PNC

The nuclear spin-dependent parity nonconserving (PNC) interaction arising from a combination of the hyperfine interaction and the coherent, spin-independent, PNC interaction from Z exchange is evaluated using many-body perturbation theory. For the 6s-7s transition in 133Cs, we obtain a result that is about 40% smaller than that found previously by Bouchiat and Piketty [Phys. Lett. B 269, 195 (1991)]. Applying this result to 133Cs, leads to an increase in the experimental value of nuclear anapole moment and exacerbates differences between constraints on PNC meson coupling constants obtained from the Cs anapole moment and those obtained from other nuclear parity violating experiments. Nuclear spin-dependent PNC dipole matrix elements, including contributions from the combined weak-hyperfine interaction, are also given for the 7s-8s transition in 211Fr and for transitions between ground-state hyperfine levels in K, Rb, Cs, Ba+, Au, Tl, Fr, and Ra+.Comment: Revtex4 preprint 19 pages 4 table

The anapole moment and nucleon weak interactions

From the recent measurement of parity nonconservation (PNC) in the Cs atom we have extracted the constant of the nuclear spin dependent electron-nucleon PNC interaction, $\kappa = 0.442 (63)$; the anapole moment constant, $\kappa_a = 0.364 (62)$; the strength of the PNC proton-nucleus potential, $g_p = 7.3 \pm 1.2 (exp.) \pm 1.5 (theor.)$; the $\pi$-meson-nucleon interaction constant, $f_\pi \equiv h_\pi^{1} = [9.5 \pm 2.1 (exp.) \pm 3.5 (theor.)] \times 10^{-7}$; and the strength of the neutron-nucleus potential, $g_n = -1.7 \pm 0.8 (exp.) \pm 1.3 (theor.)$.Comment: Uses RevTex, 12 pages. We have added an explanation of the effect of finite nuclear siz

Quantum dots coordinated with conjugated organic ligands: new nanomaterials with novel photophysics

CdSe quantum dots functionalized with oligo-(phenylene vinylene) (OPV) ligands (CdSe-OPV nanostructures) represent a new class of composite nanomaterials with significantly modified photophysics relative to bulk blends or isolated components. Single-molecule spectroscopy on these species have revealed novel photophysics such as enhanced energy transfer, spectral stability, and strongly modified excited state lifetimes and blinking statistics. Here, we review the role of ligands in quantum dot applications and summarize some of our recent efforts probing energy and charge transfer in hybrid CdSe-OPV composite nanostructures

The failure of the diffusional description of the level crossing problem I. Violation of the von Neumann conditions.

The validity of the kinetic equations describing a quantum system coupled to a classical bath was analyzed within the framework of a simple exactly solvable model. The equations were shown to violate the von Neumann conditions if the classical motion is strongly dependent on the state of the quantum system. 1 Introduction The electron transfer (ET) process in condensed media has been under intensive investigation for a few decades. Theoretically, it can be described by a radiationless transition in a quantum two-level system coupled to a large number of polarization modes of environment. The rate of electron transfer can be exactly calculated in two limiting cases. The first one corresponds to the weak coupling situation (nonadiabatic transfer). Accurate expression for the nonadiabatic transfer rate within the second order perturbation theory was found in the sixties [1-3]. The opposite adiabatic case has been successfully investigated more recently (see review [4] and reference herei..