Water vapor at a translational temperature of one kelvin

We report the creation of a confined slow beam of heavy-water (D2O) molecules with a translational temperature around 1 kelvin. This is achieved by filtering slow D2O from a thermal ensemble with inhomogeneous static electric fields exploiting the quadratic Stark shift of D2O. All previous demonstrations of electric field manipulation of cold dipolar molecules rely on a predominantly linear Stark shift. Further, on the basis of elementary molecular properties and our filtering technique we argue that our D2O beam contains molecules in only a few ro-vibrational states.Comment: 4 pages, 4 figures, 1 tabl

Characterization of a Quantum Light Source Based on Spontaneous Parametric Down-Conversion

We have built a quantum light source capable of producing different types of quantum states. The quantum light source is based on entangled state preparation in the process of spontaneous parametric down-conversion. The single-photon detection rate of eight-hundred thousand per second demonstrates that we have created a bright state-of-the-art quantum light source. As a part of the characterization we measured two-photon quantum interference in a Hong-Ou-Mandel interferometer.Comment: 33 page

Nanophotonic hybridization of narrow atomic cesium resonances and photonic stop gaps of opaline nanostructures

We study a hybrid system consisting of a narrowband atomic optical resonance and the long-range periodic order of an opaline photonic nanostructure. To this end, we have infiltrated atomic cesium vapor in a thin silica opal photonic crystal. With increasing temperature, the frequencies of the opal's reflectivity peaks shift down by >20% due to chemical reduction of the silica. Simultaneously, the photonic bands and gaps shift relative to the fixed near-infrared cesium D1 transitions. As a result the narrow atomic resonances with high finesse (f/df=8E5) dramatically change shape from a usual dispersive shape at the blue edge of a stop gap, to an inverted dispersion lineshape at the red edge of a stop gap. The lineshape, amplitude, and off-resonance reflectivity are well modeled with a transfer-matrix model that includes the dispersion and absorption of Cs hyperfine transitions and the chemically-reduced opal. An ensemble of atoms in a photonic crystal is an intriguing hybrid system that features narrow defect-like resonances with a strong dispersion, with potential applications in slow light, sensing and optical memory.Comment: 8 pages, 6 figure

Unlocking innovation for net zero: Constraints, enablers, and firm-level transition strategies

Transition pathways for net zero encompass seemingly insurmountable innovation challenges for the scaling of less mature technological solutions such as hydrogen, materials substitution, and electrification as well as societal challenges to increase the market acceptability of these solutions. In this article, we present a conceptual framework which provides a firm-level perspective on net-zero innovation which has four unique characteristics, i.e. it is complex, systemic, urgent, and directional. The framework shows that the input, process, and output constraints that incumbent firms face in the net-zero transition can be tackled through four firm-level innovation levers – i.e. recombinative, collaborative, integrative, and socio-cognitive capabilities – which, in concert, act as enablers for firms to address these net-zero constraints. We conclude the article by outlining the framework’s main insights for firms’ innovation strategies for net zero and the policy implications. We also propose avenues for future research on net-zero innovation

Continuous loading of an electrostatic trap for polar molecules

A continuously operated electrostatic trap for polar molecules is demonstrated. The trap has a volume of ~0.6 cm^3 and holds molecules with a positive Stark shift. With deuterated ammonia from a quadrupole velocity filter, a trap density of ~10^8/cm^3 is achieved with an average lifetime of 130 ms and a motional temperature of ~300 mK. The trap offers good starting conditions for high-precision measurements, and can be used as a first stage in cooling schemes for molecules and as a "reaction vessel" in cold chemistry.Comment: 4 pages, 3 figures v2: several small improvements, new intr

Trapping of Neutral Rubidium with a Macroscopic Three-Phase Electric Trap

We trap neutral ground-state rubidium atoms in a macroscopic trap based on purely electric fields. For this, three electrostatic field configurations are alternated in a periodic manner. The rubidium is precooled in a magneto-optical trap, transferred into a magnetic trap and then translated into the electric trap. The electric trap consists of six rod-shaped electrodes in cubic arrangement, giving ample optical access. Up to 10^5 atoms have been trapped with an initial temperature of around 20 microkelvin in the three-phase electric trap. The observations are in good agreement with detailed numerical simulations.Comment: 4 pages, 4 figure

Normal-mode spectroscopy of a single bound atom-cavity system

The energy-level structure of a single atom strongly coupled to the mode of a high-finesse optical cavity is investigated. The atom is stored in an intracavity dipole trap and cavity cooling is used to compensate for inevitable heating. Two well-resolved normal modes are observed both in the cavity transmission and the trap lifetime. The experiment is in good agreement with a Monte Carlo simulation, demonstrating our ability to localize the atom to within $\lambda/10$ at a cavity antinode.Comment: 4 pages, 4 figure

Spatially encoded light for Large-alphabet Quantum Key Distribution

Most Quantum Key Distribution protocols use a two-dimensional basis such as HV polarization as first proposed by Bennett and Brassard in 1984. These protocols are consequently limited to a key generation density of 1 bit per photon. We increase this key density by encoding information in the transverse spatial displacement of the used photons. Employing this higher-dimensional Hilbert space together with modern single-photon-detecting cameras, we demonstrate a proof-of-principle large-alphabet Quantum Key Distribution experiment with 1024 symbols and a shared information between sender and receiver of 7 bit per photon.Comment: 9 pages, 6 figures, Added references, Updated Fig. 1 in the main text, Updated Fig.1 in supplementary material, Added section Trojan-horse attacks in supplementary material, title changed, Added paragraphs about final key rate and overfilling the detector to result sectio

Calculating the Fine Structure of a Fabry-Perot Resonator using Spheroidal Wave Functions

A new set of vector solutions to Maxwell's equations based on solutions to the wave equation in spheroidal coordinates allows laser beams to be described beyond the paraxial approximation. Using these solutions allows us to calculate the complete first-order corrections in the short-wavelength limit to eigenmodes and eigenfrequencies in a Fabry-Perot resonator with perfectly conducting mirrors. Experimentally relevant effects are predicted. Modes which are degenerate according to the paraxial approximation are split according to their total angular momentum. This includes a splitting due to coupling between orbital angular momentum and spin angular momentum