400 research outputs found
Discerning Aggregation in Homogeneous Ensembles: A General Description of Photon Counting Spectroscopy in Diffusing Systems
In order to discern aggregation in solutions, we present a quantum mechanical
analog of the photon statistics from fluorescent molecules diffusing through a
focused beam. A generating functional is developed to fully describe the
experimental physical system as well as the statistics. Histograms of the
measured time delay between photon counts are fit by an analytical solution
describing the static as well as diffusing regimes. To determine empirical
fitting parameters, fluorescence correlation spectroscopy is used in parallel
to the photon counting. For expedient analysis, we find that the distribution's
deviation from a single Poisson shows a difference between two single fluor
moments or a double fluor aggregate of the same total intensities. Initial
studies were performed on fixed-state aggregates limited to dimerization.
However preliminary results on reactive species suggest that the method can be
used to characterize any aggregating system.Comment: 30 pages, 5 figure
Charge and spin distributions in GaMnAs/GaAs Ferromagnetic Multilayers
A self-consistent electronic structure calculation based on the
Luttinger-Kohn model is performed on GaMnAs/GaAs multilayers. The Diluted
Magnetic Semiconductor layers are assumed to be metallic and ferromagnetic. The
high Mn concentration (considered as 5% in our calculation) makes it possible
to assume the density of magnetic moments as a continuous distribution, when
treating the magnetic interaction between holes and the localized moment on the
Mn(++) sites. Our calculation shows the distribution of heavy holes and light
holes in the structure. A strong spin-polarization is observed, and the charge
is concentrated mostly on the GaMnAs layers, due to heavy and light holes with
their total angular momentum aligned anti-parallel to the average
magnetization. The charge and spin distributions are analyzed in terms of their
dependence on the number of multilayers, the widths of the GaMnAs and GaAs
layers, and the width of lateral GaAs layers at the borders of the structure.Comment: 12 pages,7 figure
Gap modification of atomically thin boron nitride by phonon mediated interactions
A theory is presented for the modification of bandgaps in atomically thin
boron nitride (BN) by attractive interactions mediated through phonons in a
polarizable substrate, or in the BN plane. Gap equations are solved, and gap
enhancements are found to range up to 70% for dimensionless electron-phonon
coupling \lambda=1, indicating that a proportion of the measured BN bandgap may
have a phonon origin
Electron-Phonon Coupling in Highly-Screened Graphene
Photoemission studies of graphene have resulted in a long-standing
controversy concerning the strength of the experimental electron-phonon
interaction in comparison with theoretical calculations. Using high-resolution
angle-resolved photoemission spectroscopy we study graphene grown on a copper
substrate, where the metallic screening of the substrate substantially reduces
the electron-electron interaction, simplifying the comparison of the
electron-phonon interaction between theory and experiment. By taking the
nonlinear bare bandstructure into account, we are able to show that the
strength of the electron-phonon interaction does indeed agree with theoretical
calculations. In addition, we observe a significant bandgap at the Dirac point
of graphene.Comment: Submitted to Phys. Rev. Lett. on July 20, 201
Generalized Painleve-Gullstrand descriptions of Kerr-Newman black holes
Generalized Painleve-Gullstrand metrics are explicitly constructed for the
Kerr-Newman family of charged rotating black holes. These descriptions are free
of all coordinate singularities; moreover, unlike the Doran and other proposed
metrics, an extra tunable function is introduced to ensure all variables in the
metrics remain real for all values of the mass M, charge Q, angular momentum
aM, and cosmological constant \Lambda > - 3/(a^2). To describe fermions in
Kerr-Newman spacetimes, the stronger requirement of non-singular vierbein
one-forms at the horizon(s) is imposed and coordinate singularities are
eliminated by local Lorentz boosts. Other known vierbein fields of Kerr-Newman
black holes are analysed and discussed; and it is revealed that some of these
descriptions are actually not related by physical Lorentz transformations to
the original Kerr-Newman expression in Boyer-Lindquist coordinates - which is
the reason complex components appear (for certain ranges of the radial
coordinate) in these metrics. As an application of our constructions the
correct effective Hawking temperature for Kerr black holes is derived with the
method of Parikh and Wilczek.Comment: 5 pages; extended to include application to derivation of Hawking
radiation for Kerr black holes with Parikh-Wilczek metho
Quantum walk of a trapped ion in phase space
We implement the proof of principle for the quantum walk of one ion in a
linear ion trap. With a single-step fidelity exceeding 0.99, we perform three
steps of an asymmetric walk on the line. We clearly reveal the differences to
its classical counterpart if we allow the walker/ion to take all classical
paths simultaneously. Quantum interferences enforce asymmetric, non-classical
distributions in the highly entangled degrees of freedom (of coin and position
states). We theoretically study and experimentally observe the limitation in
the number of steps of our approach, that is imposed by motional squeezing. We
propose an altered protocol based on methods of impulsive steps to overcome
these restrictions, in principal allowing to scale the quantum walk to several
hundreds of steps.Comment: 4 pages, 4 figure
Multi-phonon Raman scattering in semiconductor nanocrystals: importance of non-adiabatic transitions
Multi-phonon Raman scattering in semiconductor nanocrystals is treated taking
into account both adiabatic and non-adiabatic phonon-assisted optical
transitions. Because phonons of various symmetries are involved in scattering
processes, there is a considerable enhancement of intensities of multi-phonon
peaks in nanocrystal Raman spectra. Cases of strong and weak band mixing are
considered in detail. In the first case, fundamental scattering takes place via
internal electron-hole states and is participated by s- and d-phonons, while in
the second case, when the intensity of the one-phonon Raman peak is strongly
influenced by the interaction of an electron and of a hole with interface
imperfections (e. g., with trapped charge), p-phonons are most active.
Calculations of Raman scattering spectra for CdSe and PbS nanocrystals give a
good quantitative agreement with recent experimental results.Comment: 16 pages, 2 figures, E-mail addresses: [email protected],
[email protected], [email protected], accepted for publication in
Physical Review
Quantum dots and spin qubits in graphene
This is a review on graphene quantum dots and their use as a host for spin
qubits. We discuss the advantages but also the challenges to use graphene
quantum dots for spin qubits as compared to the more standard materials like
GaAs. We start with an overview of this young and fascinating field and will
then discuss gate-tunable quantum dots in detail. We calculate the bound states
for three different quantum dot architectures where a bulk gap allows for
confinement via electrostatic fields: (i) graphene nanoribbons with armchair
boundary, (ii) a disc in single-layer graphene, and (iii) a disc in bilayer
graphene. In order for graphene quantum dots to be useful in the context of
spin qubits, one needs to find reliable ways to break the valley-degeneracy.
This is achieved here, either by a specific termination of graphene in (i) or
in (ii) and (iii) by a magnetic field, without the need of a specific boundary.
We further discuss how to manipulate spin in these quantum dots and explain the
mechanism of spin decoherence and relaxation caused by spin-orbit interaction
in combination with electron-phonon coupling, and by hyperfine interaction with
the nuclear spin system.Comment: 23 pages, 10 figures, topical review prepared for Nanotechnolog
Coherence properties of a single dipole emitter in diamond
On-demand, high repetition rate sources of indistinguishable, polarised
single photons are the key component for future photonic quantum technologies.
Colour centres in diamond offer a promising solution, and the narrow line-width
of the recently identified nickel-based NE8 centre makes it particularly
appealing for realising the transform-limited sources necessary for quantum
interference. Here we report the characterisation of dipole orientation and
coherence properties of a single NE8 colour centre in a diamond nanocrystal at
room-temperature. We observe a single photon coherence time of 0.21 ps and an
emission lifetime of 1.5 ns. Combined with an emission wavelength that is
ideally suited for applications in existing quantum optical systems, these
results show that the NE8 is a far more promising source than the more commonly
studied nitrogen-vacancy centre and point the way to the realisation of a
practical diamond colour centre-based single photon source.Comment: 10 pages, 4 colour figure
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