Depth profile photoemission study of thermally diffused Mn/GaAs (001) interfaces

We have performed a depth profile study of thermally diffused Mn/GaAs (001) interfaces using photoemission spectroscopy combined with Ar$^+$-ion sputtering. We found that Mn ion was thermally diffused into the deep region of the GaAs substrate and completely reacted with GaAs. In the deep region, the Mn 2$p$ core-level and Mn 3$d$ valence-band spectra of the Mn/GaAs (001) sample heated to 600 $^{\circ}$C were similar to those of Ga$_{1-x}$Mn$_x$As, zinc-blende-type MnAs dots, and/or interstitial Mn in tetrahedrally coordinated by As atoms, suggesting that the Mn 3$d$ states were essentially localized but were hybridized with the electronic states of the host GaAs. Ferromagnetism was observed in the dilute Mn phase.Comment: 5 pages, 4 figure

Indication of antiferromagnetic interaction between paramagnetic Co ions in the diluted magnetic semiconductor Zn1−x_{1-x}Cox_{x}O

The magnetic properties of Zn$_{1-x}$Co$_x$O ($x=0.07$ and 0.10) thin films, which were homo-epitaxially grown on a ZnO(0001) substrates with varying relatively high oxygen pressure, have been investigated using x-ray magnetic circular dichroism (XMCD) at Co $2p$ core-level absorption edge. The line shapes of the absorption spectra are the same in all the films and indicate that the Co$^{2+}$ ions substitute for the Zn sites. The magnetic-field and temperature dependences of the XMCD intensity are consistent with the magnetization measurements, indicating that except for Co there are no additional sources for the magnetic moment, and demonstrate the coexistence of paramagnetic and ferromagnetic components in the homo-epitaxial Zn$_{1-x}$Co$_{x}$O thin films, in contrast to the ferromagnetism in the hetero-epitaxial Zn$_{1-x}$Co$_{x}$O films studied previously. The analysis of the XMCD intensities using the Curie-Weiss law reveals the presence of antiferromagnetic interaction between the paramagnetic Co ions. Missing XMCD intensities and magnetization signals indicate that most of Co ions are non-magnetic probably because they are strongly coupled antiferromagnetically with each other. Annealing in a high vacuum reduces both the paramagnetic and ferromagnetic signals. We attribute the reductions to thermal diffusion and aggregation of Co ions with antiferromagnetic nanoclusters in Zn$_{1-x}$Co$_{x}$O.Comment: 21 pages, 7 figures, accepted for Physical Review

Optical and transport properties in doped two-leg ladder antiferromagnet

Within the t-J model, the optical and transport properties of the doped two-leg ladder antiferromagnet are studied based on the fermion-spin theory. It is shown that the optical and transport properties of the doped two-leg ladder antiferromagnet are mainly governed by the holon scattering. The low energy peak in the optical conductivity is located at a finite energy, while the resistivity exhibits a crossover from the high temperature metallic-like behavior to the low temperature insulating-like behavior, which are consistent with the experiments.Comment: 13 pages, 5 figures, accepted for publication in Phys. Rev. B65 (2002) (April 15 issue

Nuclear Spin Relaxation in Hole Doped Two-Leg Ladders

The nuclear spin-lattice relaxation rate ($1/T_{1}$) has been measured in the single crystals of hole doped two-leg ladder compounds Sr$_{14-x}$Ca$_{x}$Cu$_{24}$O$_{41}$ and in the undoped parent material La$_6$Ca$_8$Cu$_{24}$O$_{41}$. Comparison of $1/T_{1}$ at the Cu and the two distinct oxygen sites revealed that the major spectral weight of low frequency spin fluctuations is located near $q \sim (\pi, \pi)$ for most of the temperature and doping ranges investigated. Remarkable difference in the temperature dependence of $1/T_1$ for the two oxygen sites in the heavily doped $x$=12 sample revealed reduction of singlet correlations between two legs in place of growing antiferromagnetic correlations along the leg direction with increasing temperature. Such behavior is most likely caused by the dissociation of bound hole pairs.Comment: 4 pages. to appear in J. Phys. Soc. Jpn. Vol. 6

Nonlinear optical response and spin-charge separation in one-dimensional Mott insulators

We theoretically study the nonlinear optical response and photoexcited states of the Mott insulators. The nonlinear optical susceptibility \chi^(3) is calculated by using the exact diagonalization technique on small clusters. From the systematic study of the dependence of \chi^(3) on dimensionality, we find that the spin-charge separation plays a crucial role in enhancing \chi^(3) in the one-dimensional (1D) Mott insulators. Based on this result, we propose a holon-doublon model, which describes the nonlinear response in the 1D Mott insulators. These findings show that the spin-charge separation will become a key concept of optoelectronic devices.Comment: 5 pages with 3 figures, to appear in PRB RC, 15 August 200

Quantum Spin Systems: From Spin Gaps to Pseudo Gaps

Many low dimensional spin systems with a dimerized or ladder-like antiferromagnetic exchange coupling have a gapped excitation spectrum with magnetic bound states within the spin gap. For spin ladders with an even number of legs the existence of spin gaps and within the t-J model a tendency toward superconductivity with d-wave symmetry is predicted. In the following we will characterize the spin excitation spectra of different low dimensional spin systems taking into account strong spin phonon interaction ($\rm CuGeO_3$), charge ordering ($\rm NaV_2O_5$) and doping on chains and ladders (\ladder). The spectroscopic characterization of the model systems mentioned above has been performed using magnetic inelastic light scattering originating from a spin conserving exchange scattering mechanism. This is also bound to yield more insight into the interrelation between these spin gap excitations and the origin of the pseudo gap in high temperature superconductors.Comment: 10 pages, 5 figure

Superconductivuty versus Tunneling in a Doped Antiferromagnetic Ladder

The low-energy charge excitations of a doped antiferromagnetic ladder are modeled by a system of interacting spinless fermions that live on the same ladder. A relatively large spin gap is assumed to ``freeze out'' all spin fluctuations. We find that the formation of rung hole pairs coincides with the opening of a single-particle gap for charge excitations along chains and with the absence of coherent tunneling in between chains. We also find that such hole pairs condense into either a crystalline or superconducting state as a function of the binding energy.Comment: 15 pgs. in PLAIN TeX, 2 figs. in postscript, to appear in Phys. Rev.

Cu-O network-dependent core-hole screening in low-dimensional cuprate systems: a high-resolution X-ray photoemission study

We present an experimental study of the dynamics of holes in the valence bands of zero-, one-, and two-dimensional undoped model cuprates, as expressed via the screening of a Cu 2p core hole. The response depends strongly upon the dimensionality and the details of the Cu-O-Cu network geometry and clearly goes beyond the present theoretical state-of-the-art description within the three-band d-p model

Electronic Structure of Ladder Cuprates

We study the electronic structure of the ladder compounds (SrCa)CuO 14-24-41 and SrCuO 123. LDA calculations for both give similar Cu 3d-bands near the Fermi energy. The hopping parameters estimated by fitting LDA energy bands show a strong anisotropy between the t_perp t_par intra-ladder hopping and small inter-ladder hopping. A downfolding method shows that this anisotropy arises from the ladder structure.The conductivity perpendicular to the ladders is computed assuming incoherent tunneling giving a value close to experiment.Comment: 5 pages, 3 figure

Magnetic excitations and structural change in the S=1/2 quasi-one-dimensional magnet Sr_{14-x}Y_{x}Cu_{24}O_{41} (0<x<1)

Neutron scattering measurements have been performed on the S=1/2 quasi-one-dimensional system Sr_{14-x}Y_{x}Cu_{24}O_{41}, which has both simple chains and two-leg ladders of copper ions. We observed that when a small amount of yttrium is substituted for strontium, which is expected to reduce the number of holes, the dimerized state and the structure in the chain are changed drastically. The inelastic peaks originating from the dimerized state of the chain becomes broader in energy but not in momentum space. This implies that the dimerized state becomes unstable but the spin correlations are unchanged with yttrium substitution. Furthermore, it was observed that nuclear Bragg peak intensities originating from the chain show strong temperature and x dependence, which suggests that the chains slide along the c axis as temperature and x are varied.Comment: 5 pages, 6 figures, to appear in Phys. Rev.