8 research outputs found
Frustrated network of indirect exchange paths between tetrahedrally coordinated Co in Ba2 CoO4
We present a detailed study of the electronic and magnetic interactions of Ba2CoO4, structurally very uncommon because of the isolated CoO4 distorted tetrahedral coordination. We show the presence of Co(d)-O(p) hybridized states characterized by spin polarized oxygen atoms, with their magnetic moments parallel to that on Co. The calculated isotropic exchange interaction parameters, which include the contributions from ligand spins, demonstrate the presence of a three-dimensional (3D) network of magnetic couplings that are partially frustrated in the identified magnetic ground state. Our results indicate that the dominant indirect exchange mechanism responsible for this ground state is mediated by O atoms along the Co-O »O-Co path
Mn-induced Fermi-surface reconstruction in the SmFeAsO parent compound
The electronic ground state of iron-based materials is unusually sensitive to electronic correlations. Among others, its delicate balance is profoundly affected by the insertion of magnetic impurities in the FeAs layers. Here, we address the effects of Fe-to-Mn substitution in the non-superconducting Sm-1111 pnictide parent compound via a comparative study of SmFe1-xMnxAsO samples with x(Mn) = 0.05 and 0.10. Magnetization, Hall effect, and muon-spin spectroscopy data provide a coherent picture, indicating a weakening of the commensurate Fe spin-density-wave (SDW) order, as shown by the lowering of the SDW transition temperature TSDW with increasing Mn content, and the unexpected appearance of another magnetic order, occurring at T∗≈ 10 and 20 K for x= 0.05 and 0.10, respectively. We attribute the new magnetic transition at T∗, occurring well inside the SDW phase, to a reorganization of the Fermi surface due to Fe-to-Mn substitutions. These give rise to enhanced magnetic fluctuations along the incommensurate wavevector Q2= (π± δ, π± δ) , further increased by the RKKY interactions among Mn impurities
Pressure-induced antiferromagnetic dome in the heavy-fermion Yb2Pd2In1−xSnx system
In the heavy-fermion system Yb2Pd2In1−xSnx, the interplay of crystal-field splitting, Kondo effect, and Ruderman-Kittel-Kasuya-Yosida interactions leads to complex chemical-, pressure-, and magnetic-field phase diagrams still to be explored in full detail. By using a series of techniques, we show that even modest changes of parameters other than temperature are sufficient to induce multiple quantum-critical transitions in this highly susceptible heavy-fermion family. In particular, we show that, above ∼10 kbar, hydrostatic pressure not only induces an antiferromagnetic phase at low temperature, but it likely leads to a reorientation of the Yb magnetic moments and/or the competition among different antiferromagnetic configurations