10 research outputs found

    Cross-sections for the 27 ⁣Al(γ,x)24Na{^{27}\!\rm{Al}}(\gamma,\textit{x})^{24}\rm{Na} multiparticle reaction at EγmaxE_{\rm{\gamma max}} = 40 ÷\div 95 MeV

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    The bremsstrahlung flux-averaged cross-sections σ(Eγmax)\langle{\sigma(E_{\rm{\gamma max}})}\rangle and the cross-sections per equivalent photon σ(Eγmax)Q\langle{\sigma(E_{\rm{\gamma max}})_{\rm{Q}}}\rangle were measured for the photonuclear multiparticle reaction 27 ⁣Al(γ,x;x=3He+pd+2pn)24Na^{27}\!\rm{Al}(\gamma,\textit{x}; \textit{x} = {^{3}\rm{He}} + pd + 2pn)^{24}\rm{Na} at bremsstrahlung end-point energies ranging from 40 MeV to 95 MeV. The experiments were performed using the beam from the NSC KIPT electron linear accelerator LUE-40 with the use of the γ\gamma-activation technique. The bremsstrahlung quantum flux was calculated with the program GEANT4 and, in addition, was monitored by means of the 100Mo(γ,n)99Mo^{100}\rm{Mo}(\gamma,n)^{99}\rm{Mo} reaction. The cross-sections σ(E)\sigma(E) were computed using the TALYS1.9 code with the default options. The measured average cross-sections σ(Eγmax)\langle{\sigma(E_{\rm{\gamma max}})}\rangle and σ(Eγmax)Q\langle{\sigma(E_{\rm{\gamma max}})_{\rm{Q}}}\rangle have appeared to be higher by factors of 2.0 to 2.4 than the theoretical results. The experimental results have been found to be in good agreement with the data of other laboratories. Consideration is given to special features of calculation of σ(Eγmax)\langle{\sigma(E_{\rm{\gamma max}})}\rangle and σ(Eγmax)Q\langle{\sigma(E_{\rm{\gamma max}})_{\rm{Q}}}\rangle for the 27 ⁣Al(γ,x)24Na^{27}\!\rm{Al}(\gamma,\textit{x})^{24}\rm{Na} reaction, with occurrence of three 27 ⁣Al^{27}\!\rm{Al} photodisintegration channels. The paper also discusses the possibility of using the 27 ⁣Al(γ,x)24Na^{27}\!\rm{Al}(\gamma,\textit{x})^{24}\rm{Na} reaction for monitoring the bremsstrahlung γ\gamma-quantum flux in the photon energy region above 30 MeV.Comment: 16 pages, 6 figures, 1 tabl

    Isomeric pair 95m,gNb{^{95\rm m,g}\rm{Nb}} in photonuclear reactions on nat^{\rm nat}Mo at end-point bremsstrahlung energy of 35-95 MeV

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    The natMo(γ,xnp)95m,g{^{\rm nat}\rm{Mo}}(\gamma,x\rm np)^{95\rm m,g}Nb photonuclear reaction was studied using the electron beam from the NSC KIPT linear accelerator LUE-40. Experiment was performed using the activation and off-line γ\gamma-ray spectrometric technique. The experimental isomeric yield ratio d(Eγmax)=Ym(Eγmax)/Yg(Eγmax)d(E_{\rm{\gamma max}}) = Y_{\rm m}(E_{\rm{\gamma max}}) / Y_{\rm g}(E_{\rm{\gamma max}}) was determined for the reaction products 95m,gNb^{95\rm m,g}\rm{Nb} at the end-point bremsstrahlung energy EγmaxE_{\rm{\gamma max}} range of 35-95 MeV. The obtained values of d(Eγmax)d(E_{\rm{\gamma max}}) are in satisfactory agreement with the results of other authors and extend the range of previously known data. The theoretical values of the yields Ym,g(Eγmax)Y_{\rm m,g}(E_{\rm{\gamma max}}) and the isomeric yield ratio d(Eγmax)d(E_{\rm{\gamma max}}) for the isomeric pair 95m,gNb^{95\rm m,g}\rm{Nb} from the natMo(γ,xnp){^{\rm nat}\rm{Mo}}(\gamma,x\rm np) reaction were calculated using the partial cross-sections σ(E)\sigma(E) from the TALYS1.95 code for six different level density models LDLD. The comparison showed a noticeable excess (more than 3.85 times) of the experimental isomeric yield ratio over all theoretical estimates. At the investigated range of EγmaxE_{\rm{\gamma max}} the theoretical dependence of d(Eγmax)d(E_{\rm{\gamma max}}) on energy was confirmed - the isomeric yield ratio smoothly decreases with increasing energy.Comment: 9 pages, 9 figures, 1 tabl

    Magnetic system for cleaning the gamma beam at the LUE-40 electron linac output

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    The bremsstrahlung of accelerated electrons passing through a converter is used to study multiparticle photo-nuclear reactions. The results of calculations, numerical modeling, design, and testing of a special magnetic cleaning system to obtain a "pure" beam of bremsstrahlung quanta when studying the cross-sections of such reactions at the LUE-40 linac are presented. The system is based on commercially available permanent magnets of rectangular cross-sections. The maximum on-axis field is 0.9 T, which provides sufficient separation of the electron beam and gamma rays at a distance of more than 90 mm from the magnet.Comment: 9 pages, 8 figure

    Production of 180m{^{180\rm{m}}}Hf in photoproton reaction 181{^{181}}Ta(γ,p)(\gamma,p) at energy EγmaxE_{\rm{\gamma max}} = 35-95 MeV

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    The production of the 180mHf^{180\rm{m}}\rm{Hf} nuclei in the photoproton reaction 181Ta(γ,p){^{181}\rm{Ta}}(\gamma,p) was studied at end-point bremsstrahlung energies EγmaxE_{\rm{\gamma max}} = 35-95 MeV. The experiment was performed at the electron linear accelerator LUE-40 NSC KIPT with the use of the γ\gamma activation and off-line γ\gamma-ray spectroscopy. The experimental values of the bremsstrahlung flux-averaged cross-sections σ(Eγmax)m\langle{\sigma(E_{\rm{\gamma max}})}\rangle_{\rm{m}} for the 181Ta(γ,p)180mHf{^{181}\rm{Ta}}(\gamma,p)^{180\rm{m}}\rm{Hf} reaction were determined, and at Eγmax>55E_{\rm{\gamma max}} > 55 MeV obtained for the first time. The measured values, also as the literature data, are significantly exceed the theoretical flux-averaged cross-sections σ(Eγmax)th\langle{\sigma(E_{\rm{\gamma max}})}\rangle_{\rm{th}}. The σ(Eγmax)th\langle{\sigma(E_{\rm{\gamma max}})}\rangle_{\rm{th}} values were calculated using the cross-section σ(E)\sigma(E) computed with the TALYS1.95 code for six different level density models. A comparative analysis of the calculated total cross-sections for the reactions 181Ta(γ,p)180Hf{^{181}\rm{Ta}}(\gamma,p)^{180}\rm{Hf} and 181Ta(γ,n)180Ta{^{181}\rm{Ta}}(\gamma,n)^{180}\rm{Ta} was performed. It was shown that the photoproton (γ,p)(\gamma,p) to photoneutron (γ,n)(\gamma,n) strength ratio is consistent with the estimates based on the isospin selection rules and the value from the (e,ep)(e,e'p) experiment.Comment: 9 pages, 4 figures, 2 table

    Photonuclear reactions cross-sections at energies up to 100 MeV for different experimental setups

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    In experiments on the electron linac LUE-40 of RDC "Accelerator" NSC KIPT, the flux-averaged cross-sections σ(Eγmax)exp\langle{\sigma(E_{\rm{\gamma max}})}\rangle_{\rm{exp}} of photonuclear reactions 100Mo(γ,n)99Mo{^{100}\rm{Mo}}(\gamma,n)^{99}\rm{Mo}, 27Al(γ,x)24Na{^{27}\rm{Al}}(\gamma,x)^{24}\rm{Na}, 93Nb(γ,n)92mNb{^{93}\rm{Nb}}(\gamma,n)^{92m}\rm{Nb}, 93Nb(γ,3n)90Nb{^{93}\rm{Nb}}(\gamma,3n)^{90}\rm{Nb}, and 181Ta(γ,n)180gTa{^{181}\rm{Ta}}(\gamma,n)^{180g}\rm{Ta} were measured using the γ\gamma-activation technique. The theoretical flux-average cross-sections σ(Eγmax)th\langle{\sigma(E_{\rm{\gamma max}})}\rangle_{\rm{th}} were computed using the partial cross-section σ(E)\sigma(E) values from the TALYS1.9-1.95 codes and bremsstrahlung γ\gamma-flux calculated using GEANT4.9.2. Two different experimental setups were used in the experiments: an aluminum electron absorber and a deflecting magnet to clean the bremsstrahlung γ\gamma-flux from electrons. A comparison of the flux-average cross-sections measured for two experimental setups was performed. The possibility of using the reactions 100Mo(γ,n)99Mo{^{100}\rm{Mo}}(\gamma,n)^{99}\rm{Mo}, 27Al(γ,x)24Na{^{27}\rm{Al}}(\gamma,x)^{24}\rm{Na}, 93Nb(γ,n)92mNb{^{93}\rm{Nb}}(\gamma,n)^{92m}\rm{Nb}, 93Nb(γ,3n)90Nb{^{93}\rm{Nb}}(\gamma,3n)^{90}\rm{Nb}, and 181Ta(γ,n)180gTa{^{181}\rm{Ta}}(\gamma,n)^{180g}\rm{Ta} as monitors of the bremsstrahlung γ\gamma-flux for the energy range 30-100 MeV was investigated.Comment: 8 pages, 6 figures, 1 tabl

    Photoneutron cross-sections for the reactions

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    The flux-averaged cross-sections σ(Eγmax)\langle {\sigma (E_{\gamma \mathrm{max}})}\rangle for the 181Ta(γ,xn;x=1^{181}\mathrm{Ta}(\gamma ,\textit{x}n; \textit{x} = 18)181xTa8)^{181-\textit{x}}\mathrm{Ta} reactions have been measured at the end-point bremsstrahlung energies of 80–95 MeV. The experiments were performed by using the beam from the NSC KIPT electron linear accelerator LUE-40 and measuring the residual γ\gamma -ray activities of the reaction products. The theoretical σ(Eγmax)\langle {\sigma (E_{\gamma \mathrm{max}})}\rangle values were computed using the mono-energetic cross-sections σ(E)\sigma (E) from TALYS1.9 code. A comparison between the measured average cross-sections and the theoretical values show good agreement for the (γ,1(\gamma ,16n)6\mathrm{n}) reactions but substantial differences for the (γ,7n)(\gamma ,7\mathrm{n}) and (γ,8n)(\gamma ,8\mathrm{n}) reactions. Isomeric average cross-section ratios d(Eγmax)d(E_{\gamma \mathrm{max}}) of a product 178g,mTa^{178g,m}\mathrm{Ta} produced from the 181Ta(γ,3n)^{181}\mathrm{Ta}(\gamma ,3\mathrm{n}) reaction have been obtained. The results have been compared with the literature data and the theoretical values based on TALYS1.9 code

    Cross-sections for the 27 ⁣al(γ,x)22na{^{27}\!\rm{al}}(\gamma,\textit{x})^{22}\rm{na} multichannel reaction with the 28.3 mev difference of the reaction thresholds

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    The bremsstrahlung flux-averaged cross-sections σ(Eγmax)\langle{\sigma(E_{\rm{\gamma max}})}\rangle and the cross-sections per equivalent photon σ(Eγmax)Q\langle{\sigma(E_{\rm{\gamma max}})_{\rm{Q}}}\rangle were first measured for the photonuclear multichannel reaction 27 ⁣Al(γ,x)22Na{^{27}\!\rm{Al}}(\gamma,\textit{x})^{22}\rm{Na} at end-point bremsstrahlung gamma energies ranging from 35 MeV to 95 MeV. The experiments were performed with the beam from the NSC KIPT electron linear accelerator LUE-40 with the use of the γ\gamma-activation technique. The bremsstrahlung quantum flux was calculated with the program GEANT4.9.2 and, in addition, was monitored by means of the 100Mo(γ,n)99Mo^{100}\rm{Mo}(\gamma,n)^{99}\rm{Mo} reaction. The flux-averaged cross-sections were calculated using the partial cross-section σ(E)\sigma(E) values computed with the TALYS1.95 code for different level density models. Consideration is given to special features of calculating the cross-sections σ(Eγmax)\langle{\sigma(E_{\rm{\gamma max}})}\rangle and σ(Eγmax)Q\langle{\sigma(E_{\rm{\gamma max}})_{\rm{Q}}}\rangle for the case of the final nucleus 22Na^{22}\rm{Na} production in the 27 ⁣Al^{27}\!\rm{Al} photodisintegration reaction via several partial channels x\textit{x}: nα+dt+npt+2n3He+n2d+2npd+2p3n\rm{n}\alpha + dt + npt + 2n{^{3}\rm{He}} + n2d + 2npd + 2p3n.Comment: 8 pages, 9 figures, 1 table, 19 references. arXiv admin note: text overlap with arXiv:2012.1447
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