Ferromagnetism and non-local correlations in the Hubbard model

We study the possibility and stability of band-ferromagnetism in the single-band Hubbard model for the simple cubic (SC) lattice. A non-local self-energy is derived within a modified perturbation theory. Results for the spectral density and quasiparticle density of states are shown with special attention to the effects of k-dependence. The importance of non-local correlations for the fulfillment of the Mermin-Wagner theorem is our main result. A phase digram showing regions of ferromagnetic order is calculated for the three dimensional lattice. Besides, we show results for the optical conductivity and prove that already the renormalized one-loop contribution to the conductivity cancels the Drude peak exactly in case of a local self-energy which is not anymore true for a non-local self-energy.Comment: 11 pages, 10 figures, accepted for publication in PR

Spin-filter effect of the europium chalcogenides: An exactly solved many-body model

A model Hamiltonian is introduced which considers the main features of the experimental spin filter situation as s-f interaction, planar geometry and the strong external electric field. The proposed many-body model can be solved analytically and exactly using Green functions. The spin polarization of the field-emitted electrons is expressed in terms of spin-flip probabilities, which on their part are put down to the exactly known dynamic quantities of the system. The calculated electron spin polarization shows remarkable dependencies on the electron velocity perpendicular to the emitting plane and the strength of s-f coupling. Experimentally observed polarization values of about 90% are well understood within the framework of the proposed model.Comment: accepted (Physical Review B); 10 pages, 11 figures; http://orion.physik.hu-berlin.de

Carrier induced ferromagnetism in diluted local-moment systems

The electronic and magnetic properties of concentrated and diluted ferromagnetic semiconductors are investigated by using the Kondo lattice model, which describes an interband exchange coupling between itinerant conduction electrons and localized magnetic moments. In our calculations, the electronic problem and the local magnetic problem are solved separately. For the electronic part an interpolating self-energy approach together with a coherent potential approximation (CPA) treatment of a dynamical alloy analogy is used to calculate temperature-dependent quasiparticle densities of states and the electronic self-energy of the diluted local-moment system. For constructing the magnetic phase diagram we use a modified RKKY theory by mapping the interband exchange to an effective Heisenberg model. The exchange integrals appear as functionals of the diluted electronic self-energy being therefore temperature- and carrier-concentration-dependent and covering RKKY as well as double exchange behavior. The disorder of the localized moments in the effective Heisenberg model is solved by a generalized locator CPA approach. The main results are: 1) extremely low carrier concentrations are sufficient to induce ferromagnetism; 2) the Curie temperature exhibits a strikingly non-monotonic behavior as a function of carrier concentration with a distinct maximum; 3) $T_C$ curves break down at critical $n/x$ due to antiferromagnetic correlations and 4) the dilution always lowers $T_C$ but broadens the ferromagnetic region with respect to carrier concentration.Comment: 11 pages, 5 figure

Ferromagnetic Kondo-Lattice Model

We present a many-body approach to the electronic and magnetic properties of the (multiband) Kondo-lattice model with ferromagnetic interband exchange. The coupling between itinerant conduction electrons and localized magnetic moments leads, on the one hand, to a distinct temperature-dependence of the electronic quasiparticle spectrum and, on the other hand, to magnetic properties, as e.~g.the Curie temperature T_C or the magnon dispersion, which are strongly influenced by the band electron selfenergy and therewith in particular by the carrier density. We present results for the single-band Kondo-lattice model in terms of quasiparticle densities of states and quasiparticle band structures and demonstrate the density-dependence of the self-consistently derived Curie temperature. The transition from weak-coupling (RKKY) to strong-coupling (double exchange) behaviour is worked out. The multiband model is combined with a tight-binding-LMTO bandstructure calculation to describe real magnetic materials. As an example we present results for the archetypal ferromagnetic local-moment systems EuO and EuS. The proposed method avoids the double counting of relevant interactions and takes into account the correct symmetry of atomic orbitals.Comment: 15 pages, 10 figure

Proper weak-coupling approach to the periodic s-d(f) exchange model

The periodic s-d(f) exchange model is characterized by a wide variety of interesting applications, a simple mathematical structure and a limited number of reliable approximations which take care of the quantum nature of the participating spins. We suggest the use of a projection-operator method for getting information perturbationally, which are not accessible via diagrammatic approaches. In this paper we present in particular results beyond perturbation theory, which are obtained such that almost all exactly known limiting cases are incorporated correctly. We discuss a variety of possible methods and evaluate their consequences for one-particle properties. These considerations serve as a guideline for a more effective approach to the model.Comment: 11 pages, 6 figures; accepted by Phys. Rev.

Two-band ferromagnetic Kondo-lattice model for local-moment half-metals

We introduce a two-band Kondo-lattice model to describe ferromagnetic half-metals with local magnetic moments. In a model study, the electronic and magnetic properties are presented by temperature dependent magnetization curves, band-structures, spin polarizations and plasma frequencies. These are obtained from numerically evaluated equations, based on the single-electron Green functions. We show that the mutual influence between the itinerant electrons and the local magnetic moments is responsible for several phase transitions of the half-metals, namely first and second order magnetic phase transitions, as well as half-metal to semiconductor and half-metal to semimetal transitions.Comment: 10 pages, 5 figures, submitted to Journal of Physics: Condensed Matte

Quantum effects in the quasiparticle structure of the ferromagnetic Kondo lattice model

A new ``Dynamical Mean-field theory'' based approach for the Kondo lattice model with quantum spins is introduced. The inspection of exactly solvable limiting cases and several known approximation methods, namely the second-order perturbation theory, the self-consistent CPA and finally a moment-conserving decoupling of the equations of motion help in evaluating the new approach. This comprehensive investigation gives some certainty to our results: Whereas our method is somewhat limited in the investigation of the J<0-model, the results for J>0 reveal important aspects of the physics of the model: The energetically lowest states are not completely spin-polarized.A band splitting, which occurs already for relatively low interaction strengths, can be related to distinct elementary excitations, namely magnon emission (absorption) and the formation of magnetic polarons. We demonstrate the properties of the ferromagnetic Kondo lattice model in terms of spectral densities and quasiparticle densities of states.Comment: 19 pages, 4 figure

The temperature dependent bandstructure of a ferromagnetic semiconductor film

The electronic quasiparticle spectrum of a ferromagnetic film is investigated within the framework of the s-f model. Starting from the exact solvable case of a single electron in an otherwise empty conduction band being exchange coupled to a ferromagnetically saturated localized spin system we extend the theory to finite temperatures. Our approach is a moment-conserving decoupling procedure for suitable defined Green functions. The theory for finite temperatures evolves continuously from the exact limiting case. The restriction to zero conduction band occupation may be regarded as a proper model description for ferromagnetic semiconductors like EuO and EuS. Evaluating the theory for a simple cubic film cut parallel to the (100) crystal plane, we find some marked correlation effects which depend on the spin of the test electron, on the exchange coupling, and on the temperature of the local-moment system.Comment: 11 pages, 9 figure

Spin-polarized tunneling currents through a ferromagnetic insulator between two metallic or superconducting leads

Using the Keldysh formalism the tunneling current through a hybrid structure where a confined magnetic insulator (I) is sandwiched between two non-magnetic leads is calculated. The leads can be either normal metals (M) or superconductors (S). Each region is modelled as a single band in tight-binding approximation in order to understand the formation of the tunneling current as clearly as possible. The tunneling process itself is simulated by a hybridization between the lead and insulator conduction bands. The insulator is assumed to have localized moments which can interact with the tunneling electrons. This is described by the Kondo Lattice Model (KLM) and treated within an interpolating self-energy approach. For the superconductor the mean-field BCS theory is used. The spin polarization of the current shows a strong dependence both on the applied voltage and the properties of the materials. Even for this idealized three band model there is a qualitative agreement with experiment.Comment: 15 pages, 23 figures, accepted for publication in PR

Temperature-dependent electronic structure and ferromagnetism in the d=oo Hubbard model studied by a modfied perturbation theory

The infinite-dimensional Hubbard model is studied by means of a modified perturbation theory. The approach reduces to the iterative perturbation theory for weak coupling. It is exact in the atomic limit and correctly reproduces the dispersions and the weights of the Hubbard bands in the strong-coupling regime for arbitrary fillings. Results are presented for the hyper-cubic and an fcc-type lattice. For the latter we find ferromagnetic solutions. The filling-dependent Curie temperature is compared with the results of a recent Quantum Monte Carlo study.Comment: RevTeX, 5 pages, 6 eps figures included, Phys. Rev. B (in press), Ref. 16 correcte