Measurement of the production branching ratios following nuclear muon capture for palladium isotopes using the in-beam activation method

Background: The energy distribution of excited states populated by the nuclear muon capture reaction can facilitate an understanding of the reaction mechanism; however, experimental data are fairly sparse. Purpose: We developed a new methodology, called the in-beam activation method, to measure the production probability of residual nuclei by muon capture. For the first application of the new method, we have measured muon-induced activation of five isotopically-enriched palladium targets. Methods: The experiment was conducted at the RIKEN-RAL muon facility of the Rutherford Appleton Facility in the UK. The pulsed muon beam impinged on the palladium targets and gamma rays from the beta and isomeric decays from the reaction residues were measured using high-purity germanium detectors in both the in-beam and offline setups. Results: The production branching ratios of the residual nuclei of muon capture for five palladium isotopes with mass numbers A = 104, 105, 106, 108, and 110 were obtained. The results were compared with a model calculation using the particle and heavy ion transport system (PHITS) code. The model calculation well reproduces the experimental data. Conclusion: For the first time, this study provides experimental data on the distribution of production branching ratios without any theoretical estimation or assumptions in the interpretation of the data analysisComment: 20 pages, 11 figure

Correlation dynamics between electrons and ions in the fragmentation of D2_2 molecules by short laser pulses

We studied the recollision dynamics between the electrons and D$_2^+$ ions following the tunneling ionization of D$_2$ molecules in an intense short pulse laser field. The returning electron collisionally excites the D$_2^+$ ion to excited electronic states from there D$_2^+$ can dissociate or be further ionized by the laser field, resulting in D$^+$ + D or D$^+$ + D$^+$, respectively. We modeled the fragmentation dynamics and calculated the resulting kinetic energy spectrum of D$^+$ to compare with recent experiments. Since the recollision time is locked to the tunneling ionization time which occurs only within fraction of an optical cycle, the peaks in the D$^+$ kinetic energy spectra provides a measure of the time when the recollision occurs. This collision dynamics forms the basis of the molecular clock where the clock can be read with attosecond precision, as first proposed by Corkum and coworkers. By analyzing each of the elementary processes leading to the fragmentation quantitatively, we identified how the molecular clock is to be read from the measured kinetic energy spectra of D$^+$ and what laser parameters be used in order to measure the clock more accurately.Comment: 13 pages with 14 figure

High-order harmonic generation with a strong laser field and an attosecond-pulse train: the Dirac Delta comb and monochromatic limits

In recent publications, it has been shown that high-order harmonic generation can be manipulated by employing a time-delayed attosecond pulse train superposed to a strong, near-infrared laser field. It is an open question, however, which is the most adequate way to approximate the attosecond pulse train in a semi-analytic framework. Employing the Strong-Field Approximation and saddle-point methods, we make a detailed assessment of the spectra obtained by modeling the attosecond pulse train by either a monochromatic wave or a Dirac-Delta comb. These are the two extreme limits of a real train, which is composed by a finite set of harmonics. Specifically, in the monochromatic limit, we find the downhill and uphill sets of orbits reported in the literature, and analyze their influence on the high-harmonic spectra. We show that, in principle, the downhill trajectories lead to stronger harmonics, and pronounced enhancements in the low-plateau region. These features are analyzed in terms of quantum interference effects between pairs of quantum orbits, and compared to those obtained in the Dirac-Delta limit.Comment: 10 pages, 7 figures (eps files). To appear in Laser Physic

Coherent Electron Scattering Captured by an Attosecond Quantum Stroboscope

The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with efficient detection techniques. The generation of extreme ultraviolet (XUV) attosecond (1 as = 10-18 s) pulses has, for the first time, made direct measurements of electron dynamics possible. Nevertheless, while various applications of attosecond pulses have been demonstrated experimentally, no one has yet captured or controlled the full three dimensional motion of an electron on an attosecond time scale. Here we demonstrate an attosecond quantum stroboscope capable of guiding and imaging electron motion on a sub-femtosecond (1 fs = 10-15 s) time scale. It is based on a sequence of identical attosecond pulses which are synchronized with a guiding laser field. The pulse to pulse separation in the train is tailored to exactly match an optical cycle of the laser field and the electron momentum distributions are detected with a velocity map imaging spectrometer (VMIS). This technique has enabled us to guide ionized electrons back to their parent ion and image the scattering event. We envision that coherent electron scattering from atoms, molecules and surfaces captured by the attosecond quantum stroboscope will complement more traditional scattering techniques since it provides high temporal as well as spatial resolution.Comment: 6 pages, 4 figure