Spin-Cooling of the Motion of a Trapped Diamond

Observing and controlling macroscopic quantum systems has long been a driving force in research on quantum physics. In this endeavor, strong coupling between individual quantum systems and mechanical oscillators is being actively pursued. While both read-out of mechanical motion using coherent control of spin systems and single spin read-out using pristine oscillators have been demonstrated, temperature control of the motion of a macroscopic object using long-lived electronic spins has not been reported. Here, we observe both a spin-dependent torque and spin-cooling of the motion of a trapped microdiamond. Using a combination of microwave and laser excitation enables the spin of nitrogen-vacancy centers to act on the diamond orientation and to cool the diamond libration via a dynamical back-action. Further, driving the system in the non-linear regime, we demonstrate bistability and self-sustained coherent oscillations stimulated by the spin-mechanical coupling, which offers prospects for spin-driven generation of non-classical states of motion. Such a levitating diamond operated as a compass with controlled dissipation has implications in high-precision torque sensing, emulation of the spin-boson problem and probing of quantum phase transitions. In the single spin limit and employing ultra-pure nano-diamonds, it will allow quantum non-demolition read-out of the spin of nitrogen-vacancy centers under ambient conditions, deterministic entanglement between distant individual spins and matter-wave interferometry.Comment: New version with a calibration of angular resolution and sensitivity. Fig. 1 is also replaced to show an ODMR when the diamond is static to avoid spin-torque induced distortion

Thermodynamic approach to the dewetting instability in ultrathin films

The fluid dynamics of the classical dewetting instability in ultrathin films is a non-linear process. However, the physical manifestation of the instability in terms of characteristic length and time scales can be described by a linearized form of the initial conditions of the films's dynamics. Alternately, the thermodynamic approach based on equating the rate of free energy decrease to the viscous dissipation [de Gennes, C. R. Acad. Paris.v298, 1984] can give similar information. Here we have evaluated dewetting in the presence of thermocapillary forces arising from a film-thickness (h) dependent temperature. Such a situation can be found during pulsed laser melting of ultrathin metal films where nanoscale effects lead to a local h-dependent temperature. The thermodynamic approach provides an analytical description of this thermocapillary dewetting. The results of this approach agree with those from linear theory and experimental observations provided the minimum value of viscous dissipation is equated to the rate of free energy decrease. The flow boundary condition that produces this minimum viscous dissipation is when the film-substrate tangential stress is zero. The physical implication of this finding is that the spontaneous dewetting instability follows the path of minimum rate of energy loss.Comment: 8 pages, 3 figures. Under revie

Getting a Grip on the Transverse Motion in a Zeeman Decelerator

Zeeman deceleration is an experimental technique in which inhomogeneous, time-dependent magnetic fields generated inside an array of solenoid coils are used to manipulate the velocity of a supersonic beam. A 12-stage Zeeman decelerator has been built and characterized using hydrogen atoms as a test system. The instrument has several original features including the possibility to replace each deceleration coil individually. In this article, we give a detailed description of the experimental setup, and illustrate its performance. We demonstrate that the overall acceptance in a Zeeman decelerator can be significantly increased with only minor changes to the setup itself. This is achieved by applying a rather low, anti-parallel magnetic field in one of the solenoid coils that forms a temporally varying quadrupole field, and improves particle confinement in the transverse direction. The results are reproduced by three-dimensional numerical particle trajectory simulations thus allowing for a rigorous analysis of the experimental data. The findings suggest the use of a modified coil configuration to improve transverse focusing during the deceleration process.Comment: accepted by J. Chem. Phy

An alternative approach to efficient simulation of micro/nanoscale phonon transport

Starting from the recently proposed energy-based deviational formulation for solving the Boltzmann equation [J.-P. Peraud and N. G. Hadjiconstantinou, Phys. Rev. B 84, 2011], which provides significant computational speedup compared to standard Monte Carlo methods for small deviations from equilibrium, we show that additional computational benefits are possible in the limit that the governing equation can be linearized. The proposed method exploits the observation that under linearized conditions (small temperature differences) the trajectories of individual deviational particles can be decoupled and thus simulated independently; this leads to a particularly simple and efficient algorithm for simulating steady and transient problems in arbitrary three-dimensional geometries, without introducing any additional approximation.Comment: 4 pages, 2 figure

Relation between the High Density Phase and the Very-High Density Phase of Amorphous Solid Water

It has been suggested that high-density amorphous (HDA) ice is a structurally arrested form of high-density liquid (HDL) water, while low-density amorphous (LDA) ice is a structurally arrested form of low-density liquid (LDL) water. Recent experiments and simulations have been interpreted to support the possibility of a second "distinct" high-density structural state, named very high-density amorphous (VHDA) ice, questioning the LDL-HDL hypothesis. We test this interpretation using extensive computer simulations, and find that VHDA is a more stable form of HDA and that in fact VHDA should be considered as the amorphous ice of the quenched HDL.Comment: 5 pages, 4 fig

Coherent Population Trapping with a controlled dissipation: applications in optical metrology

We analyze the properties of a pulsed Coherent Population Trapping protocol that uses a controlled decay from the excited state in a $\Lambda$-level scheme. We study this problem analytically and numerically and find regimes where narrow transmission, absorption, or fluorescence spectral lines occur. We then look for optimal frequency measurements using these spectral features by computing the Allan deviation in the presence of ground state decoherence and show that the protocol is on a par with Ramsey-CPT. We discuss possible implementations with ensembles of alkali atoms and single ions and demonstrate that typical pulsed-CPT experiments that are realized on femto-second time-scales can be implemented on micro-seconds time-scales using this scheme.Comment: 9 pages, 7 figure

Pierre Auger Data, Photons, and Top-Down Cosmic Ray Models

We consider the ultra-high energy cosmic ray (UHECR) spectrum as measured by the Pierre Auger Observatory. Top-down models for the origin of UHECRs predict an increasing photon component at energies above about $10^{19.7}$eV. Here we present a simple prescription to compare the Auger data with a prediction assuming a pure proton component or a prediction assuming a changing primary component appropriate for a top-down model. We find that the UHECR spectrum predicted in top-down models is a good fit to the Auger data. Eventually, Auger will measure a composition-independent spectrum and will be capable of either confirming or excluding the quantity of photons predicted in top-down models.Comment: 8 pages, 3 figure

Spin-mechanics with levitating ferromagnetic particles

We propose and demonstrate first steps towards schemes where the librational mode of levitating ferromagnets is strongly coupled to the electronic spin of Nitrogen-Vacancy (NV) centers in diamond. Experimentally, we levitate ferromagnets in a Paul trap and employ magnetic fields to attain oscillation frequencies in the hundreds of kHz range with Q factors close to $10^4$. These librational frequencies largely exceed the decoherence rate of NV centers in typical CVD grown diamonds offering prospects for sideband resolved operation. We also prepare and levitate composite diamond-ferromagnet particles and demonstrate both coherent spin control of the NV centers and read-out of the particle libration using the NV spin. Our results will find applications in ultra-sensitive gyroscopy and bring levitating objects a step closer to spin-mechanical experiments at the quantum level.Comment: Lengthened to 11 pages. To appear in PR

A spectroscopic search for AGN activity in the reionization era

The ubiquity of Lyman alpha (Ly$\alpha$) emission in a sample of four bright [O III]-strong star-forming galaxies with redshifts above 7 has led to the suggestion that such luminous sources represent a distinct population compared to their fainter, more numerous, counterparts. The presence of Ly$\alpha$ emission within the reionization era could indicate that these sources created early ionized bubbles due to their unusually strong radiation, possibly due to the presence of active galactic nuclei. To test this hypothesis we have secured long integration spectra with XSHOOTER on the VLT for three $z\simeq$7 sources selected to have similar luminosities and prominent excess fluxes in the IRAC 3.6 or 4.5$\mu$m band, usually attributed to strong [O III] emission. We secured additional spectroscopy for one of these galaxies at $z$=7.15 using MOSFIRE at the Keck telescope. For this, the most well-studied source in our sample with the strongest IRAC excess, we detect prominent nebular emission from He II and NV indicative of a non-thermal source. For the other two sources at $z$=6.81 and $z$=6.85, for which no previous optical/near infrared spectroscopy was initially available, Ly$\alpha$ is seen in one and CIII] emission in the other. Although a modest sample, our results further support the hypothesis that the phenomenon of intense [O III] emission is associated preferentially with sources lying in early ionized bubbles. However, even though one of our sources at $z$=7.15 clearly indicates the presence of non-thermal radiation, such ionized bubbles may not uniquely arise in this manner. We discuss the unique advantages of extending such challenging diagnostic studies with JWST.Comment: 11 pages, 7 figures, submitted to Ap