7,819 research outputs found
High performance photonic microwave filters based on a 50GHz optical soliton crystal Kerr micro-comb
We demonstrate a photonic radio frequency (RF) transversal filter based on an
integrated optical micro-comb source featuring a record low free spectral range
of 49 GHz yielding 80 micro-comb lines across the C-band. This record-high
number of taps, or wavelengths for the transversal filter results in
significantly increased performance including a QRF factor more than four times
higher than previous results. Further, by employing both positive and negative
taps, an improved out-of-band rejection of up to 48.9 dB is demonstrated using
Gaussian apodization, together with a tunable centre frequency covering the RF
spectra range, with a widely tunable 3-dB bandwidth and versatile dynamically
adjustable filter shapes. Our experimental results match well with theory,
showing that our transversal filter is a competitive solution to implement
advanced adaptive RF filters with broad operational bandwidths, high frequency
selectivity, high reconfigurability, and potentially reduced cost and
footprint. This approach is promising for applications in modern radar and
communications systems.Comment: 19 pages, 12 figures, 107 reference
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Enabling Thin and Flexible Solid-State Composite Electrolytes by the Scalable Solution Process
All solid-state batteries (ASSBs) have the potential to deliver higher energy densities, wider operating temperature range, and improved safety compared with today's liquid-electrolyte-based batteries. However, of the various solid-state electrolyte (SSE) classes - polymers, sulfides, or oxides - none alone can deliver the combined properties of ionic conductivity, mechanical, and chemical stability needed to address scalability and commercialization challenges. While promising strategies to overcome these include the use of polymer/oxide or sulfide composites, there is still a lack of fundamental understanding between different SSE-polymer-solvent systems and its selection criteria. Here, we isolate various SSE-polymer-solvent systems and study their molecular level interactions by combining various characterization tools. With these findings, we introduce a suitable Li7P3S11SSE-SEBS polymer-xylene solvent combination that significantly reduces SSE thickness (∼50 μm). The SSE-polymer composite displays high room temperature conductivity (0.7 mS cm-1) and good stability with lithium metal by plating and stripping over 2000 h at 1.1 mAh cm-2. This study suggests the importance of understanding fundamental SSE-polymer-solvent interactions and provides a design strategy for scalable production of ASSBs
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Elucidating Reversible Electrochemical Redox of Li6PS5CI Solid Electrolyte
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Revealing Nanoscale Solid-Solid Interfacial Phenomena for Long-Life and High-Energy All-Solid-State Batteries.
Enabling long cyclability of high-voltage oxide cathodes is a persistent challenge for all-solid-state batteries, largely because of their poor interfacial stabilities against sulfide solid electrolytes. While protective oxide coating layers such as LiNbO3 (LNO) have been proposed, its precise working mechanisms are still not fully understood. Existing literature attributes reductions in interfacial impedance growth to the coating's ability to prevent interfacial reactions. However, its true nature is more complex, with cathode interfacial reactions and electrolyte electrochemical decomposition occurring simultaneously, making it difficult to decouple each effect. Herein, we utilized various advanced characterization tools and first-principles calculations to probe the interfacial phenomenon between solid electrolyte Li6PS5Cl (LPSCl) and high-voltage cathode LiNi0.85Co0.1Al0.05O2 (NCA). We segregated the effects of spontaneous reaction between LPSCl and NCA at the interface and quantified the intrinsic electrochemical decomposition of LPSCl during cell cycling. Both experimental and computational results demonstrated improved thermodynamic stability between NCA and LPSCl after incorporation of the LNO coating. Additionally, we revealed the in situ passivation effect of LPSCl electrochemical decomposition. When combined, both these phenomena occurring at the first charge cycle result in a stabilized interface, enabling long cyclability of all-solid-state batteries
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