The dynamics of a hole in a CuO_4 plaquette: electron energy-loss spectroscopy of Li_2CuO_2

We have measured the energy and momentum dependent loss function of Li_2CuO_2 single crystals by means of electron energy-loss spectroscopy in transmission. Using the same values for the model parameters, the low-energy features of the spectrum as well as published Cu 2p_(3/2) x-ray photoemission data of Li_2CuO_2 are well described by a cluster model that consists of a single CuO_4 plaquette only. This demonstrates that charge excitations in Li_2CuO_2 are strongly localized.Comment: 5 pages, 5 figure

Time-resolved investigation of magnetization dynamics of arrays of non-ellipsoidal nanomagnets with a non-uniform ground state

We have performed time-resolved scanning Kerr microscopy (TRSKM) measurements upon arrays of square ferromagnetic nano-elements of different size and for a range of bias fields. The experimental results were compared to micromagnetic simulations of model arrays in order to understand the non-uniform precessional dynamics within the elements. In the experimental spectra two branches of excited modes were observed to co-exist above a particular bias field. Below the so-called crossover field, the higher frequency branch was observed to vanish. Micromagnetic simulations and Fourier imaging revealed that modes from the higher frequency branch had large amplitude at the center of the element where the effective field was parallel to the bias field and the static magnetization. Modes from the lower frequency branch had large amplitude near the edges of the element perpendicular to the bias field. The simulations revealed significant canting of the static magnetization and the effective field away from the direction of the bias field in the edge regions. For the smallest element sizes and/or at low bias field values the effective field was found to become anti-parallel to the static magnetization. The simulations revealed that the majority of the modes were de-localized with finite amplitude throughout the element, while the spatial character of a mode was found to be correlated with the spatial variation of the total effective field and the static magnetization state. The simulations also revealed that the frequencies of the edge modes are strongly affected by the spatial distribution of the static magnetization state both within an element and within its nearest neighbors

Manifestation of spin-charge separation in the dynamic dielectric response of one--dimensional Sr2CuO3

We have determined the dynamical dielectric response of a one-dimensional, correlated insulator by carrying out electron energy-loss spectroscopy on Sr2CuO3 single crystals. The observed momentum and energy dependence of the low-energy features, which correspond to collective transitions across the gap, are well described by an extended one-band Hubbard model with moderate nearest neighbor Coulomb interaction strength. An exciton-like peak appears with increasing momentum transfer. These observations provide experimental evidence for spin-charge separation in the relevant excitations of this compound, as theoretically expected for the one-dimensional Hubbard model.Comment: RevTex, 4 pages+2 figures, to appear in PRL (July 13

Resonant inelastic x-ray scattering in one-dimensional copper oxides

The Cu K-edge resonant inelastic x-ray scattering (RIXS) spectrum in one-dimensional insulating cuprates is theoretically examined by using the exact diagonalization technique for the extended one-dimensional Hubbard model with nearest neighbor Coulomb interaction. We find the following characteristic features that can be detectable by RIXS experiments: (i) The spectrum with large momentum transfer indicates the formation of excitons, i.e., bound states of holon and doublon. (ii) The spectrum with small momentum transfer depends on the incident photon energy. We propose that the RIXS provides a unique opportunity to study the upper Hubbard band in one-dimensional cuprates.Comment: 3 pages with 4 figures, minor changes, to appear in Phys.Rev.

Nonlinear Optical Response in two-dimensional Mott Insulators

We study the third-order nonlinear optical susceptibility $\chi^{(3)}$ and photoexcited states of two-dimensional (2D) Mott insulators by using an effective model in the strong-coupling limit of a half-filled Hubbard model. In the numerically exact diagonalization calculations on finite-size clusters, we find that the coupling of charge and spin degrees of freedom plays a crucial role in the distribution of the dipole-allowed states with odd parity and the dipole-forbidden states with even parity in the photoexcited states. This is in contrast with the photoexcited states in one dimension, where the charge and spin degrees of freedom are decoupled. In the third-harmonic generation (THG) spectrum, main contribution is found to come from the process of three-photon resonance associated with the odd-parity states. As a result, the two-photon resonance process is less pronounced in the THG spectrum. The calculated THG spectrum is compared with recent experimental data. We also find that $\chi^{(3)}$ with cross-polarized configuration of pump and probe photons shows spectral distributions similar to $\chi^{(3)}$ with co-polarized configuration, although the weight is small. These findings will help the analyses of the experimental data of $\chi^{(3)}$ in the 2D Mott insulators.Comment: 9 pages,5 figures,RevTeX

Resonant enhancement of damping within the free layer of a microscale magnetic tunnel valve

Copyright © 2015 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article appeared in Journal of Applied Physics Vol. 117, article 17B301 and may be found at http://dx.doi.org/10.1063/1.4907701Picosecond magnetization dynamics in the free and pinned layers of a microscale magnetic tunnel valve have been studied using time-resolved scanning Kerr microscopy. A comparison of the observed dynamics with those of individual free and pinned layers allowed the effect of interlayer coupling to be identified. A weak interlayer coupling in the tunnel valve continuous film reference sample was detected in bulk magnetometry measurements, while focused Kerr magnetometry showed that the coupling was well maintained in the patterned structure. In the tunnel valve, the free layer precession was observed to have reduced amplitude and an enhanced relaxation. During magnetization reversal in the pinned layer, its frequency approached that of the low frequency mode associated with the free layer. At the pinned layer switching field, the linewidth of the free layer became similar to that of the pinned layer. The similarity in their frequencies promotes the formation of precessional modes that exhibit strong collective properties such as frequency shifting and enhanced linewidth, while inhomogeneous magnetization of the pinned layer during reversal may also play a role in these observations. The collective character of precessional dynamics associated with mixing of the free and pinned layer magnetization dynamics must be accounted for even in tunnel valves with a small interlayer coupling.Engineering and Physical Sciences Research Council (EPSRC)European Community's Seventh Framework Programme (FP7/2007-2013

Imaging small-amplitude magnetization dynamics in a longitudinally magnetized microwire

Copyright © 2008 The American Physical SocietyWe have used time-resolved scanning Kerr microscopy to study spin waves in a magnetic microwire subjected to a bias magnetic field applied parallel to its long axis. The spin-wave spectra obtained from different points near one end of the wire reveal several normal modes. We found that modes of a higher frequency occupied regions located further from the end of the wire. This was interpreted in terms of the confinement of the spin-wave modes by a nonuniform demagnetizing field. Furthermore, at a particular distance from the end of the wire, two or more modes occupying different regions along the width of the wire were observed. This was interpreted in terms of the confinement of the spin-wave modes due to an asymmetric variation in the local angle between the static magnetization and the effective direction of the wave vector of the confined modes. Images of the dynamic magnetization that are acquired at fixed pump-probe time delays revealed stripes lying perpendicular to the long axis of the wire and, hence, to the applied magnetic field. We interpret the stripe pattern in terms of a collective mode of the quasiperiodic system of ripple domains existing within the polycrystalline sample. Cur results give an additional insight into the connection between the nonuniform static magnetic state in small magnetic elements and their precessional dynamics, which is fundamentally important for the design of future high-speed switching and spin-wave logic devices of magnonics

Nonlinear optical response and spin-charge separation in one-dimensional Mott insulators

We theoretically study the nonlinear optical response and photoexcited states of the Mott insulators. The nonlinear optical susceptibility \chi^(3) is calculated by using the exact diagonalization technique on small clusters. From the systematic study of the dependence of \chi^(3) on dimensionality, we find that the spin-charge separation plays a crucial role in enhancing \chi^(3) in the one-dimensional (1D) Mott insulators. Based on this result, we propose a holon-doublon model, which describes the nonlinear response in the 1D Mott insulators. These findings show that the spin-charge separation will become a key concept of optoelectronic devices.Comment: 5 pages with 3 figures, to appear in PRB RC, 15 August 200

Oxygen Moment Formation and Canting in Li2CuO2

The possibilities of oxygen moment formation and canting in the quasi-1D cuprate Li2CuO2 are investigated using single crystal neutron diffraction at 2 K. The observed magnetic intensities could not be explained without the inclusion of a large ordered oxygen moment of 0.11(1) Bohr magnetons. Least-squares refinement of the magnetic structure of Li2CuO2 in combination with a spin-density Patterson analysis shows that the magnetization densities of the Cu and O atoms are highly aspherical, forming quasi-1D ribbons of localised Cu and O moments. Magnetic structure refinements and low-field magnetization measurements both suggest that the magnetic structure of Li2CuO2 at 2 K may be canted. A possible model for the canted configuration is proposed.Comment: 10 pages, 8 figures (screen resolution