Electron Clusters in Inert Gases

The paper addresses counterintuitive behavior of electrons injected into dense cryogenic media with negative scattering length $a_0$. Instead of expected polaronic effect (formation of density enhancement clusters) which should substantially reduce the electron mobility, an opposite picture is observed: with increasing $|a_0|$ (the trend taking place for inert gases with the growth of atomic number) and the medium density, the electrons remain practically free. An explanation of this behaviour is provided based on consistent accounting for the non-linearity of electron interaction with the gaseous medium in the gas atom number density

On the Teleportation of Continuous Variable

The measurement procedures used in quantum teleportation are analyzed from the viewpoint of the general theory of quantum-mechanical measurements. It is shown that to find the teleported state one should only know the identity resolution (positive operator-valued measure) generated by the corresponding instrument (quantum operation describing the system state change caused by the measurement) rather than the instrument itself. A quantum teleportation protocol based on a measurement associated with a non-orthogonal identity resolution is proposed for a system with non-degenerate continuous spectrum.Comment: 13 pages, no figures. To be published in JET

Relativistic quantum coin tossing

A relativistic quantum information exchange protocol is proposed allowing two distant users to realize ``coin tossing'' procedure. The protocol is based on the point that in relativistic quantum theory reliable distinguishing between the two orthogonal states generally requires a finite time depending on the structure of these states.Comment: 6 pages, no figure

Magnetoplasmon excitations in arrays of circular and noncircular quantum dots

We have investigated the magnetoplasmon excitations in arrays of circular and noncircular quantum dots within the Thomas-Fermi-Dirac-von Weizs\"acker approximation. Deviations from the ideal collective excitations of isolated parabolically confined electrons arise from local perturbations of the confining potential as well as interdot Coulomb interactions. The latter are unimportant unless the interdot separations are of the order of the size of the dots. Local perturbations such as radial anharmonicity and noncircular symmetry lead to clear signatures of the violation of the generalized Kohn theorem. In particular, the reduction of the local symmetry from SO(2) to $C_4$ results in a resonant coupling of different modes and an observable anticrossing behaviour in the power absorption spectrum. Our results are in good agreement with recent far-infrared (FIR) transmission experiments.Comment: 25 pages, 6 figures, typeset in RevTe

Relativistic Restrictions on the Distinguishability of Orthogonal Quantum States

We analyze the restrictions on the distinguishability of quantum states imposed by special relativity. An explicit expression relating the error probability for distinguishing between two orthogonal single-photon states with the time $T$ elapsed from the start of the measurement procedure until the measurement result is obtained by the observer.Comment: 9 pages, 1 figure (misprints in formulas corrected

Transport properties of copper phthalocyanine based organic electronic devices

Ambipolar charge carrier transport in Copper phthalocyanine (CuPc) is studied experimentally in field-effect transistors and metal-insulator-semiconductor diodes at various temperatures. The electronic structure and the transport properties of CuPc attached to leads are calculated using density functional theory and scattering theory at the non-equilibrium Green's function level. We discuss, in particular, the electronic structure of CuPc molecules attached to gold chains in different geometries to mimic the different experimental setups. The combined experimental and theoretical analysis explains the dependence of the mobilityand the transmission coefficient on the charge carrier type (electrons or holes) and on the contact geometry. We demonstrate the correspondence between our experimental results on thick films and our theoretical studies of single molecule contacts. Preliminary results for fluorinated CuPc are discussed.Comment: 18 pages, 16 figures; to be published in Eur. Phys. J. Special Topic

Spontaneous Coherence and Collective Modes in Double-Layer Quantum Dot Systems

We study the ground state and the collective excitations of parabolically-confined double-layer quantum dot systems in a strong magnetic field. We identify parameter regimes where electrons form maximum density droplet states, quantum-dot analogs of the incompressible states of the bulk integer quantum Hall effect. In these regimes the Hartree-Fock approximation and the time-dependent Hartree-Fock approximations can be used to describe the ground state and collective excitations respectively. We comment on the relationship between edge excitations of dots and edge magneto-plasmon excitations of bulk double-layer systems.Comment: 20 pages (figures included) and also available at http://fangio.magnet.fsu.edu/~jhu/Paper/qdot_cond.ps, replaced to fix figure

Green function techniques in the treatment of quantum transport at the molecular scale

The theoretical investigation of charge (and spin) transport at nanometer length scales requires the use of advanced and powerful techniques able to deal with the dynamical properties of the relevant physical systems, to explicitly include out-of-equilibrium situations typical for electrical/heat transport as well as to take into account interaction effects in a systematic way. Equilibrium Green function techniques and their extension to non-equilibrium situations via the Keldysh formalism build one of the pillars of current state-of-the-art approaches to quantum transport which have been implemented in both model Hamiltonian formulations and first-principle methodologies. We offer a tutorial overview of the applications of Green functions to deal with some fundamental aspects of charge transport at the nanoscale, mainly focusing on applications to model Hamiltonian formulations.Comment: Tutorial review, LaTeX, 129 pages, 41 figures, 300 references, submitted to Springer series "Lecture Notes in Physics

Gravitational Waves from Gravitational Collapse

Gravitational wave emission from the gravitational collapse of massive stars has been studied for more than three decades. Current state of the art numerical investigations of collapse include those that use progenitors with realistic angular momentum profiles, properly treat microphysics issues, account for general relativity, and examine non--axisymmetric effects in three dimensions. Such simulations predict that gravitational waves from various phenomena associated with gravitational collapse could be detectable with advanced ground--based and future space--based interferometric observatories.Comment: 68 pages including 13 figures; revised version accepted for publication in Living Reviews in Relativity (http://www.livingreviews.org

Orbital redistribution in molecular nanostructures mediated by metal-organic bonds

Dicyanovinyl-quinquethiophene (DCV5T-Me) is a prototype conjugated oligomer for highly efficient organic solar cells. This class of oligothiophenes are built up by an electron-rich donor (D) backbone and terminal electron-deficient acceptor (A) moieties. Here, we investigated its structural and electronic properties when it is adsorbed on a Au(111) surface using low temperature scanning tunneling microscopy/spectroscopy (STM/STS) and atomic force microscopy (AFM). We find that DCV5T-Me self-assembles in extended chains, stabilized by intercalated Au atoms. The effect of metal-ligand hybridization with Au adatoms causes an energetic downshift of the DCV5T-Me lowest unoccupied molecular orbital (LUMO) with respect to the uncoordinated molecules on the surface. The asymmetric coordination of a gold atom to only one molecular end group leads to an asymmetric localization of the LUMO and LUMO+1 states at opposite sides. Using model density functional theory (DFT) calculations, we explain such orbital reshaping as a consequence of linear combinations of the original LUMO and LUMO+1 orbitals, mixed by the attachment of a bridging Au adatom. Our study shows that the alignment of molecular orbitals and their distribution within individual molecules can be modified by contacting them to metal atoms in specific sites