Application of Optimal Interpolation to Spatially and Temporally Sparse Observations of Aerosol Optical Depth

Aerosol optical depth (AOD) is one of the basic characteristics of atmospheric aerosol. A global ground-based network of sun and sky photometers, the Aerosol Robotic Network (AERONET) provides AOD data with low uncertainty. However, AERONET observations are sparse in space and time. To improve data density, we merged AERONET observations with a GEOS-Chem chemical transport model prediction using an optimal interpolation (OI) method. According to OI, we estimated AOD as a linear combination of observational data and a model forecast, with weighting coefficients chosen to minimize a mean-square error in the calculation, assuming a negligible error of AERONET AOD observations. To obtain weight coefficients, we used correlations between model errors in different grid points. In contrast with classical OI, where only spatial correlations are considered, we developed the spatial-temporal optimal interpolation (STOI) technique for atmospheric applications with the use of spatial and temporal correlation functions. Using STOI, we obtained estimates of the daily mean AOD distribution over Europe. To validate the results, we compared daily mean AOD estimated by STOI with independent AERONET observations for two months and three sites. Compared with the GEOS-Chem model results, the averaged reduction of the root-mean-square error of the AOD estimate based on the STOI method is about 25%. The study shows that STOI provides a significant improvement in AOD estimates

Application of Optimal Interpolation to Spatially and Temporally Sparse Observations of Aerosol Optical Depth

Aerosol optical depth (AOD) is one of the basic characteristics of atmospheric aerosol. A global ground-based network of sun and sky photometers, the Aerosol Robotic Network (AERONET) provides AOD data with low uncertainty. However, AERONET observations are sparse in space and time. To improve data density, we merged AERONET observations with a GEOS-Chem chemical transport model prediction using an optimal interpolation (OI) method. According to OI, we estimated AOD as a linear combination of observational data and a model forecast, with weighting coefficients chosen to minimize a mean-square error in the calculation, assuming a negligible error of AERONET AOD observations. To obtain weight coefficients, we used correlations between model errors in different grid points. In contrast with classical OI, where only spatial correlations are considered, we developed the spatial-temporal optimal interpolation (STOI) technique for atmospheric applications with the use of spatial and temporal correlation functions. Using STOI, we obtained estimates of the daily mean AOD distribution over Europe. To validate the results, we compared daily mean AOD estimated by STOI with independent AERONET observations for two months and three sites. Compared with the GEOS-Chem model results, the averaged reduction of the root-mean-square error of the AOD estimate based on the STOI method is about 25%. The study shows that STOI provides a significant improvement in AOD estimates

Spatio-Temporal Optimal Interpolation of Aerosol Optical Depth Observations Using a Chemical Transport Model

To estimate the spatial and temporal distribution of aerosol optical depth (AOD), we used the optimal interpolation (OI). In OI, observational data and a model forecast are linearly combined according to their relative accuracies. Weight coefficients are chosen to minimize the mean-square error in the estimate. To obtain weight coefficients, correlations between model errors in the different grid points are used. In classical OI, only spatial correlations are considered. We used spatial and temporal correlation functions. To obtain error statistics, we used observations from European stations of ground-based sun photometers, the Aerosol Robotic Network (AERONET), and simulations by a chemical transport model GEOS-Chem, assuming a negligible error of AERONET AOD observations. The estimates of the daily mean AOD distribution over Europe are obtained. The reduction of the root-mean-square error of the AOD estimate based on the OI method in comparison with the GEOS-Chem model results is discussed

Spring 2020 Atmospheric Aerosol Contamination over Kyiv City

Extraordinarily high aerosol contamination was observed in the atmosphere over the city of Kyiv, Ukraine, during the March–April 2020 period. The source of contamination was the large grass and forest fires in the northern part of Ukraine and the Kyiv region. The level of PM2.5 load was investigated using newly established AirVisual sensor mini-networks in five areas of the city. The aerosol data from the Kyiv AERONET sun-photometer site were analyzed for that period. Aerosol optical depth, Ångström exponent, and the aerosol particles properties (particle size distribution, single-scattering albedo, and complex refractive index) were analyzed using AERONET sun-photometer observations. The smoke particles observed at Kyiv site during the fires in general correspond to aerosol with optical properties of biomass burning aerosol. The variability of the optical properties and chemical composition indicates that the aerosol particles in the smoke plumes over Kyiv city were produced by different burning materials and phases of vegetation fires at different times. The case of enormous PM2.5 aerosol contamination in the Kyiv city reveals the need to implement strong measures for forest fire control and prevention in the Kyiv region, especially in its northwest part, where radioactive contamination from the Chernobyl disaster is still significant

Integrated Ground-Based and Satellite Remote Sensing of the Earth’s Surface and Atmosphere in East and West Antarctica with Lidar and Radiometric Systems

We have developed remote ground-based and satellite methods and hardware and software for studying atmospheric aerosols, clouds, and the underlying surface in Eastern and Western Antarctica. The ground-based equipment includes: (1) a CIMEL solar spectrum photometer, which measures the spectrum of solar radiation transmitted and scattered by the atmosphere, (2) a multi-wavelength Raman lidar, which measures the vertical backscatter profile, (3) an albedometer, which measures the spectral albedo of the surface, primarily snow, and (4) a reflectometer, which measures the directional spectral reflectance of snow. The ground-based measurement data were integrated with data from satellite radiometers MODIS or OLCI and the satellite lidar CALIOP. A synergy of the manifold data results in retrieval of various atmosphere and surface characteristics such as the aerosol optical depth, profiles of concentration of the fine and coarse aerosol fractions, spatial distribution of the effective snow grain size, fraction of outcrops, etc

Spring 2020 Atmospheric Aerosol Contamination over Kyiv City

International audienceExtraordinarily high aerosol contamination was observed in the atmosphere over the city of Kyiv, Ukraine, during the March–April 2020 period. The source of contamination was the large grass and forest fires in the northern part of Ukraine and the Kyiv region. The level of PM2.5 load was investigated using newly established AirVisual sensor mini-networks in five areas of the city. The aerosol data from the Kyiv AERONET sun-photometer site were analyzed for that period. Aerosol optical depth, Ångström exponent, and the aerosol particles properties (particle size distribution, single-scattering albedo, and complex refractive index) were analyzed using AERONET sun-photometer observations. The smoke particles observed at Kyiv site during the fires in general correspond to aerosol with optical properties of biomass burning aerosol. The variability of the optical properties and chemical composition indicates that the aerosol particles in the smoke plumes over Kyiv city were produced by different burning materials and phases of vegetation fires at different times. The case of enormous PM2.5 aerosol contamination in the Kyiv city reveals the need to implement strong measures for forest fire control and prevention in the Kyiv region, especially in its northwest part, where radioactive contamination from the Chernobyl disaster is still significant

Synergetic observations by ground-based and space lidar systems and aeronet sun-radiometers: a step to advanced regional monitoring of large scale aerosol changes

The financial support by the European Union's Horizon 2020 research and innovation program (ACTRIS-2, grant agreement no. 654109) is gratefully acknowledged. The investigation was supported by the Belarusian Republican Foundation for Fundamental, Research Agreement No. F18EA-011, by the Russian Foundation for Basic Research (grant No. 18-55-81001), and also by Vietnam Academy of Science and Technology (project code QTRU05.01/18-20). The Portuguese team acknowledges the support from the Portuguese Science Foundation, in the frame of the European Regional Development Fund -COMPETE 2020, under the projects UID/GEO/04683/2013 (POCI-01-0145-FEDER-007690)The paper presents the preliminary results of the lidar&radiometer measurement campaign (LRMC2017), estimation of statistical relations between aerosol mode concentrations retrieved from CALIOP and ground-based lidar stations and case study of fire smoke events in the Eurasian regions using combined ground-based and space lidar and radiometer observations.European Union's Horizon 2020 research and innovation program (ACTRIS-2) 654109Belarusian Republican Foundation for Fundamental, Research F18EA-011Russian Foundation for Basic Research (RFBR) 18-55-81001Vietnam Academy of Science and Technology QTRU05.01/18-20Portuguese Science Foundation, in the frame of the European Regional Development Fund -COMPETE 2020 UID/GEO/04683/2013 (POCI-01-0145-FEDER-007690