Stable operation of a synchronously pumped colliding-pulse mode-locked ring dye laser

Pulses of 100-fsec duration are obtained by synchronous pumping of a colliding-pulse ring dye laser with a mode-locked Ar+-ion laser. Stable operation of the synchronously pumped colliding-pulse mode-locked laser over hours was obtained by a suitable choice of the distance between the gain and the absorber in combination with an appro-priate pump-pulse sequence. Passive mode locking of a ring dye laser by the inter-action of two counterpropagating pulses in a thin sat-urable absorber (colliding-pulse mode locking) yields femtosecond laser pulses. ' In these lasers the gain medium (Rhodamine 6G) is pumped by a cw Ar+-ion laser. The saturable absorber (DODCI, 3,3-diethyl-oxadicarbocyanine iodide) synchronizes two counter-propagating pulses meeting in the absorber jet stream. The colliding pulses form a transient grating, which synchronizes and stabilizes the pulses.2 In order to ensure equal amplification for both counterpropagatin

Femtosecond spectroscopy of the first events of the photochemical cycle in bacteriorhodopsin

The first steps in the photochemistry of bacteriorhodopsin (BR) are investigated with light pulses of 160 fs duration. Four samples are studied: (i) the purple membrane, (ii) deuterated purple membrane, (iii) BR trimers and (iv) BR monomers. In all samples the first intermediate J is formed within 430±50 fs. No isotope effect is observed in the formation of J upon deuteration, in contrast to previous reports with much higher excitation energies. Thus proton movement to or from the retinal Schiff's base is not relevant during the first step. Comparing the data for trimeric and monomeric BR suggests an upper limit of 50 fs for the transfer of excitation energy from the excitonically coupled trimer to a single retinal chromophore

Time-variant linear pulse processing

Cataloged from PDF version of article.Previously suggested systems for linear processing of temporal pulses are limited to time-invariant (convolution-type) operations. Although these are the most general operations possible with passive components, we show that by using nonlinear optical interactions, arbitrary linear operations can be performed. Such operations may be useful for performing time-variant analog signal processing, temporal matrix-vector multiplication, and time-slot interchange of pulses for digital communications systems

Magnetotransport in Sr3PbO antiperovskite with three-dimensional massive Dirac electrons

Novel topological phenomena are anticipated for three-dimensional (3D) Dirac electrons. The magnetotransport properties of cubic ${\rm Sr_{3}PbO}$ antiperovskite, theoretically proposed to be a 3D massive Dirac electron system, are studied. The measurements of Shubnikov-de Haas oscillations and Hall resistivity indicate the presence of a low density ($\sim 1 \times 10^{18}$ ${\rm cm^{-3}}$) of holes with an extremely small cyclotron mass of 0.01-0.06$m_{e}$. The magnetoresistance $\Delta\rho_{xx}(B)$ is linear in magnetic field $B$ with the magnitude independent of temperature. These results are fully consistent with the presence of 3D massive Dirac electrons in ${\rm Sr_{3}PbO}$. The chemical flexibility of the antiperovskites and our findings in the family member, ${\rm Sr_{3}PbO}$, point to their potential as a model system in which to explore exotic topological phases