20 research outputs found
Linewidth of single photon transitions in Mn-acetate
We use time-domain terahertz spectroscopy to measure the position and
linewidth of single photon transitions in Mn-acetate. This linewidth is
compared to the linewidth measured in tunneling experiments. We conclude that
local magnetic fields (due to dipole or hyperfine interactions) cannot be
responsible for the observed linewidth, and suggest that the linewidth is due
to variations in the anisotropy constants for different clusters. We also
calculate a lower limit on the dipole field distribution that would be expected
due to random orientations of clusters and find that collective effects must
narrow this distribution in tunneling measurements.Comment: 5 pages, accepted to Physical Review
Spin-parity dependent tunneling of magnetization in single-molecule magnets
Single-molecule magnets facilitate the study of quantum tunneling of
magnetization at the mesoscopic level. The spin-parity effect is among the
fundamental predictions that have yet to be clearly observed. It is predicted
that quantum tunneling is suppressed at zero transverse field if the total spin
of the magnetic system is half-integer (Kramers degeneracy) but is allowed in
integer spin systems. The Landau-Zener method is used to measure the tunnel
splitting as a function of transverse field. Spin-parity dependent tunneling is
established by comparing the transverse field dependence of the tunnel
splitting of integer and half-integer spin systems.Comment: 4 pages, 6 figure