Harmonics generation in electron-ion collisions in a short laser pulse

Anomalously high generation efficiency of coherent higher field-harmonics in collisions between {\em oppositely charged particles} in the field of femtosecond lasers is predicted. This is based on rigorous numerical solutions of a quantum kinetic equation for dense laser plasmas which overcomes limitations of previous investigations.Comment: 4 pages, 4 eps-figures include

Introduction to Configuration Path Integral Monte Carlo

In low-temperature high-density plasmas quantum effects of the electrons are becoming increasingly important. This requires the development of new theoretical and computational tools. Quantum Monte Carlo methods are among the most successful approaches to first-principle simulations of many-body quantum systems. In this chapter we present a recently developed method---the configuration path integral Monte Carlo (CPIMC) method for moderately coupled, highly degenerate fermions at finite temperatures. It is based on the second quantization representation of the $N$-particle density operator in a basis of (anti-)symmetrized $N$-particle states (configurations of occupation numbers) and allows to tread arbitrary pair interactions in a continuous space. We give a detailed description of the method and discuss the application to electrons or, more generally, Coulomb-interacting fermions. As a test case we consider a few quantum particles in a one-dimensional harmonic trap. Depending on the coupling parameter (ratio of the interaction energy to kinetic energy), the method strongly reduces the sign problem as compared to direct path integral Monte Carlo (DPIMC) simulations in the regime of strong degeneracy which is of particular importance for dense matter in laser plasmas or compact stars. In order to provide a self-contained introduction, the chapter includes a short introduction to Metropolis Monte Carlo methods and the second quantization of quantum mechanics.Comment: chapter in book "Introduction to Complex Plasmas: Scientific Challenges and Technological Opportunities", Michael Bonitz, K. Becker, J. Lopez and H. Thomsen (Eds.) Springer Series "Atomic, Optical and Plasma Physics", vol. 82, Springer 2014, pp. 153-194 ISBN: 978-3-319-05436-0 (Print) 978-3-319-05437-7 (Online

Near-shore permafrost degradation in Siberia

Ice-rich permafrost coasts in the Arctic are susceptible to a variety of changing environmental factors, all of which currently point to increasing coastal erosion rates and mass fluxes of sediment and carbon to the shallow arctic shelf seas. Coastal erosion and flooding inundate terrestrial permafrost with seawater and create submarine permafrost. Permafrost begins to warm under marine conditions, which can destabilize the sea floor and may release greenhouse gases. The rate and spatial distribution of subsea permafrost degradation in the Laptev, East Siberian and Chukchi seas, which together comprise more than half of the Arctic Ocean continental shelf, remain poorly explored. We report on the transition of terrestrial to subsea permafrost at four coastal sites in the Laptev Sea: Cape Mamontov Klyk in the western Laptev Sea, and Buor Khaya Peninsula, Muostakh Island and the Bykovsky Peninsula in the central Laptev Sea. We use coastal erosion rates from about the last 70 years to estimate the period of inundation at these sites. Combined with direct (drilling and temperature) and indirect (geophysical) observations of thaw depths of ice-bonded permafrost, we estimate recent degradation rates of permafrost over the past centuries. Based on these observations, the unfrozen sediment layer overlying ice-bonded permafrost increased from less than a meter at the shoreline to over 30 m below seabed with increasing distance from the shoreline at our study sites, with high spatial variability between and within sites. Observed temperatures of the sediment ranged from -5 °C to positive temperatures. In coastal sediments, it is difficult to establish an age-depth model, making corroboration of estimated degradation rates a challenge. Nonetheless, as the thickness of the unfrozen sediment layer increases over time, the vertical thermal and salt concentration gradients decrease, slowing the downward heat and mass fluxes responsible for degradation. High sedimentation rates and ice contents probably stabilize subsea permafrost. We suggest that permafrost degradation relevant to gas flow is likely to have occurred where permafrost warmed prior to inundation

An orbital-free molecular dynamics study of melting in K_20, K_55, K_92, K_142, Rb_55 and Cs_55 clusters

The melting-like transition in potasium clusters K_N, with N=20, 55, 92 and 142, is studied by using an orbital-free density-functional constant-energy molecular dynamics simulation method, and compared to previous theoretical results on the melting-like transition in sodium clusters of the same sizes. Melting in potasium and sodium clusters proceeds in a similar way: a surface melting stage develops upon heating before the homogeneous melting temperature is reached. Premelting effects are nevertheless more important and more easily established in potasium clusters, and the transition regions spread over temperature intervals which are wider than in the case of sodium. For all the sizes considered, the percentage melting temperature reduction when passing from Na to K clusters is substantially larger than in the bulk. Once those two materials have been compared for a number of different cluster sizes, we study the melting-like transition in Rb_55 and Cs_55 clusters and make a comparison with the melting behavior of Na_55 and K_55. As the atomic number increases, the height of the specific heat peaks decreases, their width increases, and the melting temperature decreases as in bulk melting, but in a more pronounced way.Comment: LaTeX file. 6 pages with 17 pictures. Final version with minor change

Renormalized Coupled Cluster Approaches in the Cluster-in-Molecule Framework: Predicting Vertical Electron Binding Energies of the Anionic Water Clusters (H2O)n–

Anionic water clusters are generally considered to be extremely challenging to model using fragmentation approaches due to the diffuse nature of the excess electron distribution. The local correlation coupled cluster (CC) framework cluster-in-molecule (CIM) approach combined with the completely renormalized CR-CC(2,3) method [abbreviated CIM/CR-CC(2,3)] is shown to be a viable alternative for computing the vertical electron binding energies (VEBE). CIM/CR-CC(2,3) with the threshold parameter ζ set to 0.001, as a trade-off between accuracy and computational cost, demonstrates the reliability of predicting the VEBE, with an average percentage error of ∼15% compared to the full ab initio calculation at the same level of theory. The errors are predominantly from the electron correlation energy. The CIM/CR-CC(2,3) approach provides the ease of a black-box type calculation with few threshold parameters to manipulate. The cluster sizes that can be studied by high-level ab initio methods are significantly increased in comparison with full CC calculations. Therefore, the VEBE computed by the CIM/CR-CC(2,3) method can be used as benchmarks for testing model potential approaches in small-to-intermediate-sized water clusters